NUCLEAR SPINS AND MOMENTS OF THE ACTINIDES

APPENDIX I

NUCLEAR SPINS AND MOMENTS OF THE

ACTINIDES John C. Conway

The table lists the element and atomic mass in the first two columns. The nuclear spin (I) is in column 3. The magnetic dipole moment (J.t) in units of nuclear magnetons is in column 4. The spectroscopic electric quadrupole moment (Q) in units of barns is in column 5.

There are several references where this information has been tabulated and reference to the original work may be found. Nuclear Spins and Moments by G. H. Fuller and V. W. Cohen, Nuclear Data Tables, 5, 433 (1969) contains data for all the elements. A later compilation by S. Gerstenkorn, J. Physique, 34, 55 (1973) entitled Nuclear Properties Deduced from the Optical Spectra of the Atoms, Nuclear Moments and Isotope Shift of the Actinide and Rare Earth Series, lists the data through 1973. A report Table of Nuclear Moments by V. S. Shirley and C. M. Lederer, Lawrence Berkeley Laboratory, LBL-3450 (Dec. 1974) is a listing of all the elements. They have made corrections to the magnetic dipole moments based on a revised proton moment and have also corrected for diamagnetic shielding.

There are two later references to work since 1974. The spin and moment of 249Cfis from N. Edelstein and D. G. Karraker, J. Chem. Phys. 62, 938 (1975). The data for 253Es and 254mEs are from L. S. Goodman, H. Diamond and H. E. Stanton, Phys. Rev. 11, 499 (1975). The sign of the nuclear moment of 249Cf is negative (J. Blaise, private communication, 1979).

1647

Electric Nuclear magnetic quadrupole

Nuclear moment p. (nuclear moment Q Element A spin I magnetons) (barns)

Actinium 227 3/2 +1.1 ±0.1 +1.7±0.2 Thorium 229 5/2 +0.44 ± 0.05 +4.9±0.5 Protactinium 231 3/2 +1.98 -3.0 Protactinium 233 3/2 +3.4 Uranium 233 5/2 +0.49±0.05 +4.9 ±0.5 Uranium 235 7/2 -0.31 ±0.03 +6.4±0.7 Neptunium 237 5/2 +2.9 +5.0 Neptunium 238 2 Neptunium 239 5/2 Plutonium 239 1/2 + 0.200 ± 0.004 Plutonium 241 5/2 -0.72±0.02 +5.6±0.6 Americium 241 5/2 +1.59±0.03 +4.9 Americium 242 1 +0.382 -2.74 Americium 243 5/2 +1.59±0.03 +4.9 Curium 243 5/2 0.40 Curium 245 7/2 0.5 ±0.1 Curium 247 9/2 0.36 Berkelium 249 7/2 2.2±0.4 +5.79 Californium 249 9/2 -0.28±0.06 Einsteinium 253 7/2 4.10 ± 0.07 6.13 Einsteinium 254m 2 2.87 3.39

APPENDIX II

NUCLEAR PROPERTIES OF ACTINIDE NUCLIDES

Irshad Ahmad and Paul R. Fields

DISCUSSION

In this appendix we first present a brief and elementary discussion of the nuclear properties of heavy elements, mainly for the benefit of those readers who have no previous orientation in nuclear chemistry. For a more detailed understanding of this subject, the reader should refer to a nuclear chemistry textbook [1, 2] and for information on nuclear data he or she should consult the Table of Isotopes [3], or the Table of Radioactive Isotopes [4].

All nuclei in the actinide region are unstable towards (X decay. A few actinide nuclides are stable to {J decay, but because of (X decay they are radioactive. Thus there are no stable actinide nuclides. The higher-Z elements also decay by spontaneous fission; in particular, 248Cm and 252Cf have significant fission branching.

The most common mode of disintegration for actinide nuclei is by the emission of (X particles (4He ions). Alpha decay energies are known [3-5] for most nuclides and they can also be calculated from known atomic masses [6]. This decay process produces daughter nuclei that are two less in atomic number and have four less atomic mass units than the parent nuclei. During (X decay, about 2 % of the available decay energy is imparted to the recoiling daughter nucleus and the remainder is carried ofT by the fast-moving (X particles. Several groups of (X

particles, each with a definite energy, are emitted in most (X decay processes. For actinide nuclides, (X decay energies range from about 4 to about 11 MeV. As a general rule, (X decay energy increases with increasing Z and for a given element it decreases with increasing mass number.

The (X decay half-life of a nucleus decreases exponentially with increasing decay energy. As a rough guide every 50 keV decrease in the decay energy increases the half-life by a factor of about 2. One useful quantity that facilitates the understanding of the mechanism of the (X decay process is the hindrance factor. It is defined as the ratio of the experimental partial half-life to the theoretical halflife calculated on the assumption that the (X particle pre-exists in the nucleus as an entity and that during the decay it carries no angular momentum. Alpha transitions in which the ground-state configuration of the parent nucleus remains

1649

1650 Nuclear properties of actinide nuclides

unchanged are called 'favored transitions' and these have hindrance factors close to unity. All Q( transitions between the ground states of even-even nuclei are favored transitions.

Just like elements of lower Z, each actinide element also has one or more fJstable isotopes. Isotopes heavier than the fJ-stable nucleus decay by emission of p- particles (electrons) whereas lighter isotopes decay by electron capture (EC). In heavy elements, the r lEe ratio is very small and, as a consequence, positron (r) emission has been observed only in a few nuclei. The fJ decay energy usually increases as the nucleus gets further away from the line of fJ stability. A quantity denoted by It is very useful in classifying fJ transitions and estimating fJ decay halflives. The log It value, also called the reduced fJ transition probability, is the energy-independent transition rate.

Spontaneous fission is a decay process in which a nucleus breaks up into two almost equal fragments. Each fission event is accompanied by the release of about 200 MeV energy and the emission of 2-4 neutrons. Fission half-life depends on the fissility parameter Z2 I A and it is the major mode of decay for many isotopes of elements 100 and beyond.

Recently a new form of radioactivity has been discovered [7] in which nuclei decay by the spontaneous emission of particles heavier than alpha particles but lighter than fission fragments. The branching ratio for this decay mode is extremely small (of the order of 10- 1°). Examples of such decay modes are the 14C emission [8] by 223Ra, and 24Ne emission [9] by 231Pa and 232U.

Alpha and beta transitions usually populate the ground state as well as several excited states of the daughter nucleus. These excited states de-excite to the ground ~tate by emission of}' rays and conversion electrons. Typical half-lives of these states are between 10- 9 and 10- 14 s. However, in some cases, the decay of an excited state is forbidden for fast magnetic dipole (M1), electric dipole (E1), or electric quadrupole (E2) transitions because of the angular momentum selection rule. Such states have lifetimes of 10- 9 s to years. Excited states that have halflives of greater than 10- 9 S are called metastable states or isomers. The isomeric state either de-excites to the ground state of the same nucleus by an internal transition (IT) or it decays by the usual modes of disintegration.

Most isomers occur because of the large difference between the spins of the excited state and the ground state. However, there is a class of isomers that decay by fission, and these are caused not by the difference in the angular momenta of the states but by difference in the shapes. These are called 'fission isomers' or 'shape isomers', and have half-lives in the range of 10 - 9 S to 10 - 3 s. These isomers have deformation almost twice that of the ground-state nucleus. More than 50 fission isomers have been discovered [10].

Extensive research has been done on the nuclear structure of heavy elements using radioactive decay studies and high-resolution nuclear reaction spectroscopy. These investigations have provided important information to test and develop microscopic theoretical models. It has been established that nuclei with A ~ 225 have spheroidal shape with major: minor axes in the

Discussion 1651

approximate ratio of 5: 4. The intrinsic electric quadrupole moments of these nuclei have been measured to be about 10 - 23 e cm2 and their radii are approximately 10- 12 cm.

Recent investigations indicate that certain nuclei have octupole deformation. These pear-shaped nuclei are axially symmetric but they are reflection asymmetric. Examples [11] of pear-shaped nuclei are 229Pa and 225 Ac.

In nuclei, nucleons (protons and neutrons) move in orbits under the influence of the central nuclear potential. Nilsson [12] and others [13] have calculated the eigenvalues and wavefunctions of a nucleon in a deformed potential as a function of deformation p. A plot of eigenvalues versus deformation, commonly known as Nilsson diagram, is extremely useful in understanding the energy levels in deformed nuclei. Each Nilsson state is characterized by n, the projection of the single-particle angular momentum on the nuclear symmetry axis; n, the parity; and the asymptotic quantum numbers, N, nz and A. The quantum number N denotes the oscillator shell number, nz represents the number of oscillator quanta along the symmetry axis, and A is the projection of the orbital angular momentum on the symmetry axis. In actinide nuclei, neutrons (protons) fill each orbital above the closed shell of 126 (82) pairwise and thus the ground-state spin-parity of an odd-mass nucleus is simply the spin-parity of the state occupied by the last unpaired nucleon. All even-even nuclei have ground-state spin-parity of 0+.

Since the rotation axis of the spheroidal nucleus is perpendicular to the symmetry axis K, the projection of the total angular momentum I, is the same as n. The rotation generates a band with spin sequence K, K + 1, K + 2, ... , etc. The rotational energy of a level is given by the expression

112 EI = fj(l + 1)

where h is Planck's constant and oF is the nuclear moment of inertia. Typical values of h2 /2 oF are 7 keY for even-even nuclei and 6 keY for odd-mass nuclei. The ground-state band of an even-even nucleus has spin-parity sequence of 0 + , 2 +, 4 +, 6 +, ... ; odd spin values are not allowed.

There are several methods for the qualitative and quantitative analysis of actinide samples. The easiest technique is the gross counting in a 2n (50 %) geometry gas proportional counter. These counters have very low background for ex particles and fission events but have somewhat higher background for Pparticles. Samples with only few disintegrations per minute of ex or fission can be easily counted.

A more powerful technique involves the measurement of energy spectra with solid-state detectors. Alpha-particle spectra can be measured with an Au-Si surface barrier detector. For these measurements thin sources are required and both the source and the detector are placed in vacuum. Resolutions (full width at half maximum) of IO-30keV are easily obtained and usual geometries are 5-30%. By measuring the ex-particle spectrum, commonly known as ex pulse-height

1652 Nuclear properties of actinide nuclides

analysis, one can determine the relative quantities of various nuclides present in a sample.

Gamma-ray spectroscopy with a germanium detector is another powerful and versatile technique for the analysis of radioactive samples. In general, prominent y rays are present in the decay of odd-mass and odd-odd (odd neutron-odd proton) nuclei, and can be used to assay these nuclides. Also, nuclides that decay by electron capture almost always produce the characteristic K x-rays of the daughter nuclei. These x-rays have convenient energies in the 80-160 keY region. The advantage of y-ray spectroscopy is that samples in any quantity and in any form (solution or solid) can be assayed. The resolution of Ge detectors can be better than 1 ke V and maximum efficiency is about 25 %. The efficiency is a function of energy, and between 100 keY and 1 MeV it drops approximately by an order of magnitude.

Because of their long half-lives, 232Th, 235U, and 238U occur in nature. Each of these nuclides starts a decay chain that terminates at stable Pb isotopes. For this reason isotopes of elements between Pb and U are also found in nature. Chemical separation procedures are used to isolate samples of Ac, Th, and Pa nuclides. Enriched samples of elements, like U, for which many isotopes are present together, are commonly obtained using isotope separators.

The main source of transuranium elements is the high-flux reactor, in which 238U or heavier nuclei get transformed into higher-Z elements by multiple neutron capture. In the USA, there is a national program for the production of transuranium elements utilizing the high-flux reactor (HFIR) at Oak Ridge. The heaviest nuclide produced in the reactor is 257Fm. Neutron-deficient nuclides are synthesized in charged-particle accelerators and very neutron-rich nuclides with short half-lives are produced in reactors.

All data in the nuclear properties tables and this appendix have been taken from refs 3-5 except where a more recent reference was found. The cut-off date for literature survey was March 1986.

The notations for various decay modes used in this book are: ex for alpha decay, P - for P - decay, P + for positron decay, EC for electron capture, IT for isomeric transition, and SF for spontaneous fission. The letter 'm' after a mass number denotes an isomer. Isomers with a half-life ofless than 1 s and fission isomers are omitted from the tables. Energies are given only for the most abundant ex groups and y rays; for p- particles the maximum energies Pmax are tabulated. In the last column, only the convenient methods for the production of nuclides are given: 'nature' denotes that the nuclide occurs in nature and 'multiple neutron capture' means that this nuclide is produced by long irradiation in a high-flux reactor.

The specific activity S in disintegrations per minute per microgram was calculated using the expression

4.17449 x 1017 S=----

Tl/2A

The half-lives Tl/2 were obtained from refs 3-5 and the atomic masses A were taken from ref. 6.

Tables 1653

REFERENCES

1. Friedlander, G., Kennedy, J. W., Macias, E. S., and Miller, J. M. (1981) Nuclear and Radiochemistry, Wiley, New York.

2. Hyde, E. K., PerIman, I., and Seaborg, G. T. (1964) The Nuclear Properties of the Heavy Elements, Vol. I, Prentice-Hall, Inc. Englewood Cliffs, New Jersey.

3. Lederer, C. M. and Shirley, V. S., eds (1978) Table of Isotopes, Wiley, New York. 4. Browne, E. and Firestone, R. B. (1986) Table of Radioactive Isotopes, (ed. V. S. Shirley)

Wiley, New York. 5. Armbruster, P. (1985) Ann. Rev. Nucl. Part. Sci., 35, 135-94. 6. Wapstra, A. H. and Audi, G. (1985) Nucl. Phys., A431, 1-54. 7. Rose, H. J. and Jones, G. A. (1984) Nature, 307, 245-47. 8. Kutschera, W., Ahmad, I., Armato, S. G., III, Friedman, A. M., Gindler, J. E., Henning,

W., Ishii, T., Pau~ M., and Rehm, K. E. (1985) Phys. Rev., C32, 2036-42. 9. Barwick, S. W., Price, P. B., and Stevenson, J. D. (1985) Phys. Rev., C31, 1984-6.

10. Vandenbosch, R. (1977) Ann. Rev. Nucl. Sci., 27, 1-35. 11. Ahmad, I., Gindler, J. E., Betts, R. R., Chasman, R. R., and Friedman, A. M. (1982)

Phys. Rev. Lett., 49, 1758-61. 12. Nilsson, S. G. (1955) Kgl. Dansk Videnskab. Selskab., Mat.-Fys. Medd., 29, No. 16. 13. Chasman, R. R., Ahmad, I., Friedman, A. M., and Erskine, J. R. (1977) Rev. Mod.

Phys., 49, 833-91.

TABLES

In this appendix we now reproduce, for reference and comparative purposes, the tables in each of chapters 2 through 13 that contained details of the nuclear properties of the isotopes of actinium through lawrencium and of elements 104-109. We then give a table summarizing the specific activities of the nuclides.

Nuclear properties of actinium isotopes.

Mass Mode of Main radiations number Half-life decay (MeV) Method of production

209 0.10 S IX IX 7.59 197 AueoNe,8n) 210 0.35s IX IX 7.46 197 AueONe,7n)

203Tl( 16O,9n) 211 0.25 S IX IX 7.48 197 AueoNe,6n)

203Tl( 16O,8n) 212 0.93 S IX IX 7.38 203TW6O,7n)

213 0.80s IX IX 7.36 197 AueoNe,5n) 197 AueoNe,4n) 203Tl( 16O,6n)

214 8.2 s IX ~86% IX 7.214 (52%) 203Tl( 16O,5n) EC ~ 14% 7.082 (44%)

197 AueoNe,3n) 215 0.17 s IX 99.91 % IX 7.604 203Tl( 16O,4n)

ECO.09% 209Bi( 12C,6n) 216 ~ 0.33 ms IX IX 9.07 209BW 2C,5n) 216m 0.33 ms IX IX 9.102 (46 %)

217 0.11 Jls IX

9.024 (50%) IX 9.65 208Pbe4N,5n)

218 0.27 Jlsa IX IX 9.20 222Pa daughter 219 7 Jls IX IX 8.66 223Pa daughter 220 26ms IX IX 7.85 (24%) 208PbesN,3n)

7.68 (21 %) 224Pa daughter 7.61 (23%)

221 52ms IX IX 7.65 (70%) 2osTW2Na,1X2n) 7.44 (20%) 208Pb( 18O,p4n)

222 5s IX IX 7.00 226Ra(p,5n) 208Pb( 18O,p3n)

222m 66 s (X ~90% (X 7.00 (15%) 208Pbe 80,p3n) EC ~ 1% 6.81 (27%) 209Bi(18O,lXn) IT < 10%

223 2.2 min IX 99% IX 6.662 (32 %) 227Pa daughter EC 1% 6.647 (45%)

228Pa daughter 224 2.9h EC ~ 90% IX 6.211 (20 %) IX ~ 10% 6.139 (26%)

225 10.0d (X IX 5.830 (51 %) 22sRa daughter 5.794 (24%)

Y 0.100 (1.7%) 226 29h p- 83% IX 5.399 226Ra(d,2n)

EC17% p-UO IX 6 X 10-3 % y 0.230 (27%)

227 21.773 yr p- 98.62% IX 4.950 (47 %) nature 4.938 (40%)

IX 1.38% p-0.045 y 0.086

228 6.13 h p- p- 2.18 nature y 0.991

229 62.7 min p- p-1.09 229Ra daughter y 0.165 232Th(y,p2n)

230 122 s p- P-1.4 232Th(y,pn) y 0.455

231 7.5 min p- P-2.1 mTh(y,p) y 0.282 232Th(n,pn)

232 35 s p- 232Th(n,p) 233 2.3 min p- 23SUeHe, sB)

1655

Nuclear properties of thorium isotopes.

Mass Mode of Main radiations Method of number Half-life decay (MeV) production

213 or 214 0.12 s at: at: 7.69 206Pb('60,8 or 9n) 215 1.2 s at: at: 7.52 (40%) 206Pb('60,7n)

7.39 (52%) 216 28ms at: at: 7.92 206Pb(16O,6n) 217 0.25 ms at: at: 9.25 206Pb('60,5n) 218 0.10 lis at: at: 9.66 206Pb('60,4n)

209BW4 N,5n) 219 1.05 lis at: at: 9.34 206Pb('60,3n) 220 10 lis at: at: 8.79 208Pb('60,4n) 221 1.7ms at: at: 8.472 (32 %) 208Pb('60,3n)

8.146 (62%) 208Pb( 16O,2n) 222 2.8ms at: at: 7.98

223 O.66s at: IX 7.32 (40%) 208Pb('80,3n) 7.29 (60%)

224 1.043 s at: at: 7.17 (81 %) 228U daughter 7.00 (19%) 208Pbe2Ne,a:2n)

')' 0.177 225 8.0 min at: ~9O% at: 6.478 (43 %) 229U daughter

EC ~ 10% 6.441 (15%) 231 Pa(p,at:3n) ')' 0.321

226 30.9 min at: at: 6.335 (79 %) 230U daughter 6.225 (19%)

')' 0.1113 227 18.718 d at: 6.038 (25 %) nature

5.978 (23%) ')' 0.236

228 1.913 yr at: at: 5.423 (72.7 %) nature 5.341 (26.7 %)

')' 0.084 229 7.3 x 103 yr at: at: 4.901 (11 %) 233U daughter

4.845 (56%) ')' 0.194

230 8.0 x lW yr at: rx 4.687 (76.3 %) nature 4.621 (23.4 %)

')' 0.068 231 25.52h {r (r0.302 nature

')' 0.084 23OTh(n,,),) 232 1.41 x 1010 yr at: at: 4.016 (77 %) nature

> 1 x 1021 yr SF 3.957 (23%) 233 22.3 min {r (r 1.23 232Th(n,,),)

')' 0.086 234 24.10d {r (rO.198 nature

')' 0.093 235 6.9 min (r 238U(n,at:) 236 37 min (r ')' 0.111 238U(')',2p)

238U(p,3p)

1656

Nuclear properties of protactinium isotopes.

Mass Mode of Main radiations number Half-life decay (MeV) Method of production

216 0.20s IX IX 7.92 189Qse1 P,4n) 197 Aue4Mg,5n)

222 5.7ms IX IX 8.54 (- 30%) 209Bi(16Q,3n) - 8.18 (- 50%) 206Pbe9F,3n)

223 6ms IX IX 8.20 (45%) 208Pbe9F,4n) 8.01 (55%) 20Sne2Ne,4n)

224 0.9s IX IX 7.49 208Pbe9F,3n) 205ne2Ne,3n) 232Th(p,9n)

225 1.8s IX IX 7.25 (70%) 232Th~,8n) 7.20 (30%) 209Bi( 2Ne,1X2n)

226 1.8 min IX 74% IX 6.86(52%) 232Th(p,7n) EC26% 6.82(46%)

227 38.3 min IX -85% IX 6.466 (51 %) 232Th(p,6n) EC-15% 6.416(15%)

)I 0.065 228 22h EC-98% IX 6.105 (12%) 232Th(p,5n)

IX -2% 6.078 (21 %) 23OTh(p,3n) )I 0.410

229 1.5d EC 99.5% IX 5.669 (19%) 23OTh(d,3n) IX 0.48% 5.579 (37%) 229Th(d,2n)

230 17.7d EC90% IX 5.345 23OTh(d,2n) tr 10% tr 0.51 232Th(p,3n) IX 3.2 x 10-3% )I 0.952

231 3.28 x lQ4yr IX IX 5.012(25%) nature 4.951 (23 %)

)I 0.300 232 l.31d Ir tr 1.29 231Pa(n,)I)

)I 0.969 232Th(d,2n) 233 27.0d tr tr 0.568 233Th daughter

)I 0.312 237Np daughter 234 6.75h tr tr 1.2 nature

)I 0.570 234m 1.175 min tr 99.87% tr 2.29 nature

IT 0.13% )I 1.001 235 24.2 min tr tr 1.41 235Th daughter

238U()I,p2n) 235U(n,p)

236 9.1 min tr tr 3.1 236U(n,p) )I 0.642 238U(d,lX)

237 8.7 min tr tr 2.3 238U()I,p) )I 0.854 238U(n,pn)

238 2.3 min tr tr 2.9 238U(n,p) )I 1.014

1657

Nuclear properties of uranium isotopes. (Contd.)

Mass Main radiations Method of number Half-life Mode of decay (MeV) production

226 O.5s IX IX 7.43 232Th(IX,10n) 227 1.1 min IX IX 6.87 232Th(IX,9n)

20BPbe2Ne,3n) 228 9.1 min IX ~95% IX 6.68 (70%) 232Th(IX,8n)

EC ~5% 6.60 (29%) y 0.152

229 58 min EC - 80% IX 6.360 (64 %) 23OTheHe,4n) IX -20% 6.332 (20%) 232Th(IX,7n)

y 0.123 230 20.8d IX IX 5.888 (67.5 %) 230Pa daughter

5.818 (31.9%) 231 Pa (d,3n) y 0.072

231 4.2d EC > 99% IX 5.46 23OTh(IX,3n) IX 5.5xlO-3% y 0.084 231Pa(d,2n)

232 68.9 yr IX IX 5.320 (68.6 %) 232Th(IX,4n) ~8xlO13yr SF 5.264 (31.2 %)

y 0.058 233 1.592 x 105 yr IX IX 4.824 (82.7 %) 233Pa daughter

1.2 x 1017yr SF 4.783 (14.9 %) y 0.097

234 2.45 x lOSyr IX IX 4.777(72 %) nature 2 x 1016 yr SF 4.723 (28 %)

235 7.037 x lOB yr IX IX 4.397 (57 %) nature 3.5 x 1017 yr SF 4.367 (18 %)

y 0.186 235m 26 min IT 239pU daughter 236 2.342 x 107 yr IX IX 4.494 (74 %) 23SU(n,y)

2 x 1016 yr SF 4.445 (26%) 237 6.75d p- P-0.519 236U(n,y)

y 0.060 241 Pu daughter 238 4.47 x 109 yr IX IX 4.196 (77 %) nature

8.19 x 1015 yr SF 4.149 (23%) 239 23.5 min p- P-1.29 23BU(n,y)

y 0.075 240 14.1 h p- p-0.36 244pU daughter

y 0.044 242 17min p- P-1.2 244Pu(n,2pn)

y 0.068

1658

Nuclear properties of neptunium isotopes.

Mass Mode of Main radiations Method of number Half-life decay (MeV) production

227 or 228 60s SF 22Ne on 209Bi 229 4.0 min IX ~50% IX 6.89 233U(p,5n)

EC~50% 230 4.6 min IX >99% IX 6.66 233U(p,4n)

EC ~ 0.97% 231 48.8 min EC <99% IX 6.28 233U(d,4n)

IX >1% 'Y 0.371 235U(d,6n) 232 14.7 min EC 'Y 0.327 233U(d,3n) 233 36.2 min EC < 99% IX 5.54 233U(d,2n)

IX '""' 10-3% 'Y 0.312 23'U(d,4n) 234 4.4d EC 99.95% 'Y 1.559 235U(d,3n)

p+ 0.05% 235 396d EC>99% IX 5.022 (53%) mU(d,2n)

IX 1.6 x 10;3% 5.004 (24%)

236- 22.5 h tr 50% tr 0.54 mU(d,n) EC50% 'Y 0.642

236- 1.55 x 10' yr EC87% 'Y 0.163 235U(d,n) tr 13%

237 2.14 x 106 yr IX IX 4.788 (51 %) 237U daughter > 1 x 1018 yr SF 4.770 (19%) 241Am daughter

'Y 0.086 238 2.117 d {r tr 1.29 237Np(n,'Y)

'Y 0.984 239 2.35 d tr p- 0.72 243 Am daughter

'Y 0.106 239U daughter 240 1.032h tr tr 2.09 238U(IX,pn)

'Y 0.566 240m 7.22 min tr tr 2.05 240U daughter

'Y 0.555 '238U(IX,pn) 241 13.9 min tr tr 1.31 238U(IX,p)

'Y 0.175 244Pu(n,p3n) 242g

orm 5.5 min p- tr2.7 244Pu(n,p2n) 'Y 0.786 242pU(n,p)

242g orm 2.2 min tr tr 2.7 242U daughter

'Y 0.736

a Not known whether ground-state nuclide or isomer.

1659

Nuclear properties of plutonium isotopes.


232 34 min EC ~ 80% tx 6.60 (62%) 233U(tx,5n) tx ~20% 6.54 (38%)

233 20.9 min EC 99.88% tx 6.30 233U(tx,4n) ex 0.12% "i 0.235

234 8.8h EC94% ex 6.202 (68%) 233U(tx,3n) ex 6% 6.151 (32 %)

235 25.6 min EC > 99% ex 5.85 23SU(tx,4n) ex 3 x 10-3% "i 0.049 233U(ex,2n)

236 2.85 yr ex tx 5.768 (69%) 23SU(ex,3n) 3.5 x 109 yr SF 5.721 (31 %) 236Np daughter

237 45.4d EC > 99% tx 5.65 (21 %) 23SU(ex,2n) ex 3.3 x 10-3 % 5.36 (79%) 237Np(d,2n)

"i 0.059 238 87.74 yr ex ex 5.499 (70.9 %) 242Cm daughter

4.8 x 1010 yr SF 5.457 (29.0 %) 238Np daughter 239 2.41 x 104 yr tx tx 5.155 (73.3 %) 239Np daughter

5.5 x lOIS yr SF 5.143 (15.1 %) n capture "i 0.129

240 6.563 x 103 yr tx ex 5.168 (72.8 %) multiple n capture 1.34 x 1011 yr SF 5.123 (27.1 %)

241 14.4 yr tr > 99% tx 4.896 (83.2 %) multiple n capture tx 2.4 x 10-3 % 4.853 (21.1 %)

tr 0.021 "i 0.149

242 3.76 x lOs yr tx tx 4.901 (74 %) multiple n capture 6.8 x 1010 yr SF 4.857 (26%)

243 4.956h tr tr 0.58 multiple n capture "i 0.084

244 8.26 x 107 yr ex tx 4.589 (81 %) multiple n capture 6.6 x 1010 yr SF 4.546 (19%)

245 10.5h Ir tr 1.28 244Pu(n,"i) "i 0.327

246 10.85 d tr fr 0.374 24SPu(n,"i) "i 0.224

1660

Nue/ear properties of americium isotopes.


234 2.6 min EC 23OTheOB,6n) lOB, 11B on 233U

237 1.22 h EC >99% ex 6.042 237Np(ex,4n) ex 0.025% "I 0.280 (47%) 237NpeHe,3n)

238 1.63 h EC >99% ex 5.94 237Np(ex,3n) ex LOx 10-4 % "I 0.963 (29%)

239 11.9 h EC >99% ex 5.776 (84%) 237Np(ex,2n) 5.734 (13.8%)

ex 0.010% "I 0.278 (15%) 239Pu(d,2n) 240 50.8 h EC >99% ex 5.378 (87%) 237Np(ex,n)

ex 1.9 x 10-4 % 5.337 (12.0%) 239pu(d, n)

"I 0.988 (73%) 241 432.7yr ex ex 5.486 (84.0 %) 241 Pu daughter

1.15 x 1014 yr SF 5.443 (13.1 %) multiple n capture "I 0.059 (35.7 %)

242 16.01 h tr 82.7% tr 0.667 241 Am(n,"I) EC 17.3% "I 0.042 weak

242m 141 yr IT 99.55% ex 5.207 (89%) 241 Am(n,"I) 9.5 x 1011 yr SF

ex 0.45% 5.141 (6.0%) 241 Am(n,"I) "I 0.0493 (41 %)

243 7.38 x 103 yr ex ex 5.277 (88%) multiple 2.0 x 1014 yr SF 5.234 (10.6%) n capture

"I 0.075 (68 %) 244 10.1 h tr tr 0.387 243Am(n,"I)

"I 0.746 (67%) 244m 26 min tr >99% tr 1.50 243Am(n,"I)

EC 0.041 % 245 2.05 h tr tr 0.895 24SpU daughter

"I 0.253 (6.1 %) 2468 25.0 min tr tr 2.38 246pU daughter

"I 0.799 (25%) 2468 39 min tr "I 0.679 (52%) 244Pu(ex,d)

244PueHe,p) 247 24 min tr i' 0.285 (23%) 244pU(ex,p)


1661

Nuclear properties of curium isotopes.

Mass Main radiations number Half-life Mode of decay (MeV) Method of production

238 2.3 h EC <90% IX 6.52 239Pu(IX,5n) IX >10%

239 2.9h EC )' 0.188 239Pu(IX,4n) 240 27d IX IX 6.291 (71 %) 239Pu(IX,3n)

1.9 x 106 yr SF 6.248 (29%) 241 32.8 d EC 99.0% IX 5.939 (69 %) 239Pu(IX,2n)

IX 1.0% 5.929 (18%) )' 0.472 (71 %)

242 162.9d IX IX 6.113 (74.0 %) 239Pu(lX,n) 6.1 x 106 yr SF 6.070 (26.0 %) 242 Am daughter

243 28.5 yr IX 99.76% IX 5.785 (73.5 %) 242Cm(n,),) EC 0.24% 5.741 (10.6%)

)' 0.278 (14.0%) 244 18.11 yr IX IX 5.805 (76.7 %) multiple n capture

1.35 x 107 yr SF 5.764 (23.3 %) 244 Am daughter 245 8.5 x 103 yr IX IX 5.362 (93.2 %) multiple n capture

5.304 (5.0%) )' 0.175

246 4.73 x 103.yr IX IX 5.386 (79 %) multiple n capture 1.80 x 107 yr SF 5.343 (21 %)

P stable 247 1.56 x 107 yr IX IX 5.266(14%) multiple n capture

4.869 (71 %) )' 0.402 (72%)

248 3.40 x lOs yr IX 91.74% IX 5.078 (82 %) multiple n capture SF 8.26% 5.034 (18%)

249 64.2 min p- p-0.9 248Cm(n,),) )' 0.634 (1.5 %)

250 < 1.13 x 104 yr SF multiple n capture 251 16.8 min p- P-1.42 2S0Cm(n,)')

)' 0.543 (12 %)

1662

Nuclear properties of berkelium isotopes.


240 5 min EC 232The4N,6n) 242 7 min EC 235U e 1 B,4n)

232The5N,5n) 243 4.5h EC99.85% ex 6.758 (15%) 243Am(ex,4n)

ex 0.15% 6.574 (26%) ')' 0.755

244 4.35 h EC >99% ex 6.667 ( - 50 %) 243Am(ex,3n) ex 6xlO- 3% 6.625 (- 50%)

')' 0.218 245 4.9Od EC99.88% ex 6.349 (15.5 %) 243 Am(ex,2n)

ex 0.12% 6.145 (18.3 %) ')' 0.253 (31 %)

246 1.80d EC ')' 0.799 (61 %) 243Am(ex,n) 247 1.38

x 103 yr ex ex 5.712 (17%) 247 Cf daughter 5.532 (45%) 244Cm(ex,p)

')' 0.084 (40%) 248a 23.7h p- 70% p- 0.86 248Cm(d,2n)

EC30% ')' 0.551 248a > 9yr decay not observed 246Cm(ex,pn) 249 320d p- > 99% ex 5.417 (74.8 %) mUltiple n capture

ex 1.45 x 10-3% 5.390 (16.0%) p- 0.125 ')' 0.327 weak

250 3.217 h p- p- 1.781 254Es daughter ')' 0.989 (45%) 249Bk(n,,),)

251' 56 min p- p- -1.1 255Es daughter ')' 0.178


1663

Nuclear properties of californium isotopes.


239 39 s a a 7.63 243Fm daughter 240 1.1 min a a 7.59 233U(12C,5n) 241 3.8 min a a 7.335 233Ue2C,4n) 242 3.5 min a a 7.385 (- 80%) 233U(12C,3n)

7.351 (- 20%) 235Ue2C,5n) 243 10.7 min EC - 86% a 7.06 23SU(12C,4n)

a -14% 244 19.4 min a a 7.210 (75 %) 244Cm(a,4n)

7.168 (25%) 236Ue2C,4n) 245 43.6 min EC-70% a 7.137 244Cm(a,3n)

a -30% 238U(12C,5n) 246 35.7 h a a 6.758 (78 %) 244Cm(a,2n)

2.0 x 103 yr SF 6.719 (22%) 246Cm(a,4n) p stable

247 3.11 h EC99.96 % a 6.296 (95 %) 246Cm(a,3n) a 0.035% y 0.294 (1.0 %) 244Cm(a,n)

248 334d a a 6.258 (80.0 %) 246Cm(a,2n) 3.2 x 104yr SF 6.217 (19.6%)

P stable 249 351 yr a a 6.194 (2.2 %) 249Bk daughter

6.9 x 1010 yr SF 5.812 (84.4%) Y 0.388 (66 %)

250 13.08 yr a a 6.031 (83 %) multiple n capture 1.7 x 104yr SF 5.989 (17%)

251 898 yr a a 5.851 (27 %) multiple n capture 5.677 (35%)

Y 0.177 (17 %) 252 2.645 yr a 96.91 % a 6.118 (84%) multiple n capture

SF 3.09% 6.076 (15.8 %) 253 17.81 d p- 99.69% a 5.979 (95 %) multiple n capture

a 0.31 % 5.921 (5%) 254 6O.5d SF 99.69% a 5.834 (83 %) multiple n capture

a 0.31 % 5.792 (17%) 255 1.4h p- 254Cf(n,y) 256 12.3 min SF 254Cf(t,p)

1664

Nuclear properties of einsteinium isotopes.

Mass Main radiations number Half-life Mode of decay (MeV) Method of production

243 21s Ot Ot 7.89 233U e5N, 5n) 244 37s EC 96% Ot 7.57 233U e5N,4n)

Ot - 4% 237Np (12C, 5n) 245 1.3 min EC 60% Ot 7.73 237Np (12C,4n)

Ot 40% 246 7.7 min EC 90% Ot 7.35 241 Am (12C, Ot3n)

Ot 10% 247 4.7 min EC -93% Ot 7.32 241 Am (12C, Ot2n)

Ot - 7% 238U e4N, 5n) 248 27 min EC 99.7% Ot 6.87 249Cf(d,3n)

Ot - 0.3% ')I 0.551 249 l.70h EC 99.4% Ot 6.770 249Cf(d,2n)

Ot 0.57% ')I 0.380 250" 8.6h EC ')I 0.829 249Cf(d,n) 250" 2.22h EC ')I 0.989 249Cf(d,n) 251 33h EC 99.5% Ot 6.492 (81 %) 249Bk (Ot,2n)

Ot 0.49% 6.463 (9%) 252 472d Ot 78% Ot 6.632 (80 %) 249Bk(Ot,n)

EC 22% 6.562 (13.6 %) ')I 0.785

253 20.47d Ot Ot 6.633 (89.8 %) multiple 6.3 x 105yr SF 6.592 (7.3 %) n capture

p stable 254g 275.7 d Ot Ot 6.429 (93.2 %) multiple

>2.5 x 107yr SF 6.359 (2.4 %) n capture ')I 0.062

254m 39.3h p- 99.6% Ot 6.382 (75 %) 253Es (n,')I) >lx105yr SF 6.357 (8%)

Ot 0.33% f 0.08%

255 39.8d p- 92.0% Ot 6.300 (88 %) multiple Ot 8.0% 6.260(10%) n capture SF 4xlO- 3 %

256a 25.0 min p- 255Es (n,')I) 256a -7.6h p- 254Es (t,p)


1665

Nuclear properties of fermium isotopes.


242 0.8ms SF 204Pb(40 Ar, 2n) 243 0.18 s a a 9.55 206Pb(40 Ar, 3n) 244 3.3 ms SF 206Pb(40 Ar, 2n)

233Ue6O,5n) 245 4.2s a a 8.15 233Ue6O,4n) 246 1.1s a 92% a 8.24 235Ue6O,5n)

SF 8% 239Pu(12C,5n) 247" 35 s a ~50% a 7.93 ( - 30 %) 239Pu(12C,4n)

EC ::;; 50% 7.87(-70%) 247" 9s a a 8.18 239Pu(12C,4n) 248 36s a 99.9% a 7.87 (80 %) 240pu(12C,4n)

SF 0.1 % 7.83 (20%) 249 2.6 min a a 7.53 238Ue6O,5n)

249Cf(a,4n) 250 30 min a a 7.43 249Cf(a,3n)

SF 5.7 x 10-4% 238Ue6O,4n) 250m 1.8 s IT 249Cf(a,3n) 251 5.30h EC 98.2% a 6.834 (87 %) 249Cf(a,2n)

a 1.8% 6.783 (4.8 %) 252 25.39h a a 7.039 (84.0 %) 249Cf(a, n)

SF 2.3 x 10-3 % 6.998 (15.0 %) 253 3.0d EC 88% a 6.943 (43 %) 252Cf(a,3n)

a 12% 6.674(23%) 'l' 0.272

254 3.240h a >99% a 7.192 (85.0 %) 254mEs daughter SF 0.0592% 7.150 (14.2 %)

255 20.07h a a 7.022 (93.4 %) 255Es daughter SF 2.4 x 10-5 % 6.963 (5.0%)

256 ·2.63h SF 91.9% a 6.915 256Md daughter a 8.1% 256Es daughter

257 l00.5d a 99.79% a 6.695 (3.5 %) multiple n capture SF 0.21 % 6.520 (93.6 %)

'l' 0.241 258 0.38ms SF 257Fm(d,p) 259 1.5s SF 257Fm(t, p)

a Not known whether ground-state nuclide, isomer, or identification error.

1666

Nuclear properties of mendelevium isotopes.


247 2.9s 0( 0( 8.43 209Bi(40 Ar,2n) 248 7s EC ~ 80% 0( 8.36 ( ~ 25 %) 241 Am(12C,5n)

0( ~20% 8.32 (~75%) 239PU( 14N,5n) 249 24s EC ~ 80% 0( 8.03 241 Am( 12C,4n)

0( ~20% 250 52 s EC 94% 0( 7.82 (~30%) 243 Am( 12C,5n)

0( 6% 7.75( ~ 70%) 24OpuC5N,5n) 251 4.0 min EC ~ 94% 0( 7.55 243 Am( 12C,4n)

0( ~6% 240pUC 5N,4n) 252 2.3 min EC 243Am(13C,4n)

238UC 9F,5n) 254" 10 min EC 253Es(0(,3n) 254" 28 min EC 253Es(0(,3n) 255 27 min EC92% 0( 7.333 253Es(0(,2n)

0( 8% }' 0.453 254Es(0(,3n) 256 1.27 h EC 90.7% 0( 7.205 (63 %) 253Es(0(,n)

0( 9.9% 7.139 (16 %) 257 5.4h EC90% 0( 7.069 254Es(0(,n)

0( 10% 258" 55d IX 0( 6.790 (28 %) 255Es(0(,n)

6.716 (72 %) 258" 43 min EC? 255Es(0(,n) 259 1.6h SF 259No daughter

" Not known whether ground-state nuclide or isomer.

1667

Nuclear properties of nobelium isotopes.


250· 0.25m8 SF 233Ue2Ne,5n) 251 0.88 ex ex 8.68 (20 %) 244Cm(12C,5n)

8.60(80%) 252 2.38 ex 73% ex 8.415 ( -75 %) 244Cm(J2C,4n)

SF 27% 8.372 ( - 25 %) 239puesO,5n) 253 1.7 min ex ex 8.01 246Cm(J2C,5n)

242pue 60, 5n) 254 688 ex ex 8.086 246Cm(J2C,4n)

242pue6O,4n) 254m 0.288 IT 246Cme 2C,4n)

249Cfe 2C,ex3n) 255 3.1 min ex 61.4% ex 8.121 (46 %) 24SCm(J2C,5n)

13's EC 38.6% 8.077 (12%) 249Cf(J2C,ex2n)

256 ex -99.7% ex 8.43 24SCm(J2C,4n) SF -0.3%

257 258 ex ex 8.27 (26 %) 24SCm(J2C,3n) 8.22(55%)

258 1.2m8 SF 24SCm(J3C,3n) 259 1.ooh ex -78% ex 7.533 (23 %) 24SCmesO,ex3n)

EC -22% 7.500(38%)

• The identity of this nuclide is not well-established.

Nuclear properties of lawrencium isotopes.


253 1.38 ex ex 8.800 (56 %) 2s7105 daughter 254 138 ex ex 8.460 (64 %) 2ss105daughter 255 228 ex ex 8.43 (40%) 243Ame6O,4n)

8.37 (60%) 249Cfe 1 B,5n) 256 288 ex ex 8.52 (19 %) 243AmesO,5n)

8.43 (37%) 249Cf(1l B,4n) 257 0.658 III ex 8.86 (85 %) 249Cfe 1 B,3n)

8.80(15%) 249Cfe4N,ex2n) 258 4.38 ex ex 8.621 (25 %) 24SCmesN,5n)

8.595(46%) 249CfesN,ex2n) 259 5.48 ex ex 8.45 24SCmeSN,4n) 260 10 min ex ex 8.03 24SCmesN,3n)

Nuclear properties of element 104 isotopes.


253" -1.8s SF -50% 206Pb(50T~ 3n) 254" 0.5ms SF 206Pb(5OTi,2n) 255 1.4s IX -55% IX 8.715(70%) 207Pu(5OTi,2n)

SF -45% 256 7.4ms SF, IX IX 8.812 208Pb(50T~ 2n) 257 4.3s IX -70% IX 9.012(18%) 208Pb(50Ti, n)

SF -14%? 8.977(29%) 249Cfe 2C, 3n) EC -16%

258" l3ms SF 246Cme6O,4n) 259 3.4s IX 91% IX 8.87( -40%) 249Cf(J3C,3n)

SF 9% 8.77(-60%) 248Cme6O,5n) 260" 21ms SF 248Cme6O,4n) 261 1.1 min IX IX 8.28 248Cme 80, 5n) 262" 47ms SF 248Cm(180,4n)

" The identity of this nuclide is not well-established.

Mass number Half-life

Element 105 255" 1.5s

257 1.4s 258 4.4s

260 1.5s

261 1.8 s

262 34s

Element 106 259 0.48s 260 3.6ms 261 0.26s 263 0.9s

Element 107

1-2ms

262 5ms

Element 108 265 1-8ms

Element 109 266 3.5ms

Nuclear properties of elements 105-109 isotopes.

Mode of decay

SF -20%

IX 9.16 IX

IX ;;..90% SF ~9.6% EC :s;;2.5% IX -75% SF -25% SF -78% IX -22% EC <5%

IX

IX, SF IX

IX

SF

Main radiations (MeV)

IX 9.19 9.07

IX 9.082 (25 %) 9.047 (48%)

IX 8.93

IX 8.66 (-20%) 8.45 (-80%)

IX 9.63 IX 9.76 IX 9.56 IX 9.25

IX 10.38

IX 10.36

IX 11.10

Method of production

207Pb(51 V, 3n) 206Pb(5IV,2n) 209Bi(50Ti,2n) 262 107 daughter

249Cfe5N,4n) 243 Ame 2Ne, 5n)

243 Ame2Ne, 4n) 249Bke60,4n) 249Bk( 180, 5n)

207Pb(54Cr,2n) 208Pb(54Cr,2n) 208Pb(54Cr, n) 249Cf( 180, 4n)

209Bi(54Cr,2n) 208Pb("Mn,2n) 209Bi(,4Cr, n)

a The identity of this nuclide is not well-established.

1669

Specific activities of actinide and transactinide nuclides.

Major SC Nuclide decay mode8 Half-li/eb (dis min -1 Ilg- 1)

Ac 209 IX 0.10s 1.20 x 1018

210 IX 0.35 s 3.41 x 1017

211 IX 0.25 s 4.75 x 1017

212 IX 0.93 s 1.27 x 1017

213 IX 0.80s 1.47 x 1017

214 IX 8.2s 1.43 x 1016

215 IX 0.17 s 6.85 x 1017

216 IX 0.33 ms 3.51 x 1020

216m IX 0.33 ms 3.51 x 1020

217 IX 0.11 lIS 1.05 x 1024

218 IX 0.27 lIS 4.26 x 1023

219 IX 7 lis 1.60 X 1022

220 IX 26ms 4.38 x 1018

221 IX 52ms 2.18 x 1018

222 IX 5s 2.30 X 1016

222m IX 66s 1.71 x lOIS 223 IX 2.2 min 8.51 x 1014

224 EC 2.9h 1.07 x 1013

225 IX 1O.0d 1.29 x 1011 226 p- 29h 1.06 x 1012

227 p- 21.773 yr 1.6057 x 108

228 p- 6.13 h 4.98 x 1012

229 p- 62.7 min 2.907 x 1013

230 p- 122s 8.93 x 1014

231 p- 7.5 min 2.41 x 1014

232 p- 35 s 3.08 x lOIS

Th 213 IX 0.12s 9.8 x 1017

214 IX 0.12s 9.8 x 1017

215 IX 1.2 s 9.71 x 1016

216 IX 28ms 4.14 x 1018

217 IX 0.25 ms 4.62 x 1020

218 IX 0.10 lis 1.15 x 1024

219 IX 1.05 lis 1.09 x 1023

220 IX 10 liS 1.14 X 1022

221 IX 1.7 ms 6.67 x 1019

222 IX 2.8ms 4.03 x 1019

223 IX 0.66s 1.70 x 1017

224 IX 1.04 s 1.08 x 1017

225 IX 8.0 min 2.32 x 1014

226 IX 30.9 min 5.98 x 1013 227 IX 18.72 d 6.821 x 1010

228 IX 1.91 yr 1.82 x 109

229 IX 7.3 x 103 yr 4.75 x lOS 230 IX 8.0 x 104 yr 4.31 x 104

231 p- 25.52 h 1.180 x 1012

232 IX 1.41 x 1010 yr 0.243 233 p- 22.3 min 8.03 x 1013

1670

Specific activities of actinide and transactinide nuclides. (Contd.)

Major So Nuclide decay modea Half-lifeb (dis min-I ltg-I)

234 p- 24.10 d 5.140 x 1010 235 p- 6.9 min 2.57 x 1014 236 p- 37 min 4.78 x 1013

Pa 216 a: 0.20s 5.80 x 1017 222 a: 5.7ms 1.98 x 1019 223 a: 6ms 1.90 x 1019 224 a: 0.9s 1.20 x 1017 225 a: 1.8 s 6.18 x 1016 226 a: 1.8 min 1.03 x lOIS 227 a: 38.3 min 4.80 x 1013 228 Ee 22h 1.39 x 1012

229 Ee 1.5 d 8.44 x 1011 230 Ee 17.7 d 7.12 x 1010

231 a: 3.28 x 104 yr 1.047 x lOs 232 p- 1.31 d 9.54 x 1011 233 p- 27.0d 4.61 x 1010

234 p- 6.75 h 4.40 x 1012

234m p- 1.17 min 1.52 x lOiS 235 p- 24.2 min 7.34 x 1013 236 p- 9.1 min 1.94 x 1014 237 p- 8.7 min 2.02 x 1014 238 p- 2.3 min 7.63 x 1014

U 226 a: 0.5 s 2.20 x 1017 227 a: 1.1 min 1.67 x lOIS 228 a: 9.1 min 2.01 x 1014 229 Ee 58 min 3.14 x 1013 230 a: 20.8d 6.06 x 1010

231 Ee 4.2d 2.99 x 1011 232 a: 68.9 yr 4.965 x 107 233 a: 1.591 x lOS yr 2.141 x 104 234 a: 2.45 x lOS yr 1.384 x 104 235 a: 7.04 x 108 yr 4.797 235m IT 26 min 6.83 x 1013 236 a: 2.342 x 107 yr 1.436 x 102

237 p- 6.75d 1.812 x 1011 238 a: 4.47 x 109 yr 0.7459 239 p- 23.5 min 7.43 x 1013 240 p- 14.1 h 2.06 x 1012

242 p- 17 min 1.01 x 1014

Np 227 or 228 SF 60s 1.84 x lOIS 229 a: 4.0 min 4.56 x 1014 230 a: 4.6 min 3.95 x 1014 231 a: 48.8 min 3.70 x 1013 232 Ee 14.7 min 1.22 x 1014 233 Ee 36.2 min 4.95 x 1013 234 Ee 4.4d 2.82 x lOll 235 Ee 396d 3.115 x 109

1671

specific activities of actinide and transactinide nuclides. (Contd.)

Major SC Nuclide decay modea Half-lifeb (dis min -1 Ilg- 1)

236 p- 22.5h 1.31 x 1012 236m p- 1.55 x 105 yr 2.17 x 104 237 (X 2.14 x 106 yr 1.565 x 103 238 p- 2.117 d 5.752 x 1011 239 p- 2.35d 5.16 x 1011 240 p- 61.9 min 2.81 x 1013 240m p- 7.22 min 2.41 x 1014 241 p- 13.9 min 1.25 x 1014 242 p- 5.5 min 3.14 x 1014 242 p- 2.2 min 7.84 x 1014

Pu 232 EC 34 min 5.29 x 1013 233 EC 20.9 min 8.57 x 1013 234 EC 8.8h 3.38 x lOll 235 EC 25.6 min 6.94 x 1013 236 (X 2.85 yr 1.18 x 109

237 EC 45.4d 2.69 x 1010 238 (X 87.74 yr 3.800 x 107

239 (X 2.41 x 104 yr 1.378 x lOs 240 (X 6.563 x 103 yr 5.038 x lOs 241 p- 14.4 yr 2.29 x 108

242 (X 3.76 x lOS yr 8.721 x 103 243 p- 4.96h 5.77 x 1012 244 (X 8.26 x 107 yr 39.37 245 p- 10.5 h 2.70 x 1012 246 p- 10.85 d 1.086 x 1011

Am 234 EC 2.6 min 6.9 x 1014 237 EC 73.0 min 2.41 x 1013 238 EC 98.0 min 1.79 x 1013

239 EC 11.9 h 2.45 x 1012 240 EC 50.8h 5.71 x 1011 241 (X 432.7 yr 7.609 x 106

242 p- 16.01 h 1.795 x 1012 242m IT 141 yr 2.326 x 107

243 (X 7.38 x 103 yr 4.425 x lOS 244 p- lO.1h 2.82 x 1012

244m p- 26 min 6.58 x 1013 245 p- 2.05h 1.38 x 1013 246 p- 25.0 min 6.79 x 1013 246m p- 39.0 min 4.35 x 1013 247 p- 24 min 7.04 x 1013

Cm 238 EC 2.3 h 1.27 x 1013 239 EC 2.9h 1.00 x 1013 240 (X 27d 4.47 x 1010 241 EC 32.8d 3.67 x 1010 242 (X 162.9 d 7.352 x 109

243 (X 28.5 yr 1.146 x 108

244 (X 18.11 yr 1.796 x 108

245 (X 8.S x 103 vr 3.81 x lOS

1672


Major So Nuclide decay modea Half-lifeb (dis min -1 Jlg-l)

246 ex 4.7 x 103 yr 6.86 x 105 247 ex 1.6 x 107 yr 2.01 x 102

248 ex 3.40 x 105 yr 9.410 x 103 249 p- 64.2 min 2.61 x 1013 250 SF < 1.13 x 104 yr > 2.81 x 105 251 p- 16.8 min 9.90 x 1013

Bk 240 EC 5 min 3.5 x 1014 242 EC 7 min 2.5 x 1014 243 EC 4.5 h 6.36 x 1012

244 EC 4.4h 6.48 x 1012

245 EC 4.90d 2.41 x 1011 246 EC 1.80d 6.55 x 1011 247 ex 1.4 x 103 yr 2.30 X 106

248 p- 23.7h 1.183 x 1012

249 p- 320d 3.637 x 109

250 p- 3.22h 8.64 x 1012

251 p- 56 min 2.97 x 1013

Cf 239 ex 39 s 2.69 x 1015 240 ex 1.1 min 1.58 x 1015 241 ex 4 min 4.3 x 1014 242 ex 3.5 min 4.93 x 1014 243 EC 11 min 1.56 x 1014 244 ex 19 min 9.0 x 1013 245 EC 44 min 3.87 x 1013

246 ex 35.7 h 7.92 x 1011 247 EC 3.11 h 9.05 x 1012

248 ex 334d 3.50 x 109

249 ex 351 yr 9.079 x 106

250 ex 13.08 yr 2.426 x 108

251 ex 900yr 3.51 x 106

252 ex 2.645 yr 1.190 x 109

253 p- 17.8 d 6.44 x 1010 254 SF 60.5 d 1.886 x 1010 255 p- 1.4 h 1.95 x 1013 256 p- 12 min 1.36 x 1014

Es 243 ex 21 s 4.9 x 1015 244 EC 37 s 2.77 x 1015 245 EC 1.3 min 1.3 X 1015 246 EC 7.7 min 2.20 x 1014 247 EC 4.7 min 3.60 x 1014 248 EC 27 min 6.23 x 1013 249 EC 1.70 h 1.64 x 1013 250 EC 8.6h 3.24 x 1013 250m EC 2.22h 1.253 x 1013 251 EC 33h 8.40 x 1011 252 ex 472d 2.436 x 109

253 ex 20.47 d 5.596 x 1010

1673


Major SC Nuclide decay modea Half-li/eb (dis min-I J.tg-I)

254 IX 276d 4.134 x 109

254m p- 39.3 h 6.97 x 10" 255 p- 39.8 d 2.86 x 1010

256 p- 25.0 min 6.52 x 1013

256 p- -7.6h _ 3.57 x 1012

Fm 242 SF 0.8ms 1.30 x 1020

243 IX 0.18s 5.73 x 1017

244 SF 3.3 ms 3.11 x 1019

245 IX 4s 2.60 X 1016

246 SF 1.1s 9.25 x 1016

247 IX 35s 2.90 x 1015 247 IX 9s 1.1 X 1016

248 IX 36s 2.80 x 1015

249 IX 3 min 5.6 x 1014

250 IX 30 min 5.57 x 1013

250m IT 1.8 s 5.57 x 1016

251 EC 5.3h 5.23 x 1012

252 IX 25.4h 1.087 x 1012

253 EC 3.0d 3.82 x 10" 254 IX 3.24h 8.45 x 1012

255 IX 20.1 h 1.357 x 1012

256 SF 2.63h 1.033 x 1013

257 IX 100.5 d 1.122 x 1010

258 SF O.4ms 2.40 x 1020

259 SF 1.5s 6.45 x 1016

Md 247 IX 2.9 s 3.50 x 1016

248 EC 7s 1.40 X 1016

249 EC 24s 4.19 x 1015 250 EC 0.9 min 1.90 x 1015 251 EC 4.0 min 4.16 x 1014

252 EC 2.3 min 7.2 x 1014

254 EC 10 min 1.64 x 1014

254m EC 28 min 5.87 x 1013

255 EC 27 min 6.06 x 1013

256 EC 75 min 2.17 x 1013

257 EC 5.4h 5.01 x 1012

258 IX 55d 2.04 x 1010

258 EC 43 min 3.76 x 1013

259 SF 1.6 h 1.68 x 1013

No 250 SF 0.25ms 4.01 x 1020

251 IX 0.8 s 1.20 x 1017

252 IX 2.3 s 4.32 x 1016

253 IX 1.7 min 9.70 x 1014

254 IX 68 s 1.45 x 1015

254m IT 0.28 s 3.52 x 1017

255 IX 3.1 min 5.28 x 1014

256 IX 3.3 s 2.96 x 1016

1674


Major SC Nuclide decay mode- Half-li/eb (dis min-I Jlg-l)

257 IX 25 s 3.90 x 1015

258 SF 1.2ms 8.09 x 1019

259 IX l.00h 2.69 x 1013

Lr 253 IX 1.3s 7.6 X 1016

254 IX 13s 7.6 X 1015

255 IX 22s 4.46 x 1015

256 IX 28 s 3.5 x 1015

257 IX 0.65 s 1.50 x 1017

258 IX 4.3 s 2.26 x 1016

259 IX 5s 1.90 X 1016

260 IX 3.0 min 5.35 x 1014

104 253 SF -1.8 s 5.5 x 1016

254 SF O.5ms 2.0 x 1020

255 IX 1.4 s 7.0 x 1016

256 SF 7.4ms 1.32 x 1019

257 IX 4.3 s 2.27 x 1016

258 SF 13ms 7.5 x 1018

259 IX 3s 3.2 X 1016

260 SF 20ms 4.8 x 1018

261 IX 1.1 min 1.5 X 1015

262 SF 47ms 2.03 x 1018

105 255 IX 1.5s 6.5 x 1016

257 IX 1.4 s 7.0 x 1016

258 IX 4.4s 2.21 x 1016

260 IX 1.5s 6.4 x 1016

261 IX 2s 4.8 X 1016

262 SF 34s 2.8 x lOIS

106 259 SF ·0.48s 2.01 x 1017

260 IX, SF 3.6ms 2.7 x 1019

261 IX 0.26s 3.7 x 1017

263 IX 0.9 s 1.1 x 1017

107 261 SF 1.5 ms 6.4 x 1019

262 IX 4.7ms 2.03 x 1019

108 265 IX 1.8 ms 5.3 x 1019

109 266 IX 3.5 ms 2.7 x 1019

a Decay modes are denoted by: IX for alpha decay, fJ - for beta decay, EC for electron capture, IT for isomeric transition, and SF for spontaneous fission. The decay mode given in this column represents either the major decay mode or the only observed decay mode. b 1 year = 365.243 d. c Specific activity is given in units of disintegrations per minute per microgram and contains one more significant figure than the half-life in order to avoid rounding-off errors. 1 Curie (Ci) = 3.7 x 1010 dis S-1 = 3.7 X 1010 Sq.

AUTHOR INDEX Page numbers in italic refer to figures or tables.

Aarts, J., 1409 Abazli, H., 463, 1446 Abbe, D., 1317, 1318 Abdel-Gaward, A. S., 116, 121, 122 Abe, M., 125 Abel, E. W., 1547 Abelson, P. H., 4, 6; 181,443,444 Aberg, M., 1490, 1493, 1494, 1494, 1495, 1504 Abernathy, L. L., 270 Abragam, A., 1362, 1363 Abraham, J., 84 Abraham, D. M., 250, 251, 254, 675, 705, 707,

745, 749, 752, 753 Abraham, M., 971 Abraham, M. M., 1008, 1077, 1362, 1366,

1375, 1378, 1379, 1382 Abramson, R., 606, 623 Abu-Dari, K., 775, 779, 816 Ackerman, R. J., 223,227,228,231,264,599,

601,608,610,610,611,612,899,900, 901,973, 1315, 1322, 1337, 1341, 1389, 1390, 1397, 1565

Ackermann, R. H., 1321 Ackermann, R. J., 48, 50, 51, 52, 59, 60, 452,

456, 1279, 1280, 1315, 1320, 1321, 1334, 133~ 1340, 1341, 1347

Adair, M. L., 968, 970, 972 Adams, D. M., 72 Adams, E. T., 588, 598 Adams, F., 109, 110, III Adams, M., 548, 570 Adams, M. D., 334, 737 Adams, R. E., 288 Adams, R. M., 679 Adams, R. 0., 1337 Adamson, M. G., 1321, 1332, 1337 Adar, S., 1030 Addison, C. C., 412 Ader, M., 410, 412, 1317 Aderhold, c., 911, 996, 1050, 1373, 1375, 1462 Adi, M. D., 73 Adloff, J. P., 19, 25 Adolphe, C., 706 Adolphson, D. G., 75 Adrian, H. W. W., 1431 Adrianov, M. A., 621, 641, 642, 643, 645, 647,

648,649,651,652,653,654,656 Adwick, A. G., 683

AEC, 174, 175, 176, 177,178,180,287 Afanas'evaL T. W., 458 Affortit, C., 728, 1321, 1337 Agarwal, Y. K., 1644 Agron, P. A., 307, 308, 309 Agruss, M. S., 115 Ahmad, M. F., 1329 Ahrland, S., 142, 347, 349, 351, 352, 398, 483,

484,817, 1290, 1487, 1489, 1490, 1492, 1497, 1498, 1498, 1500, 1501, 1501, 1503, 1507, 1514, 1514, 1515, 1520, 1528

Aiken, A. M., 551 Aitken, E. A., 728, 1332, 1337 Akapiev, G. N., 1107 Akatsu, J., 567, 573, 577 Akella, J., 968, 969, 970, 1389, 1390 Akhachinskij, V. V., 56, 57, 58, 66, 234, 234,

236,23~238, 239,240,241,242,243, 281,282,283,283,288,288,455,641, 647, 653, 657, 659, 660, 1279, 1282, 1328, 1329, 1330, 1331, 1336, 1339, 1340, 1347, 1389, 1397

Akhtar, M. M., 1454 Akimoto, Y., 681, 904, 909 Akin, G. A., 177,325,326 Aksel'rud, N. V., 1289 Aksenova, N. M., 25 Albano, V. G., 1431 Albaugh, F. W., 727 Alberman, K. B., 270, 272 Albers, H., 390 Albertsson, J., 1509, 1528 Albrecht, E. D., 655, 667, 669, 670, 1433 Albridge, R. G., 106 Albutt, M., 2893 Alcock, C. D., 282, 306, 1318, 1321, 1329,

1330 Alcock, K., 1521, 1522, 1522 Alcock, N. W., 78, 1431, 1452, 1454, 1490,

1509 Alcock, P. B., 223 Al-Dahaer, A. G. M., 73 Alderhold, C., 1034 Aldred, A. T., 490, 902, 903, 904, 907, 1377,

1378 Aleksandrov, D. M., 1033 Alekseeva, D. P., 783 A1ekseeva, T. E., 1641

Author Index

Alenchikova, I. F., 753, 755, 756, 757, 1430 Alexander, C. A., 677, 691 Alexander, E. c., 505 Alexander, I. C., 62 Ali, S. A., 981, 1055, 1518 AlibegofT, G., 292 Aling, P., 1321, 1322, 1323, 1327 AI-Kazzar, A. G. M., 73 AI-Kazzar, A. M. S., 140, 141 AI-Kazzaz, Z. M. S., 74, 779, 780, 1458 Allard, B., 1170, 1171, 1172,1172,1173,1173,

1174, 1175, 1290, 1455 Allard, G., 56 Allbutt, M., 705, 706,708,709,710,711,712,

1435 Alleluia, I. B. de, 719, 720 Allen, A. L., 304 Allen, J. W., 1037 Allen, O. W., 208 Allen, R. E., 170 Allen, R. P., 623, 1403 Allen, S. J., 1372 Alles, A., 1327, 1328 Allesandri, U. A., 1372 Allison, G. M., 551 Allison, M., 23 Almasova, E. V., 1012 Alonso, C. T., 7, 1108, 1630 Alonso, J. R., 7, 1108, 1630 Alphen, P. V. van, 51 Alpress, I. G., 364 Alter, H. W., 521, 541, 1503 Alvey, P. J., 462, 779, 780 A1y, H. F., 992, 1011, 1055, 1080 Amano, R., 911, 1049 Amberger, H. D., 1362, 1374, 1375, 1376,

1554, 1558, 1577 Ames, D. P., 784, 802 Ammentorp-Schmidt, F., 141,383 Andelin, R. L., 619, 621 Anderegg, G., 1513, 1513 Anderko, K., 233, 234, 236, 237, 238, 239,

240, 241, 288, 290 Andersen, O. K., 999 Andersen, R. A., 83, 1551 Anderson, J. S., 75 Anderson, H. H., 756, 757, 766, 769, 770, 806 Anderson, H. J., 687, 727 Anderson, J., 681, 683, 694 Anderson, J. S., 270, 272, 1161 Anderson, J. W., 619, 621, 656 Anderson, M. R., 77 Anderson, O. K., 1395 Anderson, P. W., 1411 Anderson, R. A., 1432, 1605, 1606, 1611,

1611, 1612, 1612, 1622 Anderson, R. W., 304, 595, 597 Anderson, W. K., 270, 273

Andersson, J. E., 153 Andersson, S. 0., 1518 Andon, R. J. L., 1328, 1329 Andra, K., 390 Andreev, E. I., 971, 978 Andreev, V. I., 912 Andreev, V. J., 1050, 1059, 1291 Andreeva, M. A., 810 Andrews, H., 547 Andrews, H. C., 25, 26 Andreychuck, N. N., 827 Andrieux, L., 283, 285 Andruchow, W., Jr, 84 Angelucci, 0., 75, 77 ANL,1314 Ans, J. de, 81 Ansara, A., 1279, 1282, 1328, 1329, 1330,

1331,1336,1339, 1340, 1347 Ansara, I., 56, 57, 58, 66, 234, 234, 236, 237,

238,239,240,241,242,243, 281, 282, 283, 283, 288, 288, 455, 641, 657, 659, 660, 1279, 1282,1328, 1329, 1330, 1331, 1336, 1339, 1340, 1347, 1389, 1397

Anselin, F., 669, 675, 677, 679 Anthony, A. M., 260, 263 Antill, J. E., 227 AntonofT, G. N., 104 Aoyagi, M., 994, 1034 Apgar, S. A., III, 595 Apraksin, I. A., 77 Arajs, S., 232 Arapaki, H., 152 Arapaki-Strapelias, H., 122, 142, 146, 153 Arbman, E., 106 Arden, T. V., 347, 352 Arder, S., 394, 395 Ardisson, C., 106 Ardisson, G., 106 Arendt, J. W., 308 Argruss, M. S., 104, 113, 114, 115 Arita, K., 67 Arke1, A. E. van, 51, 53 Arkipov, V. A., 1335 Arkipova, N. F., 1641 Arko, A. J., 232, 292, 295, 614, 615, 617,

1395, 14tO, 1412, 1412 Armagan, N., 1431, 1458 Armbruster, P., 7, 1110, 1112, 1630, 1644 Armstrong, D. E., 895, 1530, 1536 Arnaudet, L., 1596, 1598 Arnek, R., 1495, 1496 Arnold, G. P., 56, 62, 667, 1433 Arnoux, M., 19, 25 Aronson, S., 61, 63, 1322 Arrowsmith, H. W., 1403 Artna-Cohen, A., 106 Artyukin, P. A., 814, 815 Artyukin, P. I., 812, 813, 814, 818, 819, 822

Author Index

Arutyunyan, E. G., 1452 Asano, M., 57 Ashbrook, A., 1518 ASM,I405 Asprey, B., 319, 587 Asprey, L. B., 67, 68, 126, 128, 135, 136, 137,

152, 306, 318, 319, 456, 702, 752, 757, 769,804, 806, 818,820, 887, 895, 897, 900,902,903,904,910, 911, 912, 913, 915,917,918,919,922,926,927,928, 929,967, 972, 973, 974, 978, 996, 1004, 1005, 1033, 1035, 1036, 1036, 1037, 1042, 1045, 1046, 1050, 1077, 1260, 1265, 1431, 1440, 1441, 1444, 1445, 1481, 1482, 1530, 1536

Astheimer, L., 151, 196, 398, 1501, 1507 Aston, F. W., 181 Astrom, B., 1096 Atabeck, E., 1333, 1340, 1343 Aten, A. H., Jr, 1053 Atherton, N. J., 125 Atlas, L. M., 684, 697 Atterling, H., 1096 Atwood, J. L., 83, 381, 1459, 1460, 1563, 1596 Aubin, L., 1091, 1483 Auer, C., 41 Auerman, L., 1009 Auerman, L. N., 1034, 1053, 1081, 1091,

1095, 1344, 1345, 1481 Auge, R. G., 544, 546 Aurov, N. A., 1333, 1334 Auskern, A. B., 61,63 Avdeef, A., 83, 382,383, 1462, 1573, 1574 Avignant, D., 67, 71, 1446 Avivi, E., 646, 656, 657 Avogadro, A., 1170 Avona, V. L., 500 Avril, R., 1231 Awasthi, S. K., 457, 715, 717 Awwal, M. A., 1518 Axe, J. D., 125, 1370 Axelson, B., 215 Ayling, S., 340 Aymonino, P. J., 82 Aziz, A., 979, 980, 981, 1507

Baaso, D. L., 452 Babcock, B. Q., 593 Babelot, J. F., 1321, 1328, 1337 Babko, A. K., 1504 Babrova, V. N., 515 Bach, R. A., 270 Bacher, W., 309,314 Bachmann, H. G., 358 Bacon, W. E., 78 Baenziger, N., 327 Baenziger, N. C., 60, 61, 284, 289 Baerands, E. J., 1273

Baes, C., 352 Baes, C. F., Jr, 85, 206, 362, 368, 979, 1141,

1287, 1289, 1484, 1485, 1486, 148~ 1492, 1495, 1496, 1497, 1505

Baetsle, L. H., 16, 25, 26, 27 Bagawde, S. V., 1498, 1499, 1503, 1514 Bagnall, K. W., 12, 15, 69, 72, 73, 74, 75, 78,

83, 84, 135, 136, 139, 325, 326, 327, 334, 456,461,462,703,887,903, 911, 962, 971, 1442, 1443, 1444, 1446, 1447, 1452, 1455, 1458, 1460, 1556, 1557, 1560, 1561, 1562, 1569

Bagnall, V. W., 129, 141 Bagrova, V. I., 641,653 Baibuz, V. F., 1279 Baidron, M., 129 Bailey, D. M., 69, 74, 1441 Bailey, W. E., 690, 728, 728, 729 Bairot, H., 697 Baisden, P. A., 1080, 1092, 1094, 1095, 1481,

1644 Baker, E. C., 1458, 1460, 1463 Baker, F., 921 Baker, F. B., 1536, 1538 Baker, R. D., 224, 590, 591,592,593 Bakes, E., 574, 575 Bakes, S. E., 574, 578, 733 Balagna, J. P., 551 Balakaeva, T. A., 79 Balakayeba, T. A., 81 Balcazar Pinal, J. L., 74 Baldock, C. R., 177 Baldwin, C. E., 544, 546, 593 Baldwin, N. L., 54, 56 Baldwin, W. H., 465, 911, 1448, 1449, 1454,

1456,1461 Ball, J. G., 588, 598, 614 Ballhausen, C. J., 219, 220 Baluka, M., 461, 1440 Band, W. D., 686 Banic, G. M., 503 Banick, C. J., 963 Banks, C. V., 82 Banks, R., 1440 Banks, R. H., 141,461,463,464,468, 1376,

1575 Bansal, B. M., 970, 1432 Bansal, B. M. L., 1507 Baran, E. J., 82 Baranov, A. A., 1012, 1013, 1014 Baranov, A. Yu., 974, 1004 Barbanel, Yu. A., 463, 926, 967, 971 Barbe, B., 645, 657 Barber, C. M., 1327 Barber, E. J., 315 Barbieri, G. A., 82 Barclay, G. A., 1431, 1452, 1517 Bard, A. J., 396

Author Index

Bardeen, J., 51 Barghusen, J., 559 Barin, I., 223 Barinov, V. I., 1331 Barker, J. J., 673 Barker, M. G., 62 Barketov, E. S., 1056 Barnanov, A. A., 1050 Barnard, R., 336, 337, 347 Barnes, A. H., 177 Barnes, E., 227 Barnes, J. W., 551 Barnes, R. F., 996, 1030, 1050, 1081 Barnett, G. A., 485 Barnett, M. K., 368 Barnighausen, H., 1456 Barre, M., 80, 81 Barrett, S. A., 271 Barringhausen, H., 1047 Barry, J. A., 132 Barsukova, K. V., 992 Barten, H., 1328 Barthelemy, P., 674 Barthellier, A., 538 Bartolin, H., 292, 294 Barton, C. J., 661, 662 Barton, P. G., 1180 Bartram, S., 55 Basile, L. J., 930 Baskerville, C., 71, 75, 80 Baskin, Y., 60, 63, 293, 676 Bastin-Scoffier, G., 22 Bates, C. F., 1483 Bates, J. L., 904, 909 Bathellier, A., 538, 539, 893 Batlogg, B., 1411 Battles, J. E., 671, 691, 691, 692, 693, 694 Bauche, J. K., 1227 Bauche-Arnoult, C., 1227 Baud, G., 270, 271 Bauer, A. A., 233, 234, 234, 236, 237, 238,

239,240,241,289,290 Bauer, D. P., 1574, 1577 Bauer, R. S., 1037 Baumann, E. W., 1501 Baumbach, H. L., 589, 598, 643 Baumgartner, F., 84, 141, 379, 381, 506, 526,

528, 533, 534, 9ll, 977, 1166, 1367, 1368, 1370,1371, 1373, 1375, 1461, 1550, 1552, 1553, 1554, 1559

Bauminger, E. R., 581 Bayat, I., 1056 Baybarz, R. D., 29, 126,218,887,890,893,

894, 895, 899, 900, 902, 903, 904, 907, 909,910,911, 9ll, 913, 915, 917, 918, 926, 964, 965, 968, 970, 972, 974, 975, 976, 979, 992, 993, 995, 996, 998, 999, 1000, 1001,1003, 1004, 1006, lOll, 1012,

1013, 1013, 1014, 1030, 1031, 1033, 1035, 1036, 1036, 1037, 1039, 1041, 1042, 1043, 1044, 1045, 1046, 1047, 1048, 1052, 1052, 1053, 1055, 1056, 1058, 1075, 1077, 1078, 1080, 1081, 1091, 1260, 1280, 1432, 1439, 1440, 1441, 1447, 1448, 1481

Bazan, C., 292, 295, 1410 Beahm, E. C., 1318, 1329 Beams, J. W., 182 Bearden, J. A;, 29, 49, 215, 580 Beasley, M. C., 9(J4 Beasley, M. L., 976 Beaumont, A. J., 516, 567, 570 Bebikh, G. F., 982 Beck, P. A., 1398,1398 Becker, E. W., 182 Beckman, 0., 215 Beckmann, W., 16 Becquerel, A. H., 3, 169, 368 Begun, G. M., 484, 930, 998, 1007, 1538 Beheshti, A., 1561, 1562, 1569 Behesti, A., 83 Beintema, C. D., 282, 361 Beintema, J., 1453 Beitz, J. V., 976, 995, 996, 997, 998, 1255,

1272 Bellamy, R. G., 197 Bell, J. T., 222, 396,928, 1264, 1531 Bell, M. J., 891 Bell, W. A., 503 Belle, J., 256, 260, 266, 280, 1322 Belov, V. Z., 1090, 1091, 1102, 1106, 1107,

1108 Belyaev, Yu. I., 456, 1338 Belyakova, Z. V., 78 Belyatskii, A. F., 25 Bemis, C. E., Jr., 994, 1076, 1088, 1090, 1096,

1097, 1098, 1101, llOI, 1104, 1105, 1107 Bemiss, C. E., 217, 1630, 1643 Bendict, G. E., 687 Benedict, G. E., 186,447, 501, 513, 554,687 Benedict, M., 174 Benedict, U., 127,680,684, 725, 725,'900,

902, 904, 907, 908, 970, 972, 975, 976, 999, 1037, 1061, 1152, 1153, 1389, 1390

Benedict, V., 127 Benesova, M., 1505 Benesovsky, F., 54, 56 Benes, P., 1130, ll62 Benetollo, F., 1431, 1557, 1558 Benjamin, B. M., 83, 381, 1563 Benker, D. E., 993, 1031 Bennelick, E. J., 662 Bennett, M. R., 184, 186 Ben Osman, Z., 212, 212, 213, 1226 Benny, J. A., 133 Benrath, A., 362 Bentley, W. C., 963

Author Index

Benz, R., 61, 62, 63, 66, 1338, 1340, 1436 Benznosikova, A. V., 641, 653 Berdonosov, S. S., 1095 Berg, J. 0., 215 Berger, M., 1375, 1376 Berger, R., 1012, 1013 Bergman, A. G., 67, 70, 72, 1279 Bergstrom, G., 1493 Bergvall, P., 215 BerIincourt, T. G., 232, 233 Berman, A. S., 174 Berman, H., 191,1453 Bernal, J. D., 85 Bernardinelli, R. J., 186 Berndt, A. F., 648, 652, 655 Berndt, A. F., Jr., 241 Berndt, U., 300, 718, 720, 722,904, 907, 909 Bernhardt, H. A., 311 Bernstein, E. R., 255, 255, 256, 257, 258,

1362, 1432 Berryhill, S. R., 1463, 1574, 1576, 1577, 1578 Berry, J. W., 544, 546, 890, 899 Bersin, Th., 390 Bertant, F., 1432, 1434 Bertaut, F., 54, 56, 82 Bertha, E. L., 937 Berthold, H. J., 289 Bertino, J. P., 224 Berzelius, J. 1., 41, 52, 61, 64, 66, 67, 71, 73,

74, 75, 77, 79, 80, 81, 82 Besancon, P., 706 Besmann, T. M., 1297, 1318, 1329, 1337 Best, G. F., 1521, 1522 Betts, R. H., 338, 339, 349, 352, 582, 1495,

1496 Beyerlein, R. A., 53, 54 Beyrich, W., 182 Bezjak, A., 1454 Beznosikova, A. V., 648, 650, 651, 652 Bhandari, A. M., 141 Bhatki, K. S., 19, 25 Bhupathy, M., 1317, 1323 Bibler, N. E., 974, 976 Bidoglio, G., 1170 Bidwell, R. M., 621 Bieganski, Z., 1327 Bier, K., 182 Bierman, S. R., 502, 502, 899 Bigeleisen, 1., 174 Bigelow, J., 965 Bigelow, J. E., 891, 893, 965, 990, 993, 1028,

1031, 1032, 1087, 1088 Biggers, R. E., 222, 396, 1531 Biggs, F., 1035 Billiau, F., 1579 Billich, H., 379, 977, 1551, 1553 Biltz, W., 52, 66, 293 Bindschadler, E., 387, 389, 394,395

Binnewies, M., 72, 73, 85 Biradar, N. S., 84 Birkel, I., 1037 Bishop, D. 1., 1411 Bismondo, A., 1507, 1508, 1510, 1517 Bittner, H., 55 Bixby, G. E., 620 Bixon, M., 1335 Bjorkland, C. 1., 677 Bjorkland, C. W., 680, 683, 687, 690, 699,

700, 700, 701, 1453 Bj0rnholm, S., 19, 25 Black, R. M., 700 Blackburn, P. E., 671, 691, 692, 1321, 1322 Blackledge, J. P., 1432 Blair, A., 325, 327 Blaise, A., 139,295,297, 710, 711,969, 1326,

1327, 1328, 1372, 1377, 1379 Blaise, 1., 47, 212, 212, 213, 214, 577, 578,

579, 580, 1034, 1050, 1224, 1225, 1226, 1227, 1228, 1229, 1237

Blaise, J. K., 995 Blake, C. A., 206, 359 Blakey, R. C., 270, 272 Blancard, 1., 1231 Blanco, R. c., 234 Blanco, R. E., 186,529 Blank, H., 13,588,589,621,623,641,642,

643, 644, 646, 647, 649, 652, 659, 680, 684,725

Blanke, B. C., 16 Bleaney, B., 1362, 1363 Bleany, B., 1186 Blitz, W., 392 Bloembergen, N., 1251 Blokhin, N. B., 925, 926 Blokin, V. I., 487 Bloomquist, C. A. A., 450, 451, 894, 897, 992,

1030, 1091, 1094 Bloomster, C. H., 623 Bluestein, B. A., 574, 576 Blum, P., 54, 56, 283, 1432, 1434 Blum, P. L., 282 Blume, D., 389, 394, 395 Blume, M., 1372 Blumenthal, 8., 227, 595 Blunck, H., 62 Blyckert, W. A., 502, 502 Boatner, L. A., 1008, 1077, 1362, 1366, 1375,

1378, 1379, 1382 Bobkov, Y. V., 599, 606 Bobleter, 0.,551 Bochvar, A. A., 621, 623, 641, 642, 643, 644,

645,648,650,651,653,654,655,656, 660

Bock, E., 77 Bock, R., 77 Bode, D. D., 996, 997, 1074, 1075, 1088

Author Index

Boden, R., 992 Boerrigter, P. M., 1273 Boeuf, A., 1378 Boeyens, J. C. A., 1456 Bogacz, A., 1332 Bogatskii, A. V., 77 Bogdanovic, B., 83 Boggs, J. E., 61 Bohet, J., 29, 126, 968, 970, 972, 1320 Bohm, M., 701, 763, 766, 767 Bohres, E. W., 82, 140, 141, 1367 Boisbaudran, L. de, 60 Boivineau, J. C., 725, 727 Bok, L. D. C., 84, 1456 Boldt, A. L., 893 Bole, A., 71 Bolton, W. von, 52, 71, 73 Bombieri, G., 1430, 1431, 1442, 1452, 1458,

1460, 1504, 1516, 1557, 1558, 1560, 1561, 1562

Bomse, M., 903, 931 Bond, W. D., 965 Bones, R. J., 695, 696, 696, 698, 1321 Bonnell, P. H., 678 Bonnelle, C., 215 Bonner, N. A., 446, 503 Bonnet, M., 146 Boocock, G., 1180, 1181 Boom, R., 636, 637 Booth, H. S., 304 Bordarier, Y., 1217 Boring, A. M., 1271 Borisov, S. V., 1442 Borlera, M. L., 80, 81, 1453 Borsese, A., 66 Borzone, G., 66 Bos, K., 172, 173, 174, 175, 500, 554 Bottari, E., 1513 Boucher, R., 606, 674 Boucher, R. R., 674, 902 Bouder, R., 623 Boudreaux, E. A., 1366 Bougon, R., 319, 1324 Bouissieres, G., 15, 30, 32, 129, 134, 149,

1005, 1046, 1052, 1077, 1091, 1313, 1482, 1483, 1489, 1490

Bourderie, L., 1055 Bourges, J. Y., 913, 917, 918, 926, 928 Bourion, F., 71, 74 Bourion, R., 71 Boutard, J. L., 1317, 1318 Bovey, L., 213 Bowen, S., 893 Bowen, S. M., 981 Bowersox, D. F., 641, 645, 654, 655 Bowie, S. H. U., 187, 190, 192, 193, 195 Bowman, A. L., 56, 1433 Bowman, K., 1431, 1455

Bowman, M. G., 25, 29 Bowman, R. G., 1616 Boxer, L. W., 192 Boyd, G. E., 563, 572 Boyle, J. S., 368 Bozzola, S., 247 Brabers, M. J., 27, 82 Brachet, G., 902 Bradbury, M. H., 127, 1320, 1337 Bradley, D. C., 84, 326, 390 Bradley, D. G., 73 Bradley, M. J., 287 Brady, J. D., 1092, 1095, 1481, 1483 Braga, D., 1431 Brand, J. R., 465, 469 Brandau, E., 1055, 1507 Brandi, G., 1169, 1458, 1459 Brandi, G. T., 1548 Brandl, 8., 335 Brandt, L., 483, 484, 1498, 1500, 1503, 1520 Brandt, S. S., 184, 186 Brater, D. C., 309 Bratsch, S. G., 1293 Brauer, G., 56, 270, 276 Brauer, F. P., 551 Brault, J. W., 1226 Bray, J. E., 1376 Bray, L. A., 700, 889, 896 Brcic, B. S., 319 Bredl, C. D., 1409 Breeze, E. W., 295, 296, 297 Breizy, C. E., 690 Brennan,1. G., 1551 Brett, N. H., 295, 296, 297, 690, 717, 718,

720, 722, 725, 727 Brewer, H., 1203, 1204 Brewer, L., 29, 56, 59, 64, 65, 218, 265, 293,

329, 398, 462, 628, 633, 634, 635, 690, 697, 700,966, 994, 1033, 1040, 1075, 1237, 1239, 1258, 1261, 1631

Brickwedde, F. G., 1323 Bridger, N. J., 676, 678, 1366, 1435 Bridgman, P. W., 51, 612 Briggs, E. A., 1035 Briggs, G. G., 53, 67 Briggs, R. 8., 317,325 Brillard, L., 931, 935, 942, 980, 1010, 1011,

1054, 1055, 1057, 1080, 1483 Brintzinger, H., 52 Brisianes, G., 287 Brisi, c., 270, 271 Britt, R. D., 487 Brittain, R. D., 1323, 1324 Britton, H. T. S., 81 Brletic, P. A., 1333 Broach, R., 1614, 1615 Broach, R. W., 1460 Brochu, R., 294, 295, 296

Author Index

Brock, C. P., 1567, 1608, 1623 Brockway, M. C., 718 Brodsky, M. B., 232, 233, 453, 488, 491, 595,

614,615,617, 899, 1366, 1379, 1394, 1395, 1406, 1407, 1407, 1408, 1408, 1409, 1411

Bromisz, S. E., 614 Bromley, L., 697, 700 Bromley, L. A., 59, 64, 65, 265, 293, 329, 398,

462 Brooks, M. S. S., 139 Brooksbank, R. E., 186 Bros, J. P., 1332 Brossmann, G., 621, 623, 642 Brown, A., 54, 56, 195, 1433 Brown, D., 12, 66, 67, 69, 72, 73, 74, 75, 84,

126, 132, 133, 134, 135, 136, 137, 138, 139, 141, 145, 298, 303, 319, 326, 327, 334, 335, 383,461,462,463,464,887, 902,903,910,969,971, 1000, 1040, 1076, 1148, 1267, 1269, 1309, 1310, 1311, 1320, 1341, 1343, 1369, 1369, 1401, 1430, 1439, 1440, 1441, 1442, 1443, 1444, 1444, 1446, 1446, 1447, 1448, 1455, 1456, 1458, 1556, 1557, 1574, 1575

Brown, E. D., 75, 79, 81 Brown, F., 662, 663, 669,675 Brown, G. H., 78 Brown, G. M., 1445, 1460, 1614, 1615 Brown, H., 255, 256 Brown, H. C., 394, 395 Brown, H. D., 511 Brown, J. C., 544, 546 Brown, J. D., 1242, 1258 Brown, K. B., 186, 195,206,359, 1521 Brown, L. D., 1460 Brown, N. L., 540, 567 Brown, P. L., 85 Brown, R. T., 1035 Brown, W. A., 516, 567 Brown, W. D., 701 Browne, C. I., 6, 551, 1086 Browne, E., 990 Browne, J. C., 1500 Browne, W. M., 1071 Bruce, F. R., 506, 551, 561,570 Bruchertseifer, H., 1644 Briichie, W., 1644 Bruger, J. B., 1033 Briigger, M., 1644 Bruin, T. L. de, 48 Brumme, G. D., 1321, 1337 Brun, T. 0., 53, 54, 1395, 1396 Brundage, R. T., 1257 Brunelli, M., 1169, 1459, 1460, 1548, 1549,

1549 Brunn, H., 60 Bruno, J. W., 84, 1551, 1552, 1593, 1594,

1598, 1600, 1602, 1602, 1605, 1610 Bruns, L. E., 542, 543 Brunton, G., 67, 68, 70, 71, 1445,1446 Brunton, G. D., 320 Briiser, W., 83, 1463, 1592 Bruyne, R. de, 82 Bryan, G. H., 677 Bryan, R. G., 487 Bryukher, E., 25 Buchanan, J. M., 1503 Bucher, E., 65 Bucholz, C. F., 399 Buckingham, J. S., 487 Bug!, J., 289 Buhrer, C. F., 292, 1435 Buijs, 891 Buijs, K., 29, 126, 127,902,904,965,968,

970,972 Bukhsh, M. N., 146, 149 Bukianov, G. V., 1106, 1644 Bullock, I., 336, 337, 347 Bullock, J. I., 1454, 1524, 1524 Bulman, J. B., 51 Bulman, R. A., 1178, 1180, 1181, 1183, 1184 Bunce, J. L., 677 Bunker, M. E., 551 Bunnell, L. R., 287 Burdese, A., 80, 81, 1453 Burgess, J., 1141 Burghard, H. P. G., 141, 1575 BurghotT, H., 182 Burkhart, M. J., 1537 Burleson, C. E., 232 Burmeister, J. L., 1514 Burnett, J., 971 Burnett, J. L., 29, 903, 913, 915, 917, 918,

976,979,995, 1000, 1012, 1013, 1013, 1037, 1040, 1045, 1052, 1052, 1053, 1058, 1076, 1077, 1081, 1280, 1281, 1282, 1297, 1315, 1397, 1481, 1636, 1641

Burney, G. A., 12,447,451,457,467,473, 485,486,487,501,896,902,911,976

Burnham, J. B., 671, 687 Bums, J., 1553 Bums, J. A., 1335, 1336 Bums, J. H., 83, 306, 379, 379, 381, 382, 461,

464,465,897,903,907,908,911,971, 972, 973, 976, 977, 998, 1003, 1005, 1006, 1007, 1037, 1041, 1042, 1043, 1046, 1048, 1050, 1057, 1323, 1435, 1436, 1439, 1440, 1441, 1442, 1442, 1443, 1445, 1447, 1448, 1448, 1449, 1452, 1453, 1454, 1454, 1456, 1457, 1459, 1459, 1460, 1461, 1554, 1554, 1563, 1564

Burr, A. F., 29, 49, 216, 216, 580 Burris, L., Jr, 541 Burton, D. A., 452 Burton, M., 1594

Author Index

Burwell, R. L., Jr, 1616 Busch, G., 292, 293, 294 Buschow, K. H. J., 55 Busey, R. H., 1291 Bush, R. A., 623 Bushuev, N. N., 82 Butcher, J. A., 1577 Butler, J. E., 1368 Butler, T., 327 Butler, T. A., 1527' Butterfield, D., 30 Buyers, W. J. L., 1407 Byrne, J. T., 619, 621

Cabell, M. J., 23, 25, 26 Cain, A., 924 Caira, M. R., 1442, 1443 Caird, J. A., 996, 1034, 1050 Caldwell, J. J., 690 Calestani, G., 139 Caletka, R., 116, 1098, 1102, 1106 Cali, R., 1517 Californium 252 Progress Reports, 1029 Calkins, V., 326 Callderazzo, F., 1455 Callihan, D., 502, 502 Calvin, M., 84,394,816,817 Cameron, A. E., 177 Cameron, J., 192 Campbell, D.O., 145, 896, 993, 1031, 1074 Campbell, G. M., 668, 672, 677, 1338, 1339 Campbell, W. M., 539 Camus, P., 995, 1226, 1228 Candela, O. A., 1372 Canneri, G., 79 Cannon, J. F., 54,56 Capocchi, J. D. T., 53 Caputi, R. W., 1332, 1337 Cardiac Pacemakers and Mechanical Hearts,

501 Carleson, G., 918, 1528 Carlier, R., 151, 152 Carls, E. L., 740 Carlson, L. R., 1231 Carlson, O. N., 50,50 Carlson, T. A., 29, 898, 899, 994, 995, 1034,

1088,1090, 1098, 1101, 1292, 1293, 1635, 1636,1641

Carnall, W. T., 13, 218, 219, 396,459,464, 468, 577, 578,579, 580, 585, 587, 731, 784, 785, 802, 902, 903, 911, 911, 913, 914, 926, 976, 978, 995, 996, 997, 998, 1033, 1034, 1047, 1050, 1058, 1058, 1059, 1059, 1081, 1222, 1227, 1235, 1237, 1247, 1249, 1251, 1254, 1255, 1256, 1260, 1264, 1267, 1271, 1272, 1272, 1273, 1362, 1373, 1380

Camiglia, S. C., 582, 731, 734,903

Caroli, S., 398 Carr, E. M., 282 Carr, W. H., 548, 570 Carrano, C. J., 1187 Carrara, C. J., 394 Carrere, J. P., 150 Carritt, D. E., 540, 567 Carroll, D. F., 674, 675, 714 Carsell, O. J., 123 Carswell, D. J., 124, 1518 Carter, F. L., 1034 Carter, J. M., 326 Carter, R. D., 502, 502 Carter, W. J., 1251 Carvalho, R. G. de, 932, 944, 946, 980, 1054,

1056, 1058 Case, F. N., 181 Case, G. N., 1099, 1483 Casellato, U., 78, 1450 Casey, A. T., 145, 149 Casey, C. P., 1623 Casimir, H., 1244 Cassol, A., 484, 795, 796, 799, 807,808, 1492,

1493, 1493, 1507, 1508, 1509, 1510, 1516, 1517

Catenet, J. J. de, 612 Cathers, G. I., 452, 548, 570 Caton, R. H., 53, 54 Cauchetier, P., 486, 1513 Cauchois, Y., 125,215, 580 Caughlan, C. N., 1452 Cavendish, J. H., 53, 67 Cavin, O. B., 54, 56 Cazaussus, A., 141, 142 Cefola, M., 659 Cercignani, C., 1321 Cermak, A. F., 534 Cemia, E., 1458, 1573 Cesari, M., 1459, 1463, 1572, 1593, 1593, 1596 Chackraburtly, D. M., 761, 762 Chackraburtly, D. M., 669, 670, 714, 715,

717, 718, 1434, 1454 Chackravarti, B. M., 326, 390 Chakravorthy, V., 121 Chambers, J. Q., 1577 Chan, S. K., 709, 711, 1378, 1394, 1407 Chander, G., 788 Chander, K., 1483 Chandrasekharaiah, M. S., 456, 1315, 1322,

1337,1341 Chang, A. T., 264, 1322 Chang, C. C., 1550, 1573 Chang, C. T., 1550, 1573 Chang, H. P., 116, 125 Chang-Wen-Ching, 812, 815 Charpin, P., 267, 319, 1324, 1456, 1458 Charvillat, J. P., 139,270,271,902,904,907,

908, 969, 970, 972, 975, 976, 1435

Author Index

Chasanov, M. G., 644,1321 Chatelet, I., 1231, 1327 Chatt, I., 72, 1497 Chatterjee, A. K., 326, 390 Chattin, F. R., 993, 1031 Chauvenet, E., 52, 62, 67, 71, 72, 73, 74, 75,

76,79 Chavastelon, R., 80 Chavrillat, I. P., 460 Chayawattanangkur, K., 19 Cheborarev, N. T., 757 Chebotarev, N. I., 621, 641, 642, 643, 645,

647, 648, 649, 651, 652, 653, 654, 656 Chebotarev, N. T., 599, 606, 621, 623, 641,

642,643,644,645,648,650,651,652, 653, 654, 655, 656, 660, 756, 75~ 1430

Chebotarev, N. V., 641, 653 Cheda, I. A. R., 76, 1317 Chelnokov, L. P., 1106, 1107 Chern. Eng. News, 192, 204 Chemical Processing of Irradiated Fuels, 506 Chemistry of Uranium and Plutonium, 567,

572 Chemla, M., 1080 Chen, B., 77 Chen, M. H., 1034 Chen, M. M. H., 994 Cheng-chi Kuo, 191 Chepigin, V. I., 1644 Chepovoy, V. I., 1012 Cherdyntsev, V. V., 503 Chereau, P., 695, 725 Cheriau, P., 1297, 1316, 1337 Chemorukov, N. G., 82 Chemyaev, I. I., 79 Chemyayev, I. I., 336, 347, 348,350, 351, 353,

354, 359, 360, 363 Chemyayevskaya, N. B., 515, 806 Chemyi, A. V., 648, 650, 651, 652 Chervet, I., 191, 197 Chesne, A., 447, 448, 448, 538 Chetham-Strode, A., Ir, 120 Chetverikov, A. P., 963 Chevalier, R., 67, 68, 71, 1446 ChevaJ1ier, A., 17 Chevallier, I., 17 ChevaJ1ier, I. C., 250 ChevaJ1ier, P., 106 Cheveau, P., 728 Chiakhorskii, A. A., 456, 465, 469 Chiarizia, R., 482, 483 Chikalla, T. D., 287, 456, 643, 671, 680, 683,

690, 697, 904, 909, 909, 911, 974, 1003, 1004, 1004, 1341

Childs, W. 1., 1226, 1264, 1272, 1272 Chilton, G. R., 1337 Chilton, I. M., 146, 183 Chiotti, P., 52, 56, 57, 57, 58, 60, 61, 66, 69,

72, 74, 75, 229, 232, 234, 234, 236, 237, 238,239,240, 241, 242, 243, 281, 282, 282, 283, 283, 284, 288, 288, 290, 455, 641, 657, 659, 660, 1279, 1282, 1328, 1329, 1330, 1331, 1336, 1339, 1340, 1347, 1389, 1397, 1440, 1441

Chipman, I., 590, 591 Chirkov, A. K., 974 Chirkst, D. E., 1332, 1333, 1334, 1445 Chistyakov, V. M., 456, 923, 925 Chiswick, H. H., 247 Chmertova, M. K., 982 Chmidt, V. S., 982 Chmutova, M. K., 804, 810, 816, 993, 1031,

1057,1080 Chmutova, M. S., 12,887,892 Choi, I. K., 1298, 1302, 1331, 1336 Choivalsek, 1644 Chong, C. H. H., 701 Chopey, N. P., 533 Choporov, D. Y., 462 Choporov, D. Ya., 731, 734, 903, 1338, 1341 Choppin, G. R., 7, 13, 506,508, 799, 887,

893, 895, 915, 930, 931, 932, 933, 934, 937,943, 944, 946, 947, 979, 980, 981, 982, 1010, lOll, 1012, 1030, 1054, 1055, 1056, 1057, 1058, 1074, 1088, 1091, 1092, 1094, 1125, 1126, 1127, 1128, 1171, 1176, 1499, 1502, 1503, 1507, 1510, 1513,1514, 1527, 1528, 1530

Chrisney, I., 577, 578, 579, 585 Christ, C. L., 1450 Christensen, D. c., 593, 595 Christensen, E. L., 516, 540, 550, 553,554,

558, 559, 561, 566, 567, 568, 570, 574, 575, 700, 747

Christensen, T. E., 215 Chu, Y. Y., 17,963 Chuburkov, Y. T., 1098, 1102, 1106 Chudinov, E. G., 462, 487, 731, 734,903, 982,

992, 1010, 1057, 1074, 1081, 1338, 1341 Chudnovskaya, G. P., 463 Chydenius, I. I., 52, 60, 65, 67, 71, 72, 73, 75,

76, 79, 80, 81 Ciavatta, L., 1504 Ciliberto, E., 1560, 1600 Ci1indro, L. G., 939, 942 Cinader, G., 1377, 1378 Cinneide, S. 0., 1504 Cirafici, S., 1318 Claasen, H., 743 Claassen, H. H., 1272 Clark, G. L., 73 Clark, G. W., 688 Clark, H. M., 123 Clark, J. P., 83 Clark, J. R., 1450 Clark, R. J., 75

Author Index

Clarke, G. W., 971 Clarke, R. W., 15 Clayton, E. D., 502, 502, 899 Clayton, H., 1329 Clegg, J. W., 191, 197,201,203,204 Cleve, P. T., 60, 72, 73, 75, 77, 79, 80, 81, 82 Cleveland, J. M., 12,465,467,500,513,521,

525, 534, 548, 567, 570, 571, 572, 574, 593, 598, 620, 658, 664, 665, 677, 678, 700,703, 732,760, 798,800,801,819, 835,838, 839, 1291

Cleveland, O. H., 359 Clinch, J., 392 Clincton, J., 55 Cline, D., 67, 73 Clinton, S. D., 183 Clusius, K., 181 Coanes, P., 212, 212 Cobble, J. W., 465, 469, 472 Cobble, R. W., 1291, 1327 CODATA, 1315, 1321, 1322 Codding, J. W., 106, 109, 110, 124 Coffinberry, A. S., 500, 588, 590, 591, 598,

599,605,606,612,613,620,621,623, 642,643,644,645,646,647,648,649, 650

Coffinberry, W. N., 652, 653, 654 Cogliati, G., 679 Cohen, A., 1053 Cohen, D., 217, 217, 218, 219, 396, 456, 465,

467,470, 471, 472, 475, 476, 477, 479, 480, 482, 483, 488, 489, 582, 784, 786, 787,802,806,899,908,911,912,913, 926, 970, 979, 995, 996, 998, 1003, 1006, 1012, 1042, 1043, 1046, 1081, 1137, 1260, 1335, 1441, 1443, 1481, 1482, 1536, 1537, 1538

Cohen, J., 614, 616 Cohen, K., 174, 176 Cohen, L. H., 1053 Colani, A., 73, 74, 81, 364 Coleman, C. F., 206, 538, 540,979, 1011,

1054, 1056, 1080, 1521 Coleman, G. H., 12 Coleman, J. A., 920, 921, 921 Coleman, J. S., 895, 902, 903, 904, 913, 914,

917, 918, 920, 976, 978, 1530, 1536, 1538 Coli, 802, 806 Collins, D. A., 104, 113,114,117,118,120,

456 Collins, E. D., 542, 891, 893, 965, 990, 993,

1031, 1032, 1087, 1088 Collman, J. P., 1547 Collongues, R., 60 Colsen, L., 968, 970, 972 Colson, L., 29, 126 Colvin, C. A., 486 Colvin, R. V., 232

Compton, V., 227 Comstock, A. A., 604, 612, 614, 615, 616 Comyns, A. E., 364 Concilio, c., 1431 Condon, E. U., 1207, 1209, 1253 Condon, J. B., 249, 250 Condorelli, G., 83, 1577, 1600 Conf. on Peaceful Uses of Atomic Energy,

194, 197,260 Conn, G. K. T., 340 Conner, W. V., 452, 576, 903 Connes, J., 212, 212 Connick, R. E., 500, 582, 584, 585, 586, 657,

704,784, 799,818,819,820,822,828, 834

Connor, J. A., 1554, 1593 Connor, W. V., 891 Conolly, T. F., 506 Constantini, J. M., 710 Contract number W-31-109-ENG-38, 1235 Conway, J. C., 1034 Conway, J. G., 213, 215,578,579,585,587,

748, 926, 976, 994, 995, 996, 998, 1033, 1034, 1050, 1058, 1058, 1075, 1076, 1198, 1226, 1227, 1228, 1229, 1231, 1251, 1260, 1264, 1293, 1362, 1382

Coogler, A. L., 501 Cook, G. B., 551 Cooper, J., 481 Cooper, J. H., 992 Cooper, L. N., 51 Cooper, S. R., 775, 779,816 Cooper, V. R., 513, 528, 529, 1518 Coops, M. S., 544, 546, 593, 594, 596, 895,

895,943, 1074, 1092, 1095, 1481, 1483 Cope, R. G., 650, 652, 656 Copeland, J. c., 1042, 1043, 1044, 1046, 1443 Coqblin, 8., 1001 Corbett, B. L., 990, 1028 Corbett, J. D., 75 Cordero-Montalvo, C. D., 1251, 1260 Cordfunke, E. H. P., 12,256,260,261,262,

263, 264, 265, 270, 272, 276, 296, 298, 1279, 1302, 1317, 1318, 1321, 1322, 1323, 1324, 1325, 1326, 1327, 1328, 1329, 1331, 1332, 1333, 1333, 1335, 1336, 1337, 1338, 1339, 1347

Corliss, C. H., 47, 48, 214,1199,1224 Cornish, J. B., 1318, 1329, 1330 Corsini, A., 84 Costanzo, D. A., 1531 Costa, P., 615, 677, 1317, 1329 Coste, A., 1231 Costes, R. M., 1458 Cotton, F. A., 1572, 1572, 1573 Couffin, F., 465, 470, 1335 Coulter, L. V., 1327 Coulter, V., 344

Author Index

Counsell, F. J., 1327 Counsell, J. F., 1327, 1328, 1329 Countryman, R., 1458 Cousseins, J. C., 67, 71, 85 Cousson, A., 67, 68, 71, 85, 463, 710, 756,

1446 Coutures, J.-P., 59, 60 Cowan, G. A., 505 Cowan, H. D., 827, 1538 Cowan, H. 0., 802, 818, 819, 820, 822, 827 Cowan, R. D., 212, 212, 213, 1217, 1226,

1242, 1244, 1252, 1258 Cox, D. E .• 1372 Cox, L. E., 251, 253, 254 Crabtree, G. W., 292, 295, 1410, 1411, 1411,

1412 Cracknei, A. P., 1372 Cramer, E. M., 599, 606, 607, 607, 623,

650,651,654,655,656,660,1397 Cramer, R. E., 1460, 1596, 1597, 1597, 1598 Crandall, H. W., 534,535, 536, 538, 541 Crandall, J. L., 889 Crandall, W., 344 Crane, W. W. T., 106,551 Cranshaw, T. E., 43 Cranston, J. A., 15, 103 Crasemann, B., 994, 1034 Cremers, T. L., 82 Criss, C. M., 1291, 1327 Cristallini, 0., 123 Croatto, U., 1430, 1452 Crocker, H. W., 701 Croft, W. L., 125 Crokett, T. W., 701 Crom, J., 574, 578, 733 Cromer, D. T., 642, 644, 647, 648, 649, 650,

651,652,654,655,656,657,670,674, 1035, 1258, 1430, 1433, 1434, 1440, 1444, 1445, 1446, 1448, 1450

Crookes, W., 124 Crosby, G. A., 319, 1269, 1271 Crossby, D., 701 Crosswhite, H., 215, 218, 577, 579, 996, 997,

998, 1034, 1050, 1217, 1218, 1222, 1227, 1236, 1237, 1240, 1242, 1245, 1247, 1251, 1259, 1260, 1362, 1380

Crosswhite, H. M., 215, 218, 577, 578,579, 580, 996, 1050, 1218, 1220, 1222, 1223, 1227, 1235, 1236, 1237, 1240, 1242, 1245, 1247, 1249, 1251, 1259, 1362

Crosswhite, H. N., 1034 Crouch, E. A. C., 551 Crouse, D. J., 195,206 Crouthamel, C. E., 109, 110, 111 Croxton, E. c., 284 Croxton, F. E., 170 Culbert, H. Y., 1408, 1408 Culler, F. L., 415, 521, 536, 537

Cullity, B., 287 Cuneo, D. R., 61 Cuninghame, J. C., 534, 535 Cunningham, B. B., 6, 119, 126, 127, 128,

461,472,472,500,511,512,582,585, 602,605,657,659,731,734,752,760, 812,814, 887, 897, 900, 903, 904, 909, 911,917,968,969,970,971,972,974, 981,990, 995, 1002, 1003, 1005, 1012, 1013, 1035, 1036, 1037, 1042, 1043, 1044, 1046, 1049, 1050, 1052, 1053, 1078, 1080, 1095, 1105, 1110, 1112, 1113, 1285, 1439, 1440, 1443, 1449, 1481, 1483, 1513, 1527, 1633

Cunningham, J. E., 288 Curie, M., 112 Curie, P., 103 Curtis, C. E., 621 Curtis, M. H., 662, 666 Curtis, M. L., 112, 117 Cuthbert, F. L., 43, 48 Cvjecanin, D., 551 Cymbaluk, T. H., 1569,1570, 1571, 1572,

1605, 1606 Czaynik, A., 294, 295, 296

Daane, A. H., 284 Dabeka, R. Y., 75 Dabretstov, Y. N., 1335 da Costa, N. L., 106 Dahlgren, S. D., 623 Dahlke, 0., 66 Dairiki, J. M., 990 D'Alessandro, G., 85, 482, 483 Dalley, N. K., 1430, 1452 Dallinger, R. F., 1577 Dallinger, R. P., 1332 Da1masso, J., 19 Dalton, J. T., 670, 673 Dam, J. R., 788, 790, 794, 794, 795, 796,

1488, 1493 Damien, A., 284 Damien, D., 62, 64, 64, 460,709, 710, 711,

712, 729, 902, 904, 907, 908, 970, 972, 975,976, 1043, 1048, 1432, 1435, 1436

Damien, D. A., 972, 975, 976, 1001, 1003, 1006, 1047, 1048

Damien, N., 460, 925 Damiens, A., 57 Dams, R., 109, 110, III Danan, J., 56, 1317 Danesi, P. R., 85, 482, 483 Danford, M. D., 911, 1456, 1457 Daniels, F., 1527 Daniels, W. R., 1644 Danilov, N. A., 1108, 1110, 1630 Danisi, P. R., 799,800,801 Danon, J., 27, 490

Author Index

Danpure, C. J., 1181 Danuschenkova, M. A., 813 Danze, D. F., 551 Darby, J. B., 12, 1417, 1435 Darby, J. B., Jr, 62, 64, 232, 280, 621,642,

887, 1148, 1149, 1151, 1366, 1390, 1394, 1399, 1409

Darby, J. S., 241 Darken, R. S., 632 Das, D. K., 56 Date, M., 66 Dauben, C. H., 56, 904, 909, 1443, 1447 David, D. F., 917 Davidenko, V. A., 1073 David, F., 29,30,32,912,915, 1000, 1013,

/013, 1014, 1038, 1040, 1045, 1046, 1052, /052, 1053, 1054, 1058, 1077, 1080, 1081, 1090, 1091, 1092, 1095, 1099, 1102, 1280, 1281, 1282, 1283, 1284, 1285, 1297, J3J5, 1320, 1334, 1343, 1344, 1345, 1346, 1397

Davidov, A. V., 1007 Davidsohn, J., 67, 71, 72, 73, 74, 75, 79, 80 Davidson, J. M., 72 Davidson, N., 311,452,455,460,462, 736,

749,752 Davidson, N. R., 675, 705, 707, 745, 749, 750,

751, 752, 753 Davies, D., 106, 109, 736, 737, 742, 746, 748 Davies, N. R., 1497 Davies, G. R., 1463 Davis, D., 731, 733, 734, 736 Davis, H. L., 1435, 1638 Davis, M. W., Jr, 534, 536 Davis, W., Jr, 316, 316 Davri1ov, K. A., 1107 Davydov, A. V., 102, 119, 121, 122, 124, 125,

139, 142, 149, 150, 91I, 932, 933, 976 Dawih1, W., 81 Dawson, H. M., 79 Dawson, J. K., 304, 614, 687, 733, 735, 736,

748, 761, 773 Day, C. S., 83, 1460, 1560, 1561, 1562, 1566,

1567, 1568, 1600, 1602, 1603, 1607 Day, R. A., 24 Day, R. A., Jr, 84, 349,351,352, 1503 Day, V. W., 83, 384, 385, 1456, 1460, 1461,

1560, 1561, 1562, 1566, 1567, 1568, 1568, 1569, 1570, 1571, 1571, 1599, 1599, 1600, 1602, 1603, 1605, 1606, 1607, 1608, 1609, 1610, 1610, 1611, 1614, 1614, 1620

Dayton, R. W., 683, 684 De, A. K., 485 Deal, R. A., 106, 109, 110, 124 Dean, D. J., 599, 610 Dean, G., 669, 695, 725, 727, 728, 1297, 1316,

1337 Dean, J. J., 608, 697 Dean, O. C., 234

Deane, A. M., 779, 780 Deardorff, E. A., 1514 Debbabi, M., 718, 720, 722,907,909 Debets, P. C., 268, 269 Debierne, A., 15 deBoer, F. R., 636, 637 deBoer, J. H., 51, 53 deBruin, T. L., 1251 Decker, W. R., 51 Declercq, J. P., 1564, 1565 Dec1erq, J. P., 1565 Dedov, V. B., 892, 934, 965, 976, 980 DeFranco, M., 695, 1297, 1316, 1337 Degetto, S., 1431, 1452 Degischer, G., 101 I Dejonghe, P., 25, 26, 27 DeKock, C. W., 748, 748, 749, 750, 750,751,

1312, 1338, 1574 DeKock, R. L., 1273 De1amoye, P., 1262, 1264 Delapalme, A., 1377 Deleuis, H., 212, 212 Deleon, A., 208 Delepine, M., 51, 52, 53, 61 Dell, D. M., 2893 Dell, R. M., 676, 678, 705,706,708,710,711,

712,1327, 1366, 1435 DellAmieo, G., 1455 Delliehausen, C., 289 Delong, L. E., 65 DeLong, L. E., 1412 Delphin, W. H., 450 Del Piero, G., 1458 Del Pra, A., 1460, 1561 Delsa, J. L., 1564 DeLuca, L. S., 690 Delvin, W. L., 487 Demers, P., 43 Demi, A. G., 1107 Demiehelis, R., 970, 978 Demildt, A. c., 16,25,26,27 Demin, A. G., 1107, 1108, 1110, 1630 deMiranda, c., 102, 121 deMiranda, C. F., 102, 106, 116, 142, 146,

146, 148, 149, 151, 152 Demmer, P., 337, 347 Dempf, D., 383, 1575 Dempster, A. J., 15, 104 Denig, R., 106 Denisov, A. F., 25 Dennard, F. S., 669 Denning, R. G., 344, 784, 802, 1273-, 1367 Dennis, L. M., 75, 76 Denotkina, R. G., 767, 805, 806 DePaoli, G., 132, 135, 1430, 1431, 1458, 1550,

1560, 1561, 1562 Depaus, R., 1329 DePlano, A., 1170

Author Index

deRango, C., 1456, 1458 Derevyanko, E. P., 1057 Detgunov, E. P., 67, 70, 72 Dervin, 1., 79 Desai, P. D., 1279, 1337 Desai, V. P., 1368, 1370, 1371 deSando, R. J., 763 Desclaux, J.-P., 1631 Desire, B., 912, 931, 978, 1054, 1055, 1057,

1483, 1484 Desmoulin, J. P., 1324 Desmoulin,1. R., 319 Desne, P., 250 Despres, J., 641, 646, 647, 648, 659 Desreux, J. F., 1564 Desyatnik, V. N., 71, 72 Detourmine, R. J., 282 DeTrey, P., 51 Deutsch, M., 390 Devalette, M., 59, 60 deViIlardi, G. C., 1458 Dewally, D., 1331 DeWitt, R., 452, 453 Deworm, 1. P., 27 Dey, A. K., 85 D'Eye, R. W. M., 59, 65, 67, 68, 74, 75, 85,

304 Dharwadkar, S. R., 1322 Dhers, J., 129, 130, 145 Diamond, R., 6,503,963, 1004, 1035, 1050,

1071, 1076, 1086, 1229 Diamond, R., 802 Diamond, R. M., 550, 552, 1088, 1527 Dianom, A. J., 308, 1368 Diatokova, R. A., 1053 Di Bemado, P., 1507, 1510, 1516, 1517 Dickel, G., 181 Diehl, R., 82 Diehl, R. G., 270, 276 Dieke, G. R., 217, 219, 221, 362, 1236, 1240,

1245, 1251, 1260 Dietrich, M., 53, 62 DiGrazio, R. P., 755, 759 Dijkwel, N., 212, 212, 213 Dillan, I. G., 541 Dillin, D. R., 1289 Diness, A. M., 60 Diringer, M., 212, 212, 213 Dirkmaat, A. J., 1409 Dittner, P. E., 1483 Dittner, P. F., 994, 1076, 1088, 1090, 1096,

1097, 1098, 1099, 1l01, 1101, 1l04, 1107, 1346

Dittrich, c., 340 Dixon, S. N., 106, 117, 121, 122 Dobretsov, V. N., 1338 Dobrowski, J., 719 Dock, C. R., 75

Dod, R. L., 126, 127, 128, 129 Dode, M., 261 Dodge, R. P., 1440, 1443 Dodgen, H. W., 577, 578, 579, 585, 1498,

1500 Doebler, R. E., 990 Doelter, C., 191 Dolidze, M. S., 992 Domanov, V. p" 1090, 1091, 1106, 1108 Donnan, M. Y., 485 Dontsov, Iu. P., 578 Dontsov, Yu. P., 1199 Dooley, G. J., 57 Doom, L. G., 599 Dorain, P., 1375 Doretti, L., 1561, 1562 Dori, Z., 1431, 1455 Dormand, A., 1551 Dormond, A., 1558, 1567, 1623 Domberger, E., 84, 379, 381, 911, 977, 1367,

1373, 1375, 1376, 1461, 1550, 1551, 1552, 1553

Domhofer, R., 1644 Dosch, R. G., 897 Doty, J. W., 70t Dougan, R., 1095 Dougan, R. J., 964 Dougherty, R. C., 119O Douglass, R., 756, 757 Douglass, R. M., 669, 758, 759, 763, 764, 767 Dover, D., 232 Downer, M. c., 1260 Drabkina, L. D., 812 Drabkina, L. E., 811, 812 Dresler, E. N., 981 Driscoll, W. J., 893, 931, 933 Drobot, D. V., 72 Drobyshevskii, Iu. V., 903, 910, 914 Drobyshevskii, Yu. V., 461 Droissart, A., 25, 26, 27 Drowart, J., 228, 1279, 1317, 1326, 1338,

1339,1347 Drozdova, V. M., 334 Druin, V. A., 106, llOO, 1l03, 1107 Drummond, J., 669, 673 Drummond, J. L., 685, 686, 687, 700 Dryssen, D., 1505 Dubeck, L. W., 51 Dubeck, M., 83 Duboin, A., 60, 64, 67, 75 Dubrovskaya, G. N., 65 Duffy, D., 516, 567 Dufour, c., 999, 1037, 1061 Dufour, J. P., 1644 Dufuor, S., 902 Duke, F. R., 399 Dukes, E. K., 448, 457, 485 DuMond, J. W. M., 580

Author Index

Dumont, G., 25, 26 Duncan, A. B. F., 217, 219, 221, 362 Duncan, L. R., 487 Dunlap, B. D., 217, 217, 453, 488, 489, 490,

491, 582, 899, 902, 903, 904, 907, 1382, 1406, 1407, 14()7, 1411, 1411, 1412

Dunning, R. G., 218 Dunsmore, H. S., 1491, 1492, 1495 Dunster, H. J., 662 Duplessis, J., 121,472,912, 1080 du-Preesz, G. H., 326, 327 duPreez, J. G. H., 1442, 1443 Dupuis, T., 76, 81, 82 Dupzyk, R. J., 1092 Durbin, P. W., 394,775, 779,816, 1181, 1186,

1187 Durham, R. W., 551 Durif, A., 82 Durin, V. A., 1107 Durrett, D. G., 219, 220 Diising, W., 61 DuTemple, 0., 548, 570 Duttera, M. R., 1566, 1567, 1602, 1616, 1618,

1619 Duval, c., 76, 81, 82, 1558 Duyckaerts, G., 25, 83, 457, 458, 783,972,

974, 1081, 1517, 1519, 1563, 1564, 1565, 1574

Dwyer, O. E., 544 D'yachkova, R. A., 120, 125, 142, 149, 1009,

1034 Dye, D. H., 292, 295 Dyrssen, D., 407, 817, 1512, 1520 Dzhelepov, B. S., 22, 887 Dzyubenko, V. I., 970, 979

Eakins, J. D., 24, 25 Easey, J. R., 69, 72, 74, 75, 461 Easey, J. F., 127, 135, 334, 1443, 1444, 1446,

1448 Easley, W., 967, 971, 973, 1260, 1379 Easley, W. C., 1378 Eastman, D. E., 55, 1395 Eastman, E. D., 59, 64, 65, 293 Eastman, M. P., 306, 1368 Ebbsjo, I., 51 Eberle, S. H., 911, 935, 938, 982,1055,1056,

1507, 1513, 1518 Eberle, S. M., 981 Edelstein, L. N., 1154 Edelstein, N., 83, 585, 587, 915, 967, 969, 970,

971, 973, 1005, 1038, 1040, 1045, 1049, 1050, 1052, 1054, 1058, 1077, 1081, 1090, 1091, 1095, 1099, 1102, 1260, 1262, 1267, 1269, 1280, 1281, 1282, 1297, 1315, 1320, 1322, 1334, 1335, 1337, 1341, 1342, 1343, 1345, 1346, 1362, 1369, 1369, 1370, 1371, 1374, 1376, 1377, 1378, 1379, 1382, 1432,

144(), 1447, 1462, 1573, 1577 Edelstein, N. M., 13,29, 32,461,463, 1397,

1458, 1575, 1580 Eder, J. M., 212, 212 Edgington, D. N., 270 Eding, H. J., 282 Edward, J., 462 Edwards, J., 462, 1337, 1440, 1441, 1443,

1560, 1561, 1562 Edwards, P. G., 83, 1606, 1611, 1612 Edwards, R. K., 259, 260, 671 Efimove, A. I., 335 Efremov, Yu. V., 896, 992 Efremova, A., 60 Egan, J. J., 544 Egorov, P. P., 599, 606 Ehemann, M., 56 Ehrlich, P., 1046 Ehrmann, W., 82 Eichberger, K., 219, 1264, 1269, 1362, 1369,

1370 Eichelberger, J. F., 25, 26 Eichler, B., 1644 Eick, H. A., 455, 643, 902, 1047, 1433 Eidelstein, N., 1038 Eigenbrot, C. W., 1458, 1459 Eigenbrot, C. W., Jr, 1566,1566 Eisenstein, J. C., 1264, 1267, 1367, 1369,

1370 Eister, W. K., 85 Eiswirth, R. M., 587,588 Elbouadili, A. A., 1596, 1604 EI-Dessouky, M. M., 120 Electromagnetic Isotope Separation Data

Sheets, 503 Elesin, A. A., 980, 981 Eliseev, A. A., 295, 297, 1454 Eliseeva, O. P., 125 Eller, P. G., 82, 306, 385, 386, 387, 702, 893,

898, 1458 Ellert, G. V., 295, 297, 1435 Ellinger, F. H., 251, 251, 456, 588, 598, 599,

604,606,607,607,621,623,632,640, 641, 642, 643, 644, 645, 646, 647, 648, 649,650,651,652,653,654,655,656, 656,657,657,658,659,660,661,662, 664,667,669,670,674,675,676,680, 681,681,683,690,694,699,700,700, 724, 725, 897, 900, 903, 905, 974, 1006, 1397, 1426, 1431, 1432, 1433

Ellinger, P. H., 1433 Elliot, R. 0., 1397 Elliot, R. P., 1397, 1397 Elliott, M. C., 570, 705 Elliott, N., 270 Elliott, R., 654, 656, 660 Elliott, R. M., 687 Elliott, R. 0., 602, 606, 607, 614, 623, 639

Author Index

Elliott, R. P., 233, 234, 236, 237, 238, 239, 240, 241, 283, 288, 290

Ellis, D. E., 489, 974 Ellis, J., 85 Ellis, P., 669 Ellis, Y. A., 106, 887 Ellison, R. D., 1445, 1452 E1minger, A., 112, 117 Elson, R., 112, 115 Elson, R. E., 69, 72, 102, 121, 126, 127, 128,

129, 130, 131, 142, 151, 1427, 1440 Elson, R. F., 1443 Elving, P. J., 485 Ely, N., 1459 Emel'yanov, N. M., 72 Emiliani, c., 111 Emmanuel-Zavizziano, Mme., 115 Engel, E., 82 Engel, N., 633 Engel, T. K., 599,609, 610, 612, 697,699,

700 Enge1hardt,1. J., 29, 1389 Engelhardt, W., 344 Engerer, H., 270, 276, 718, 720, 722, 723, 724,

907,909 Engle, P. M., 23, 27 Englekemeir, D. W., 1224 Engleman, R., 214, 1224, 1225, 1226 Engleman, R., Jr, 213, 1224, 1225, 1226 Engles, M., 51 English, A. c., 42 English, 1. 1., 700 Ensor, D. D., 915, 991, 992, 997, 998, 998,

1005, 1014, 1046, 1047, 1050, 1078, 1079, 1440

Epstein, L. F., 728 Erasmus, C. S., 1456 Erbacher, 0., 19 Erdmann, B., 128, 300,453, 624, 649, 651,

652, 904, 906, 907, 969, 972 Erdos, P., 12, 1377 Erin, E. A., 912, 913, 970, 971, 978, 979, 992,

1004, 1012, 1013, 1014, 1050, 1054, 1059 Erin, I. A., 1291 Ermakov, V. A., 920, 922, 923, 924, 925, 926,

1055, 1056, 1091 Ermakov, V. S., 470 Ermo1aev, N. P., 487, 1513 Ernst, B. B., 659 Ernst, R. D., 83, 1166, 1169, 1460, 1461,

1548, 1550, 1553, 1555, 1560, 1561, 1562, 1569, 1570, 1571,1571, 1572, 1588, 1590, 1593, 1608

Ernst, R. E., 1605, 1606 Esch, U., 284 Eshaya, A. M., 544 Eskola, K., 7, 1097, 1098, 1100, 1104, 1105,

1107, 1630

Eskola, P., 7, 1097, 1098, 1100, 1104, 1105, 1107, 1630

EsperAs, S., 78, 1452, 1490 Essen, L. N., 1507 Etard, A., 52, 56, 57, 64, 67, 71, 73, 74 Etourneau, J., 56 Etter, D. E., 317,644 Ettmayer, P., 56 Eubanks, I. D., 969 Eusebius, L. C. T., 85 Evans, H. T., 1450 Evans, H. T., Jr, 1504, 1513, 1517 Evans, J. E., 106, 1075, 1092 Evans, S. W., 728 Evans, W. H., 29, 1279, 1315, 1316, 1317,

1318, 1319, 1321, 1322, 1323, 1324, 1326, 1327, 1328, 1329, 1330, 1331, 1332, 1347

Evans, W. J., 1590 Evers, E. c., 306 Evteeva, L. 1., 350,351 Exner, F., 212, 212 Eyring, H., 480 Eyring, L., 452, 904, 909, 909, 911, 974, 1004,

1304, 1341

Faber, J., Jr, 1372 Fabian, D. J., 216, 216 Fabre, R., 606, 623 Facer, J. F., 687 Fachseminar zur Wiederaufbereitung, 186 Fagan, P. J., 83, 381, 1460, 1548, 1565, 1566,

1567, 1568, 1568, 1571, 1588, 1600, 1602, 1603,1607, 1614,1615, 1616, 1617, 1618, 1619, 1623

Fahey, J. A., 456, 460, 904, 907, 908, 909, 972,975,998, 999, 1000, 1001, 1003, 1004, 1004, 1006, 1007, 1041, 1042, 1043, 1044, 1045, 1048, 1303, 1305, 1432

Faiers, M. E., 1403 Fair, K., 1598, 1602, 1605 Fairchild, J. G., 1453 Faircloth, R. L., 456, 691, 697, 699, 1335 Fajans, K., 103, 106, 124 Fa1eschini, S., 1561, 1562 Fa1k, B. G., 1327, 1328 Fang, D., 727, 902 Fankuchen, 340, 354 Faragalia, G., 1561, 1562 Farah, K., 116, 122 Fardy, J. J., 992, 1012, 1503 Farina, F., 1459, 1593, 1593, 1596 Farkas, M. S., 718, 723, 724 Farnsworth, P. B., 54, 56 Farr, J. D., 25, 29, 1392 Farrar, L. G., 992 Farraro, I. R., 364, 930 Farrer, H. N., 1499, 1500

Author Index

Fauble, L. G., 29 Faucherre, J., 79 Fava, J., 59, 60 Feber, R. C., 1315, 1340, 1342, 1343, 1344,

1345,1346 Feder, H. M., 409, 409, 1330 Fedorov, V. L., 1332, 1333, 1334, 1445 Fedoseev, E. V., 976, 1007 Fefilov, B. V., 1107 Feinhauser, D., 1056 Feldman, C, 701 Felermonov, V. T., 1056 Fellows, J. A., 226 Fellows, R. L., 968, 979, 991, 995, 997, 998,

1003, 1005, 1006, 1014, 1042, 1046, 1047, 1050, 1051, 1078, 1079, 1260, 1341, 1441

Felsmaekers, J., 261 Felt, R. E., 662 Fender, B. E. F., 271 Fendrick, C. M., 83, 1571, 1602, 1609,1614,

1620, 1622, 1622 Feraday, M. A., 247 Ferguson, D. E., 186, 549,990, 1073 Ferguson, D. W., 186 Ferguson, R. L., 1644 Fermi, E., 3, 443 Femades, L., 80 Ferraro, 1. R., 72, 76, 77, 408 Ferri, D., 1490, 1504 Ferris, L. M., 287,311,529,891,1033,1053,

1323 Ferro, R., 63, 66 Fertig, W. A., 51, 65 Fidelis, J., 125 Field, E. I., 687 Fields, P., 1058, 1058 Fields, P. R., 6, 13, 211, 503, 505, 585, 902,

903,911,911,926,996, 1030, 1033, 1050, 1071, 1081, 1086, 1096, 1251, 1254, 1260

Fieuw, G., 27 Fiffins, P. E., 186 Figgins, P. E., 106, 112, 114, 115, 119, 145 Filimonov, V. T., 982 Fillmore, C L. F., 270, 271 Finch, C. B., 82, 688, 968, 971, 995, 1008,

1077, 1379, 1382 Finder, B. E. F., 268 Fine, M. A., 227 Fink, F. H., 1461 Fink, J. K., 1315, 1321 Fink, R. M., 661 Finke, R. G., 1567, 1569 Finkelnburg, W., 29 Finkle, R., 1183 Finnemore, D. K., 51 Fischer, B., 311 Fischer, C. F., 1242 Fischer, D. F., 1315, 1321

Fischer, E. 0., 83, 378, 379, 381,977, 1166, 1548, 1550, 1553, 1554, 1559

Fischer, H., 1553 Fischer, J., 315, 316 Fischer, R. D., 383, 911,1166,1374,1459,

1460, 1548, 1554, 1555, 1556, 1557, 1558, 1560, 1574, 1577, 1578, 1588, 1594, 1596, 1598

Fischer, W., 72, 74 Fisher, E. 0., 911 Fisher, E. S., 232, 1401, 1405 Fisher, J., 548, 570 Fisher, K. J., 212, 212, 213, 214 Fisher, R. W., 77 Fisk, Z., 1409, 1410, 1410, 1411, 1412, 1412 Fitzgibbon, G. C., 223 Flach, R., 51 Flagg, J. F., 506 F1ahaut, J., 294, 295, 296, 706 Flanary, J. R., 525, 529 F1egenheimer, 1., 123 Fleischer, M., 188, 191 Fleming, G. B., 516, 567 Fleming, J. E., 361, 414, 1452 Fleming, W. H., 504 Flerov, G. N., 1103, 1107, 1108, 1110,

1630 Fletcher, H. G., 74 Fletcher, J. M., 144, 149, 408, 408, 506, 570,

674,679 Fletcher, S., 902, 903, 1439 Flett, D. S., 1518 Florin, A. E., 461 Flotow, H. E., 53, 228, 251, 665, 683, 694,

695,697,699, 700, 705, 1279, 1294, 1316, 1322, 1323, 1326, 1330, 1331, 1332, 1333, 1335, 133~ 1338, 1341, 1347

Flynn, K. F., 963 Fochler, M.,·974, 976,1454 Foex, M., 59, 60 Folcher, F. G., 1594 Folcher, G., 1373, 1458, 1579, 1596, 1598 Foley, D. D., 191, 197, 201, 203, 204 Folger, H., 1630 Follmer, S. H., 1603 Folmer, M. M., 614 Fomin, V. V., 1430 Foos, J., 891 Foote, F., 227, 232 Forbes, R. L., 681, 683, 694 Forcrand, M., 364 Ford, J. L. C., 217 Ford, J. 0., 668, 672 Foreman, B. M., Jr, 24 Foreman, J. K., 1513 Forrest, J. H., 124 Forrester, J. D., 69, 74, 1441 Forsberg, H. C., 1331

Author Index

Forsellini, E., 1430, 1431, 1442, 1452, 1458, 1504, 1516

Forsling, W., 1096 Forte, M., 1377 Foster, K. W., 23, 29 Foster, L. S., 55 Foti, S., 120, 124 Fouche, K. F., 75 Fouque, Y., 1332 Fourest, B., 912, 1080 Fournier, J., 295, 297 Fournier, J. M., 29, 711, 969, 1001, 1281,

1377, 1378, 1379 Fowler, B. F., 501 Fowler, M., 1105 Fowler, M. M., 1644 Fowler, R. D., 126, 128, 588, 589,621, 623,

628,629,630,631,631,632,641,645, 649, 653, 1405

Fowler, R. H., 85 Fowler, W. A., 188 Fox, A. c., 727 Foxx, C. L., 593 Foyentin, M., 1262 Fradin, F. Y., 679 Fragahi, I., 83, 1560, 1577, 1600 Fragala, I. L., 1548, 1588 Frampton, o. D., 61 Franchini, R. C., 544, 546 Francis, E. L., 588, 598 Franck, J. C., 146, 148, 149 Frank, A., 75 Frankel, V. Ya., 919 Franz, W., 311, 1409 Fratiello, A., 85, 1490 Fraymond, K. N., 1575, 1575 Frazer, B., 1372 Frazer, M. J., 84 Fred, M., 27, 28, 125,213, 577, 578,579, 580,

897, 1198, 1200, 1224, 1226, 1227, 1229, 1236, 1237, 1264, 1269, 1272, 1272

Fred, M. S., 1088, 1237 Freed, S., 218 Freedman, M. S., 1088, 1090 Freeman, A. J., 12,49,232,280,489,621,

642, 887, 1001, 1148, 1149, 1366, 1392,1393,1394,1395,1409,1411

Freeman, G. E., 1179, 1187 Freiser, H., 1511, 1512, 1517,1519 Frenkel, V. Ya., 919, 928, 932, 970, 978, 1012,

1013, 1014 Freundich, W. S., 904 Freundlich, W., 60, 81, 82, 713, 714, 716, 719,

721, 723 Frezotti, A., 1321, 1328 Fricke, B., 1101, 1105, 1108, 1109, 1110, 1111,

1112, 1113, 1633, 1635, 1641 Friddle, R. J., 1401

Fridkin, A. M., 1010 Fried, 103, 134 Fried, S., 126, 127, 128, 129, 130, 131, 151,

152,902,903,911,974, 996, 998, 1003, 1006, 1033, 1034, 1042, 1043, 1046, 1050, 1053, 1058,1058, 1059, 1312, 1427,1441, 1443,1453

Fried, Sh., 311, 589,590, 598,643 Fried, S. M., 6, 30,31,452, 455, 456, 459,

460, 462, 465, 467, 472, 697, 700, 1047, 1050, 1071, 1086, 1337, 1338

Friedel, J., 614, 1389 Friedman, A. M., 505, 1096 Friedman, H. A., 300, 465, 468, 949, 995,

1009, 1052, 1080, 1481, 1531 Friedman, M. S., 216 Friedt, J. M., 488, 489, 490, 491 Frink, C., 1644 Frlec, M., 319 Frolov, A. A., 1538 Fromage, F., 79 Froman, D. K., 485 Fronaeus, S., 1514, 1530 Fronczek, F. R., 1460, 1461 Frondel, C., 43, 191,1453 Frondel, CI., 188 Frondel, J. W., 188, 191 Frydman, M., 1492 Fryell, R. E., 259 Fuchtenbusch, F., 291 Fuel Elements Conf., 247 Fuel Elements Fabrication, 247 Fuger, J., 72, 74, 83, 306, 312, 332, 335, 397,

457,463,469,903,904,909,917,972, 973,974,979,999, 1000, 1003, 1005, 1009, 1012, 1013, 1013, 1014, 1038, 1045, 1055, 1057, 1058, 1060, 1162, 1279, 1280, 1282, 1283, 1284, 1285, 1291, 1294, 1297, 1299, 1300, 1302, 1304, 1306, 1307, 1308, 1309, 1310, 1311, 1312, 1313, 1314, 1314, 1315, 1316, 1317, 1319, 1320,1320, 1321, 1322, 1323, 1324, 1325, 1327, 1331, 1332, 1333, 1334, 1335, 1336, 1336, 1337, 1338, 1340, 1341, 1342, 1343, 1347, 1379, 1446, 1447, 1448, 1499, 1513, 1563, 1574

Fuger, J. K., 915, 1011 Fuggle, J. c., 216, 216 Fuhrman, N., 53, 681, 683, 694 Fuhse, 0., 76 Fuji, K., 1368, 1371 Fujimo, T., 318 Fujino, T., 1302, 1303, 1331 Fujita, D., 1260 Fujita, D. D., 1047 Fujita, D. K., 969, 970, 995, 1000, 1007, 1035,

1038, 1049, 1050, 1078, 1080, 1380, 1380, 1381, 1382, 1440, 1443

Fukishima, E., 1260, 1558

Author Index

Fukusawa, T., 34 Fukushima, E., 904, 910,1441 Fulda, M. 0., 487 Fuller, J. E., 657 Fulmer, E. I., 1527 Fulton, R. B., 1532, 1533, 1534 Funk, R., 390 Furman, N. R., 410

Gabelman, J. W., 189 Gabeskiriya, V. Ya., 963 Gadd, K. F., 84 Gaeggeler, R., 1644 Giiggeler, R., 1644 Gal, 1., 581 Galateanu, I., 149, 150 Gal'chenko, G. L., 1279 Galin, M., 1484 Galkin, N. P., 197 Gallagher, C J., 106 Gallagher, E. X., 259, 263, 263, 264, 266, 267,

268 Gallatly, B. J., 1442, 1443 Galleani d'AgJiano, E., 1001 Galy, J., 1431 Gamp, E., 1262 Ganguly, J., 83 Ganguly, L., 381, 1563 Ganivet, M., 705 Gans, W., 66 Gantzel, P. K., 54, 56 Garber, D. I., 887 Garden, N. B., 662 Gardener, A. W., 410, 412 Gardner, E. R., 680, 683, 695, 696, 696, 698 Gardner, R. R., 612, 617, 623 Gardner, M., 227 Garner, C. S., 446, 503, 574, 575, 576, 578,

733,745 Garrett, A. B., 284 Garstone, J., 606, 613, 623, 641,643,654 Garvin, D., 1306, 1309, 1310, 1311 Gaskill, E. A., 208, 210 Gasparinetti, B., 80 Gasperin, M., 1446 Gatehouse, B. M., 364 Gates, J. E., 678, 679 Gatterer, A., 212, 212 Gatti, R. C., 6 Gaughan, G., 1567, 1569 Gaumer, L., 548, 570 Gaune-Escard, M., 1332 Gavin, B. F., 1644 Gavrilov, K. A., 1030, 1103, 1104, 1107, 1644 Gebala, A. E., 1169, 1459, 1548, 1596 Gebert, E., 459, 905, 909 Geichman, J. R., 319 Geipel, G., 78

Geiren, A., 1457 Geise, J., III Gelman, A. D., 13,457,458,464,469,484,

485, 703, 715, 911, 914, 929, 930, 935, 941, 1482, 1513

Genet, M., 151, 152,472, 1262, 1264 Genova, M., 247 Gens, R., 1331, 1334, 1336, 1340, 1341 Gentil, L. A., 82 Geranian, P., 1297, 1316, 1337 Gerbanovskaya, M. M., 361 Gerdanian, P., 261, 1321 Gerdanion, P., 728 Gerding, T. J., 461, 1336 Gerds, A. F., 284, 287, 289 Gergel, M. V., 116, 446, 450, 503, 505 Gergen, J. B., 540, 567 Gerke, R., 62, 63 Germain, G., 1565 Germain, M., 893 German, G., 1564, 1565 Gerratt, J., 72 Gerstenkom, S., 1224, 1227 Gewehr, R., 72, 74 Gey, W., 53 Gfaller, R., 390, 393 Ghiorso, A., 6, 7, 10, 43, 106, 962, 964, 990,

1025, 1071, 1086, 1092, 1093, 1096, 1097, 1098, 1099, 1100, 1101, 1102, 1104, 1105, 1106, 1107, 1108, 1127, 1285, 1481, 1527, 1630, 1644

Ghose, A. K., 85 Ghotra, J. S., 73 Giacchetti, A., 47, 1224, 1225 Giacometti, G., 1548 Giaechetti, A., 125 Giannoni, G., 351 Giannotti, C, 1594 Gibb, T. C., 488 Gibb, T. R. P., 1432 Gibinski, T., 294, 295, 296 Gibney, R., 668 Gibney, R. B., 308, 599, 610, 613, 613, 1336,

1339 Gibson, G., 76, 280, 361 Gibson, 1. K., 1003, 1007 Gibson, W. B., 516, 567 Gieren, A., 383, 384 Giese, R., 60, 80 Giesel, F., 15 Giessen, B. C., 623 Giessing, D., 16 Gilford, F. E., 270, 271 Gilbert, B., 83, 1081, 1563, 1564 Gilbert, B. P., 1564 Gilje, J. W., 1460, 1596, 1597, 1597, 1598 Gill, J. S., 362 Gilles, F. W., 697, 700

Author Index

Gilles, P. W., 59, 64, 65, 265, 293, 329, 398, 462

Gilman, H., 335, 387, 389, 394, 395, 1547, 1589

Gilman, W. S., 700, 701 Gindler, J. F., 12, 1224 Gingerich, K. A., 63, 66, 67, 283, 1328, 1329 Giorgi, A. L., 25, 29, 57 Girdhar, H. L., 1322 Girgis, C., 121 Gitlitz, M. H., 84 Gittus, J. H., 191, 197 Givon, H., 1030 Givon, M., 893, 912, 918, 919, 926, 930, 931,

932,943 Glacometti, G., 1460 Gladrow, E. M., 1527 Glamm, A., 227 Glaser, C., 75 Glaser, F. S .. 54, 56 Glaser, F. W., 1432 Glaser, J., 1490, 1504 Glasner, A., 679 Glass, R. A., 1527 Glassner, A., 223 Glavic, P., 71 Gleiser, M., 1279, 1337 Glendenin, L. E., 506, 507 Glotzel, D., 1395 Glover, K. M., 106 Glueckauf, E., 410, 411 Glushko, V. P., 1279 Gme/in Handbook, 14, 15,32,42,58,59, 170,

191, 197,213,214,214,215,216,217, 218, 221, 227, 233, 248, 256, 266, 272, 296,297,298,323,324,329,329,330, 333, 335, 344, 345, 353, 369, 373, 381, 387,388,391, 396, 398,414,455,461, 463,481, 500,511, 580, 588, 589, 598, 621, 624, 624, 626, 627, 657, 658, 664, 673,679,691,698, 708, 725, 725, 728, 732, 760, 764, 774, 779, 813, 887, 899, 910, Il28, Il31, Il34, Il54, 1162, 1289, 1290,1301,1306,1309,1310,1311

Goble, A. G., 104, Il4, Il7, Il9, 121 Gobusch, M., 1527 Goby, G., 980, 1055, 1080 Godbole, A. G., 488 Godlewski, T., 15 Goeller, H. E., 186 Goeppert Meyer, M., 1205 Goertz, R. C., 618, 661 Goffart, J., 83, 382, 974, 1294,1341,1343,

1379, 1563, 1564, 1565, 1574 Gofman, J. W., 42, 106 Gohring, 0., 103, 106, 124 Gojmerac, A., 121 Goldacker, H., 528, 533, 534

Goldberg, A., 1403 Golden, J., 104, Il4, Il7, Il9, 121 Goldenberg, J. A., 686 Gol'din, L. L., 16, 21 Golding, B., 1411 Goldman, S., 1010, 1058, 1293 Goldschmidt, B., 227 Goldschimdt, Z. B., 1236, 1241 Goldstein, J. H., 250 Gollnow, H., 125 Golovina, V. A., 79 Golovyna, V. A., 80 Gol'tsev, V. P., 1331 Golub, A. M., 75 Gomm, P. J., 24, 25 Gonzales, A. L., 576, 616,721,723 Good, P. T., 669 Goode, J. H., 125 Goodman, C. D., 1088, 1090, 1096, 1097,

1098, 1104, 1630 Goodman, G., 1373 Goodman, G. L., 1264, 1269, 1272 Goodman, L. S., 1076, 1088,1226,1229,

1264, 1272, 1272 Googin, J. M., 224 Gorbenko-Germanov, D. S., 902, 907, 913,

1450 Gorbunov, L. V., 72 Gordon, J. E., 308, 309, 1337 Gordon, S., 481, 9Il, 912, 926, 970, 979,

ll37, ll39, 1260, 1481 Goring, G., 548, 570 Gorskii, A. G., 926 Gorum, A. E., 676, 678, 679, 680, 708, 709,

710, 712, 713 Goryacheva, E. G., 25 Gourisse, D., 921 Gove, N. B., 16, 887 Gracheva, N. V., 295, 297, 300 Gradinger, H., 270, 276 Graeves, G., 268 Graham, J., 65 Graham, R. L., 994 Graham, Th., 175 Grainger, L., 226 Gramoteeva, N., 1554, 1577 Grandjean, D., 294, 295, 296 Grant, C. B., 1577 Graue, G., 104, Il2, lIS, 119 Graves, A. C., 485 Graw, D., 383 Gray, P. R., 22, Ill, 446 Graziani, R., 358, 358, 359, 1430, 1431, 1442,

1452, 1504, 1516 Grdenic, D., 1454 Grebenchikova, V. I., 515 Greek, B. F., 208 Green, D., 678

Author Index

Green, D. M., 1375 Green, D. W., 1315, 1321, 1322, 1337 Green, J. c., 83, 1565 Green, J. L., 576, 577, 667, 973, 1042, 1044,

1046, 1050, 1058 Greenberg, E., 1324, 1325 Greenwood, N. N., 488 Gregor'eva, S. I., 992 Gregorich, K. E., 1644 Gregory, J. G., 407 Gregory, N. W., 326, 327 Greiner, W., 1633 Greis, 0., 82 Grenall, A., 308 Grenthe, I., 980, 1490, 1504,1507, 1509 Gresky, A. T., 184, 184, 186, 506, 570 Greulich, N., 1644 Grieneisen, A., 538, 539 Grier, R. S., 1184 Griesse1, A., 1409 Grieveson, P., 282, 1318, 1329, 1330 Griffin, C. D., 1242, 1244, 1252 Griffin, N. 1., 232, 233 Griffin, P. M., 1227 Griffin, R. G., 1181 Griffioen, R. D., 1093 Griffith, C. B., 248 Griffith, J. W., 194 Griffith, W. L., 224 Griffo, J. S., 576, 577, 621 Grigorescu-Sabau, C. S., 936, 940, 942, 945,

946 Grimes, W. R., 300, 317, 320 Grimley, S. S., 1522 Grinberg, A. A., 350,351 Grisard, J. W., 313 Grison, E., 588, 589,614,621,623,628,629,

630,631,631,632,641,645,649,653 Grisson, E., 1405 Groh, R. J., 964 Grl2lDvo1d, F., 265, 1279, 1315, 1317, 1320,

1321, 1322, 1326, 1327, 1328, 1335, 1337, 1338, 1339, 1341, 1342, 1343, 1347

Groot, c., 542 Gross, A. V., 106 Gross, P., 1329 Grosse, A. V., 103, 104, 112, Il3, 114, 115,

119, 136, 1642 Grossman, R., 80 Grossman, N., 229, 229, 232 Groth, W. E., 182 Grove, G. R., 23, 25, 26, 613, 645, 646, 654,

656, 657, 686 Gruber, J. B., 1264, 1373, 1376 Gruen, D. M., 218, 219, 220, 456, 462, 483,

585,690,909, 1041, 1262, 1269, 1270, 1290, 1312, 1338

Grundy, B. R., 22, 111

Grunzweig, J., 251, 253 Gryntakis, E. M., 106 Gschneidner, K. A., Jr, 632, 633, 639, 640 Gubanov, V. A., 974 Gudaitis, M. N., 71 Guegnon, J. F., 1378 Guelachvili, G., 212, 212, 213, 1226 Guempel, 0., 362 Guertin, R. P., 51 Guggenberger, L. J., 69, 75, 1441 Guichard, c., 486, 1513 Guidotti, R. A., 75 Guillamont, R., 1482, 1489 Guillaumant, R., 1055 Guillaume, B., 484, 913, 917, 918, 926, 928,

1504, 1538 Guillaumont, R., 29, 32,69,74, 102, 116, 121,

122, 129, 132, 133, 134, 142, 143, 144, 145, 146, 146, 147, 147, 148, 148, 149, 150,151,152,153,153,472,710,891, 912,931,935,942,978,980, 1000, 1010, lOll, 1013, 1013, 1014, 1038, 1040, 1045, 1052, 1054, 1054, 1055, 1057, 1058, 1080, 1081, 1090, 1091, 1095, 1099, 1102, 1264, 1280, 1281, 1282, 1297, 1315, 1320, 1334, 1343, 1345, 1346, 1397, 1483, 1484, 1486, 1487, 1488, 1489, 1490

Guillot, P., 122, 146 Guinet, P., 250 Giildner, R., 1338, 1341 Gulino, A., 1577 Gulyas, E., 86 Gumperz, A., 71, 80 Gund1ich, C., 74 Gunn, S. R., 917, 918 Gunten, R. R. von, 1630 Gunze1, F. R., Jr, 270 Gupta, S. K., 1328, 1329 Gureev, E. S., 892, 893, 934 Gurrich, L. W., 1279 Gurry, R. W., 632 Gurvich, L. V., 1279, 1293, 1300, 1316, 1317,

1323, 1324, 1325, 1338, 1346 Gusev, N. I., 12,485 Guseva, L. I., 12, 887, 892, 965, 992, 993,

1031, 1080 Gustison, R. A., 548, 570 Guthrie, A., 177 Gutina, E. A., 1335 Gutmacher, R. D., 996, 997 Gutmacher, R. G., 213, 895, 895, 943, 976,

994, 995, 996, 1033, 1034, 1058, 1058, 1074, 1075, 1076, 1198, 1227, 1228, 1229

Guy, W. G., 124 Guymont, M., 76 Guyon, F., 214 Gvozdev, B. A., 1095

Author Index

Gvudz, E., 1030 Gwozdz, R., 125

Haas, P. A., 686 Haas, W.O., 541 Haas, W.O., Jr, 185, 186 Haber, L., 81 Hadari, Z., 55, 581, 1335 Haeffner, E., 538 Haemmerle, W. H., 1411 Hafey, F., 122 Hagan, L., 1033, 1094, 1098, 1103, 1292, 1293 Hagan, P. G., 465, 467 Hagee, G. R., 106 Hagemann, F., 184, 1453 Hagemann, F. T., 15, 23, 25, 26, 30, 31, 43 Hagen, C. E., 540, 567 Hagenberg, W., 383 Hagenbruch, R., 911 Hagenmuller, P., 59,60,82 Hagg, A. C., 182 Hagiwara, K., 1574, 1577 Hagstrom, I., 122 Hagstrom, S., 49 Hahn, D. K., 212, 212, 213, 214 Hahn, 0., 4, 15, 19, 103, 106, 110, 112, 115,

124, 170,443 Hahn, R. L., 106, 484, 1095, 1098, 1101, 1101,

1104, 1107, 1538, 1630, 1644 Haines, C. F., 1596 Haines, H. R., 645, 646, 668, 671, 673, 674,

1339 Hains, C. F., 1459 Haire, J. R., 999 Haire, R. G., 67, 68, 460, 686, 703, 704, 791,

792, 900, 904, 907, 908, 969, 972, 973, 974, 975, 976, 991, 997, 998, 998, 999, 1000, 1001, 1002, 1003, 1004, 1005, 1006, 1007, 1007, 1008, 1()()8, 1009, 1009, 1013, 1013, 1014, 1035, 1036, 1036, 1037, 1038, 1039, 1040, 1041, 1042, 1043, 1044, 1045, 1046, 1047, 1048, 1050, 1051, 1052, 1052, 1053, 1057, 1058, 1059, 1059, 1060, 1060, 1061, 1075, 1076, 1078, 1079, 1148, 1153, 1260, 1265, 1279, 1280, 1281, 1290, 1291, 1294, 1340, 1341, 1342, 1343, 1344, 1379, 1380, 1381, 1382, 1389, 1390, 1393, 1401, 1406, 1435, 1436, 1440, 1441

Haissinsky, M., 30, 102, 119, 124, 142, 145, 151, 152, 1482

Hakonson, T. E., 1170 Hale, W., 895 Hale, W. H., 896 Hale, W. H., Jr, 974 Hale, W. M., 968 Hall, D. A., 1430, 1452 Hall, G. R., 582, 907, 926, 928 Hall, H. T., 54, 56

Hall, L., 463 Hall, N. F., 77 Hall, R. O. A, 308, 309, 452, 613, 614, 615,

616, 668, 671, 677, 1337, 1339, 1340 Hall, T. L., 69, 74, 1440, 1441 Halla, F., 80 Halstead, G. W., 306, 1458, 1460, 1461, 1463 Hamaker, J. W., 60, 61 Hambley, T. W., 1455 Hamblyn, AN., 364 Hamer, AN., 22, III Hamill, D., 1589 Hamilton, F. D., 349, 1503 Hamilton, J. H., 106 Hamilton, W. C., 255, 256, 258, 1432 Hampel, C. A., 613 Hancock, C., 54, 56 Handler, P., 1371 Handley, T. H., 106, 110 Handwerk, J. H., 60, 270, 679 Hanford Technical Information Operations,

500,691 Hansen, M., 233, 234, 236, 237, 238, 239, 240,

241,288,290 Hansen, N. J. S., 106, 109 Hanson, W. C., 1170 Hansson, E., 1454 Haque, M.-U., 1452 Hara, M., 913, 934 Harada, Y., 60 Harari, A., 60 Harbour, R. M., 12,447,451,467,473,485,

486,487,896,992,1076 Harbur, D. R., 619, 621 Hardt, P., 83 Hardy, A., 60, 82 Hardy, C. J., 144, 149 Hardy-Grena, C., 335 Harmatz, B., 181, 186 Harmon, C. A., 1574, 1575, 1577 Harmon, H. D., 979,1011, lOBO, 1499 Harmon, K. M., 567, 569, 570, 573, 574, 589,

591,598,643,687 Harper, P. E., 1430, 1450 Harrington, C. D., 197,209, 224, 226, 232,

305,310 Harris, B. S., 668, 672 Harris, H. B., 71 Harris, J., 7, 1104, 1105, 1107, 1630 Harris, L. A, 82 Harris, W. E., 339 Harris, W. R., 394, 1187 Harrison, G. R., 211, 212, 212, 213, 214 Harrison, J. D. L., 690, 717, 718, 720, 722,725 Harschke, J. M., 665, 697, 699, 705 Harshman, E. N., 189 Hart, F. A., 73, 1452 Hart, R. G., 551

Author Index

Hartl, K., 365, 1453 Harvey, B. G., 7, 10, 106, 124, 304, 582, 658,

1030, 1088, 109\, 1092, 1094, 1105, 1527, 1528, 1530, 1633

Harvey, B. H., 1030 Harvey, J. A., 43 Harvey, M. R., 653 Harvey, P. G., 701 Hasbrouck, M. E., 598, 612, 613, 617, 621,

623 Haschek, E., 212, 212 Haschke, J. M., 620, 681, 694, 909, 1047,

1279, 1294, 1316, 1323, 1335, 1337, 1341, 1347, 1423

Hasegawa, Y., 34 Hass, W. 1. de, 51 Hasselberg, B., 212, 212 Hasty, R. A., 61 Hatch, L. P., 548, 570 Hatcher, J. B., 1335 Hattori, H., 61 Haubach, W. J., 114 Haug, H., 270, 273, 276, 723, 724, 976 Haug, H. 0., 380, 965, 974, 1003, 1004 Haug, H. W., 1042, 1045, 1046 Hauge, R. H., 1589 Haung, K., 1034 Hauser, 0., 80 Hauske, H., 30, 31, 32, 903, 973 Hausman, E., 112, 115 Hiiussermann, W., 192 Hawes, L. L., 599, 606, 607, 607 Hawkins, D. T., 1279, 1337 Hawkinson, D. E., 120 Hay, P. J., 1623 Hayek, E., 75 Hayes, R. G., 1374, 1577 Hayes, W. N., 1042, 1046, 1047, 1050, 1260,

1441 Hayman, C., 1329 Hayward, B. R., 224 Hazen, W. C., 593 He, M.-Y., 1616 He, P., 25 Head, E. L., 680, 683, 690, 697, 699, 700, 700,

1328 Heady, O. E., 548, 570 Heal, H. G., 339, 658, 701 Healy, T. V., 407, 527, 1057, 1522 Hearth, R. E., 304 Heath, R. L., 20 Heatley, F., 83, 1561, 1562, 1569 Hecht, A. c., 82 Hecht, F., 81, 326 Hecht, H. G., 1271, 1368, 1373 Hecker, S. S., 1403, 1405 Hedger, H. J., 1328, 1329 Hegarty, J., 1257

Hegedus, L. S., 1547 Heiberger, 1. J., 455 Heidt, R., 340 Heier, K. W., 187 Heiks, J. R., 368 Heimann, P., 1395 Heimbach, P., 83 Hein, R. E., 511 Heindl, F., 65 Heinrich, E. W., 191, 194 Heinzelmann, A., 308 Heiple, C. R., 677 He-Jian, Yu., 534 Hejl, V., 189 Helgeson, H. c., 1291 Hellman, N. N., 590, 591 Hellwege, H. E., 998, 1007 Helminski, E. L., 889 Hempelmann, L. H., 1184 Henderson, D. J., 894, 897, 992, 1030, 1091 Hendrich, H., 1368, 1370, 1371 Hendricks, M. E., 125, 1008, 1364, 1365,

1367, 1367, 1373, 1375, 1376, 1377, 1378, 1380

Hendrix, G. S., 667, 669, 670, 1433 Henkie, Z., 66, 292,295, 1410 Hennelly, E. J., 890 Henrickson, A. V., 516, 567, 570, 593 Henry, K. H., 529, 534 Hensley, D. c., 1088, 1090, 1096, 1097, 1098,

1101,1101,1104,1107,1630 Hentz, F. c., 1540 Hentz, F. c., Jr, 1485, 1487 Herak, M. J., 121 Herasymenko, P., 339 Herbst, J. F., 1001 Hermann, G., 121, 142, 146 Hermann, J. A., 567, 570, 891 Herment, M., 19, 25 Hemiman, P. D., 582, 926 Herpin, P., 79 Herrero, J. A., 1431 Herrick, C. C., 82, 604, 606, 1315, 1340, 1342,

1343, 1344, 1345, 1346 Herrman, G., 1105 Herrmann, G., 19, 106, 1633, 1644 Herrmann, G. H., 10 Herrmann, H., 292 Herrmann, J. A., 516 Hertz, M. R., 112, 114, 115 Hesford, E., 1521, 1522 Hessberger, F. P., 7, 1110, 1112, 1630, 1644 Hessler, J. P., 585, 976, 996, 1034, 1050, 1059,

1257, 1362 Heumann, F. K., 1503 Heydemann, A., 22, III Hickman, R. C., 195 Hickmann, U., 1644

Author Index

Hicks, H. G., 120 Hicks, T., 534, 536 Hicks, T. E., 534, 541 Hien, H. G., 289 Hietanen, S., 85, 338, 347, 1484, 1485, 1487,

1488, 1488, 1492 Higa, K. T., 1597, 1598 Higgens, G. H., 1086 Higgins, C. E., 911, 1456 Higgins, G. H., 6, 551 Higgins, I. R., 533, 553 Higgins, L. R., 304 Higgins, S. G., 1071 Hilary, J. J., 104, 114, 117, 120 Hildebrand, D. L., 1323, 1324, 1325, 1338,

1346 Hildebrand, J. H., 632 Hildebrand, N., 1644 Hildebrandt, R. A., 410, 412 Hildenbrand, D. L., 48, 60, 1279, 1293, 1300,

1316, 131~ 1323, 1324 Hill, D. G., 359 Hill, F. D., S44 Hill, H. H., 29, 57, 126, 128, 915, 969, 1000,

1040, 1045, 1281, 1341, 1345, 1346, 1390, 1394

Hill, J., 1441 Hill, J. D., 599, 606, 610 Hill, M. W., 106, 120, 120 Hill, N. A., 54, 56, 197 Hill, O. F., 513 Hill, R. F., 270, 271 Hill, R. J., 1456 Hillary, J. J., 104 Himes, R. C., 295, 297 Hinatsu, Y., 1373, 1375 Hinchey, J. C., 465, 472 Hincks' E. P., 43 Hincks, J. A., 686 Hinderburger, E. J., Jr, 484 Hindman, J. C., 151, 152,396,461,465,469,

470,471,471,472,472,475,476,477, 479, 481, 482, 483, 484, 500, 502, 502, 582, 657, 784, 788, 790, 795, 798, 802, 807,818,921, 1264, 1272, 1272, 1487, 1488, 1489, 1503, 1536, 1537, 1538

Hingmann, R., 7,1630 Hinton, Sir C., 536 Hirose, Y., 1569 Hirsch, A., 6, 1071, 1086 Hitterman, R. L., 76, 1452 Hoard, J. L., 1445, 1456 Hobart, D. E., 912, 913, 917, 917, 918, 926,

928,930,971,998, 1007, 1052, 1059, 1059, 1060, 1095, 1290, 1291, 1340

Ho, C. K., 125 Ho, C. Y., 1077 Hoch, M., 1321

Hochied, D., 641, 646, 647, 648, 659 Hocks, L., 83, 1563 Hodge, H. C., 661 Hodge, N., 282, 412, 673 Hodges, A. E., 620, 1337 Hodgson, K. 0., 83,382,383, 1459, 1462,

1463, 1555, 1573, 1574, 1575, 1575, 1579 Hoekstra, H. R., 259, 263, 263, 264, 265, 266,

267,268,269,459,905,909,1004,1331, 1332, 1333

Hoenig, C. L., 270 Hoeskstra, H. R., 1035 Hoff, H. A., 676 Hoff, R. W., 10,551,963, 1087, 1088, 1092,

1105, 1633 Hoffert, F., 892 Hoffman, C. G., 61, 63 Hoffman, D. C., 106,505,551, 1105, 1125,

1127, 1170, 1644 Hoffman, G., 355, 365, 366, 367, 373 Hoffman, J. G., 668, 672 Hoffman, J. I., 399 Hoffman, P., 460 Hoffman, R., 1589 Hoffmann, A., 60 Hofmann, D. C., 10 Hoffmann, G., 687, 690, 703, 727, 1453 Hofmann, P., 1603 Hoffmann, R., 344, 1603 Hofmann, S., 7, 1110, 1112, 1630, 1644 Hofmann, U., 365, 1453 Hoge, H. J., 1323 Hohlein, G., 551 Holah, D. G., 84, 902, 903, 1439, 1446, 1455 Holcomb, H. P., 970, 978 Holden, A. N., 227, 232 Holden, N. E., 106, 161, 171 Holden, R. B., 53, 227 Hollander, J. M., 106, 887, 963, 994 Holleck, H., 673 Holley, C. E., 1279, 1317, 1318, 1320, 1328,

1329, 1336, 1339, 1347 Holley, C. E., Jr, 223, 697, 700, 1006, 1317,

1318, 1321, 1328, 1329, 1335, 1336, 1339 Holley, C. S., Jr, 680, 683, 690, 699, 700, 700 Hollock, H., 667 Holm, L. W., 1096 Holmberg, R. W., 1484, 1485, 1488 Holmes, H. F., 1291 Holmes, J. A., 227 Holtkamp, H., 79 Holtz, M. D., 994 Honan, G. J., 1490 Honigschmid, 0., 52, 56, 65, 325, 326 Hoover, J. I., 181 Hopkins, H. H., 542 Hopkins, H. H., Jr, 106, 574, 575, 576, 747 Hopkins, S. W. J., 1328

Author Index

Hoppe, R., 60 Hoppe, W., 383, 384, 1457 Horen, D. J., 19 Horn, F. L., 549 Horton, R. W., 548, 570 Horwitz, E. P., 450, 451, 893, 894, 896, 897,

992, 1091, 1094, 1528, 1529 Hoshi, M., 79, 907 Hough, H., 714 Howell, G. R., 520 Howells, G. R., 536, 1517 Howerton, R. J., 887, 1035 Howitz, E. P., 1030 Howland, J. J., Jr, 582 Howlett, B., 283 Hoyle, F., 188 Hristidu, Y., 378, 1548, 1553 Hseu, C. S., 1550, 1573 Hsian-Yun, W., 1452 Huang, C. Y., 1340 Huang, K., 994 Huang, K. N., 1034 Hubbard, R. P., 1226 Hubbard, W. N., 72, 74, 306, 312, 332,677,

700, 1279, 1300, 1304, 1306, 1307, 1308, 1309, 1310, 1311, 1312, 1313, 1314, 1316, 1317, 1319, 1320, 1323, 1324, 1325, 1327, 1330, 1332, 1333, 1334, 1335, 1336, 1337, 1338, 1339, 1340, 1341, 1342, 1347

Hubbell, J. H., 1035 Hiibener, S., 1076, 1281, 1632 Huber, E. J., Jr, 680, 683, 690, 697, 699, 700,

700, 1317, 1321, 1328, 1335 Huber, J. G., 51 Huber-Buser, E., 1456 Hubert, S., 931, 935, 942, 980,1011,1054,

1055, 1057, 1080, 1091, 1262, 1264, 1483 Hubin, R., 81, 82 Hucleux, M., 486 HUdgens, C. R., 317, 644 Hudson, E. D., 177 Huebener, S., 1090, 1091 Huffman, A. A., 317 Hiifner, S., 1236, 1245 Hughes, D. G., 650, 652, 656 Hughes, T. G., 520,536, 1517 Huizenga, J. R., 6, 470, 474, 475, 1071, 1086 Hulet, E. K., 7, 895, 895, 943, 963, 964, 976,

995,996,997, 1030, 1033, 1034, 1042, 1046, 1047, 1050, 1075, 1075, 1080, 1087, 1088, 1092, 1094, 1095, 1105, 1106, 1108, 1227, 1228, 1260, 1345, 1441, 1481, 1483, 1630,1644

Hulet, E. M., 1074 Hulet, K., 1644 Hull, G., 224 Hulliger, F., 63, 66, 292, 293, 294 Hultgren, A., 538

Hultgren, A. Y., 538 Hultgren, R., 1279, 1337 Humbach, W., 29 Hume-Rothery, W., 633, 634, 635 Humphreys, C. J., 212, 212, 213 Hund, F., 270, 276 Hiiniger, M., 61 Hunt, E. B., 56 Hunt, J. E., 1190 Hunt, L. D., 1098, 1101, 1101, 1104, 1107,

1630 Hunt, P. D., 1321 Huntoon, R. D., 964 Huntzicker, J. J., 1321 Huray, P. G., 489, 973, 974, 1000, 1008, 1008,

1009, /009, 1013, 1013, 1038, 1379, 1380, 138/, 1382, 1406

Hursh, 1. B., 661 Hurst, F. J., 195 Hurst, H. J., 1430 Hurtgen, C., 335, 463, 904, 909, 1310 Hush, N. J., 480 Hussonnois, H., 1091, 1485 Hussonnois, M., 978, 980, 1010, 1011, 1054,

1055, 1057, 1080, 1091, 1107, 1108, 1262, 1264, 1483

Hussonois, M., 912, 931, 935, 942, 1106 Hutchison, C. A., 1272 Hutchison, C. A., Jr, 183, 1368, 1369, 1371,

1372, 1375 Huys, D., 25, 26 Hybert, S., 1010 Hyde, E. K., 10,21,42,43,77, 106, 121, 124,

500, 503, 511, 554, 887, 1026, 1028, 1105, 1123, 1127, 1633

Hyde, K. R., 674, 679 Hyder, L., 1481 Hyder, M. L., 1012, 1013, 1053 Hyman, H. H., 208, 211, 319, 506, 548, 570 Hynes, M. J., 1504

IAEA, 197,208,260,262,506,662, 1279, 1280, 1297, 1321, 1337

Iandelli, A., 293 Iddings, G. M., 106 Ihara, N., 1511 Ihde, A. J., 15 Ihle, H., 325, 327 Ikawa, M., 106 Iliff, J. E., 53, 61, 67 Ilijnov, A. S., 1630 Ilin, E. G., 74 Hlige, J. D., 964 Immirzi, A., 1430, 1431, 1458 Imoto, S., 1368, 1371, 1373, 1375 Imre, L., 77 Inoue, Y., 120 Insley, H., 320

Author Index

International Centre for Diffraction Data, 1041

International Nuclear Fuel Cycle Evaluation (INFC),173

Ionova, G. V., 979, 1002, 1034, 1054, 1081 Irish, E. R., 528, 529, 533 Isaacson, R. E., 447, 449 Ishida, V., 125 Ishii, T., 267 Ishikawa, N., 318 Ishimori, T., 1031, 1057 IUPAC, 990 Ivanov, A. A., 599, 606 Ivanov, M. I., 700 Ivanov, M. P., 1108, 1117, 1630 Ivanov, R. B., 22 Ivanova, L. A., 119, 1007 Ivanova, L. J., 122 Ivanova, O. M., 74, 78, 1454 Iwasaki, M., 318 Izumi, S., 1315, 1321

Jackson, E. F., 723, 724 Jackson, G., 1442 Jackson, H. K., 521 Jackson, N., 104, 114, 120,551 Jacob, C. W., 229 Jacob, E., 309,314 Jacobi, E., 124 Jacobs, J. M., 506, 562 Jacobson, A. J., 271 Jacobson, R. A., 69, 75, 1441 Jacoby, R., 78 Jacoby, W. R., 270, 276 Jaffe, I., 1279 Jaffey, A. H., 963 Jakes, D., 1331 Jamerson, J. D., 1559, 1560 James, A. C., 1186 James, D. B., 553, 554 James, R. A., 6, 887, 962 James, W. J., 50 Jander, G., 326, 412 Jangida, B. L., 85 Jannasch, P., 75 Jansen, G., Jr, 687 Jarry, R. L., 316,316 Jarvin, J. A., 1592 Jarvis, J. A. T., 1463 Jasaitis, Z. V., 589, 598, 643 Jassonneix, B. du, 56 Javed, N. A., 1321, 1329 Javorsky, C. A., 63, 66 Jayadevan, N. C., 669, 670, 714, 715, 717,

718,1434 Jefferes, J. M., 623 Jeffries, C. D., 125

Jekel, E. C., 1291, 1327 Jelenic, I., 1454 Jelley, J. V., 43 Jellinek, F., 295, 297, 299 Jenkins, H. D. B., 1005,1331,1335,1336 Jenkins, I. L., 117, 121,123,894 Jenkins, J. L., 687 Jenkins, T. L., 407 Jenkins, W. J., 620 Jennings, I. L., 410, 412 Jensen, R. J., 173 Jeppson, D. W., 529, 534, 553 Jere, G. V., 60, 61 Jeske, G., 1616 Jette, E. R., 588, 598, 602, 606, 614 Jha, M. C., 69, 72, 74, 1440, 1441 Jin, J., 77 Jin, Z., 77 Jochem, 0., 285 Johanson, L. I., 1037 Johanson, W. R., 292, 295, 1410 Johansson, B., 51,999, 1000, 1034, 1035,

1040, 1090, 1395 Johansson, G., 77, 85, 1452, 1485, 1489 John, W., 580 Johns, I. B., 574, 575, 578, 733 Johns, J. B., 662, 666 Johnson, D. A., 1292 Johnson, E. B., 502, 502 Johnson, G. K., 677,700, 1306, 1313,1317,

1323, 1337, 1339 Johnson, G. L., 61, 339 Johnson, I., 644, 1330, 1331 Johnson, J. S., 347, 1485, 1487, 1492, 1493,

1494,1540 Johnson, K. A., 641, 643, 647, 649, 651, 653,

65~670, 674,675, 681, 694, 900,1433 Johnson, K. R., 81 Johnson, K. W. R., 516, 567, 570, 574, 575,

575, 578, 593, 595, 705, 747, 750 Johnson, L. J., 1489 Johnson, 0., 77, 298, 327 Johnson, Q., 69, 72, 1389, 1390, 1440, 1443 Johnson, Q. C., 654 Johnson, S. A., 1231 Johnson, T. I., 455 Johnson, W. C., 1527 Johnston, C. P., 667 Johnston, D., 219, 223, 1262 Johnston, D. A., 1362 Johnston, D. C., 65 Johnston, D. R., 1262 Johnstone, J. K., 897 Jolibois, 340 Jonassen, H. E., 662 Jones, A. D., 887, 930, 943, 947, 981, 1056,

1499, 1502, 1503, 1513, 1514 Jones, E. R., 1374, 1375, 1462

Author Index

Jones, E. R., Jr, 125, 489, 1008, 1364, 1365, 1367, 1367, 1375, 1376, 1377, 1378, 1380, 1573

Jones, E. W., 1187 Jones, L. H., 344, 345, 484, 902, 903, 913,

914, 928, 976, 978 Jones, L. V., 25, 26,317,368,612,613,686,

688,728 Jones, M. E., 903 Jones, M. M., 572 Jones, P. J., 117, 119, 121, 122, 127,135, 136,

138, 139, 145, 326, 327, 1446 Jones, R. G., 335, 387, 389, 394, 395 Jones, R. S., 188, 191 Jones, W. M., 616 Jonke, A. A., 548, 559, 570 Jordan, J., 396 Jordan, K. c., 16, 599, 610 Jordan, R. A., 174 Jordon, R. F., 1623 Jergensen, C. K., 218, 917, 928, 1239, 1264,

1267, 1273 Jorgensen, J. D., 53, 54 Jorgensen, J. L., 389 Joshi, J. K., 1483 Jouniaux, B., 1046, 1077, 1313 Jove, 1., 460, 463, 907, 908, 917 Judd, B. R., 125, 585,971, 1209, 1210, 1227,

1236, 1240, 1245, 1254, 1363, 1371 Judson, B. F., 447, 449, 541, 542, 589, 598,

-643 Jullien, R., 1001 Junkes, J., 212, 212 Junkison, A. R., 293, 705, 706, 708, 709, 710,

711, 712, 1327 Jurriaanse, A., 992 Juui, J., 551 Juza, R., 62, 63, 335

Kackenmaster, H. P., 177,325,326 Kading, H., 104, 112, 115, 119 Kaffnell, N., 106 Kahn, M., 32 Kahn, S., 120 Kahn-Harari, A., 60 Kakihana, H., 1492 Kakovlev, G. N., 982 Kalibabchuk, V. A., 75 Kalina, D. G., 84, 1367, 1551, 1552, 1593,

1594 Kalvius, G. M., 217, 217, 453, 488, 489, 490,

491, 582, 899 Kamaratseva, N. 1.,264 Kamenskaiai, A. N., 1053 Kamenskaya, A. M., 1095 Kamenskaya, A. N., 125, 1053, 1081, 1091,

1095, 1344, 1345, 1481 Kamm, R., 599

Kandil, A. T., 121 Kanellakopoulos, B., 379, 380, 381 Kanellakopuios, B., 84, 910, 911, 969, 974, 975,

976,977, 1166, 1366, 1367, 1373, 1374, 1375, 1376, 1377, 1459, 1460, 1461, 1462, 1550, 1554, 1555, 1556, 1556, 1558, 1559, 1577

Kanellukopuios, B., 1368, 1370,1371 Kang, S. H., 1306 Kannellakopulos, B., 1551, 1552, 1553 Kanno, M., 1315, 1321, 1327 Kant, A., 511 Kaplan, G. E., 52, 67 Kaplan, L., 52,410,412 Kappel, M. J., 394, 1179, 1187 Kappelmann, F. A., 893, 1521 Kapshukov, I. I., 78, 456, 902, 913, 915, 974,

1004, 1291, 1431, 1452 Karabasch, A. G., 52 Karaker, D. G., 911 Karalova, Z. K., 25, 122,992, 1031, 1057 Karkhanavala, M. D., 1322 Karmas, G., 335, 387, 389, 394, 395 Karpacheva, S. M., 892, 934 Karraker, D., 1049, 1050 Karraker, D. G., 84, 125, 489, 912, 913, 1008,

1269, 1269, 1364, 1365, 1367, 1367, 1374, 1375, 1376, 1376, 1377, 1378, 1379, 1380, 1382, 1456, 1462, 1463, 1550, 1552, 1559, 1560, 1563, 1573, 1574, 1575, 1577, 1579

Karstens, H., 52 Kartasheva, N. A., 77, 932 Karuppannasamy, S., 61 Kascheyev, N. F., 116 Kaseta, F. W., 1251 Kasha, M., 582, 584, 585, 586, 784 Kaspar, J., 189 Kasper, J., 84 Kasper, J. S., 56 Kasten, P. R., 317, 325 Kasumakumari, M., 979, 980 Kasuya, T., 66 Katahira, D. A., 1608, 1617 Katayama, Y. B., 705 Kately, J. A., 1330 Katharia, D. A., 1617 Katz, J. J., 10, 12, 15, 102, 170,208,211,223,

248,249,280,282, 298,301, 303,303, 310, 361, 394,395,456,465,483,499, 506,547,548,570,643,644,645,648, 652,653,658, 690, 904, 909, 962, 971, 1030,1041, 1056, 1091, 1094, 1098, 1101, 1102, 1105, 1135, 1190, 1278, 1324, 1483, 1484, 1633

Katz, S., 452 Katzin, L. 1.,42,43, 52, 76, 77, 78, 86, 102,

106, 112, 115, 124, 170, 171, 184,364, 408,410,412,658

Author Index

Kauffman, 0., 81 Kaufman, A., 244 Kaufman, A. R., 287 Kaufman, V., 215, 1224, 1225, 1267 Kaufmann, G., 334 Kawamura, K., 73 Kawasuji, I., 34 Kay, A., 599, 609, 610 Kay, A. E., 588, 589, 599, 610, 612, 613, 621,

623,641,642,643,658,669 Kayser, H., 212 K.azachevsky, I. V., 503 Kazakova, G. M., 992, 1012 Kazanskii, K. S., 907 Keally, T. J., 1164 Keder, W. E., 1526 Keeler, W. A., 225 Keenan, T. H., 904, 911, 917, 918, 920, 926 Keenan, T. K., 67, 68, 71, 892, 895, 902, 903,

904, 913, 914, 967, 972, 973, 976, 978, 995,996, 1004, 1005, 1430, 1444, 1445, 1482, 1530, 1536

Kehman, L. R., 247 Keideriing, T. A., 255, 255, 256, 257, 258,

1362, 1432 Keirn, W., 83 Kelchner, B. L., 516, 567, 659 Keller, C., 12, 15, 30, 33, 60, 69, 71, 102,

120, 128, 131, 131, 194,257,263,270, 274, 276, 277, 398, 447, 449, 453, 455, 455,457,458,459,463, 500, 598, 624, 649,651,652,658,713,714,715, 716,717,718,719, 720, 721, 722,727, 887,902,903,904,905, 906, 90~908, 909,910,911,913,915,917,918,930, 934, 935, 938, 939, 942, 943, 944, 962, 963,969,972,976,981,982, 1031, 1055, 1056, 1056, 1057, 1148, 1366, 1368, 1370, 1371, 1376, 1446, 1453, 1520

Keller, D. L., 674, 678, 679, 691, 697, 699, 700,701

Keller, E. L., 311 Keller, J., 7, 1630 Keller, O. L., 976, 978, 1097, 1098, 1445,

1641 Keller, O. L., Jr, 10, 120,995, 1081, 1098,

1099, 1104, 1l05, IllO, 1111, 11l2, 1125, 1127, 1283, 1337, 1483, 1630, 1633, 1635, 1636,1637

Keller, R. A., 214, 1226 Keller, W. H., 53, 61, 67 Kelley, K. K., 265, 1279, 1321, 1337 Kelley, R. E., 1389 Kelley, R. G., 900 Kelley, W. E., 224, 225 Kelly, D. P., 500, 686 Kelly, M. J., 61 Kelman, L. R., 618, 620, 661

Kelmy, M., 79 Kemmerich, M., 621, 623, 642 Kemp, T. J., 1454 Kempter, C. P., 54, 58 Kenelly, W. J., 1560, 1561, 1562 Kenna, B. T., 897 Kennan, T. K., 1440, 1441 Kennedy, D. J., 995, 1035 Kennedy, J., 1522 Kennedy, J. W., 4, 6, 499, 643, 644, 645, 648,

652,653 Kennelly, W., 1460 Kennelly, W. F., 1569, 1571 Kennelly, W. J., 83, 1461, 1608 Kent, R. A., 610, 611, 668, 672, 677,

1338 Kepert, D. L., 1455 Kerko, P. F., 1331 Kern, D. M. H., 399 Kerrigan, W. J., 963 Kerr, P. F., 191 Kertes, A. S., 85, 1506, 1517, 1518, 1519,

1521, 1523 Kes, P. H., 1409 Kesel, G. P., 542 Keski-Rahkonen, 0., 215 Kester, F., 54, 56 Ketels, J., 1054, 1056 Kettle, S. F. A., 1446 Keys, J. D., 106 Khan, A. S., 65 Kharitonov, Y. P., 1107 Kharitonov, Yu. Ya., 79 Khazrouni, S., 17 KhIebinikov, V. P., 142, 149 Khodadad, P., 295, 296 Khopkar, P. K., 892, 931, 932, 933, 979, 980,

992, 1056, 1499, 1503 Kidd, P. W., 215 Kieffer, R., 56 Kierkegaard, P., 1452 Kiess, C. C., 212, 212, 213 Kilbourn, B. T .• 1463, 1592 Kilimov, S. I., 1095 Kim, J. I., 106 Kim, K. Y., 1306 Kim, Y. C., 1306 Kimura, K., 106 Kimura, M., 1439 Kinard, W. F., 1011 King, E., 614, 616 King, E. L., 81 King, H. W., 659 King, L. J., 542, 891, 893, 965, 990, 1028,

1031, 1032, 1087, 1088 Kinser, H. B., 894, 1030 Kinsley, S. A., 1574, 1577, 1578, 1579 Kinsman, P. R., 1321, 1337

Author Index

Kirby, H. W., 15, 16, 19,22,23,26,27,29, 32, 34, 102, 106, lll, 112, 115, 117, 119, 120, 121, 124, 144, 145

Kirchner, J. A., 224 Kirin,1 S., 383, 384, 911, 1457 Kiriyama, T., 85 Kirk, P. L., 589, 598, 643 Kirkbride, L. D., 619, 621 Kirslis, S. H., 311 Kiselev, Yu. M., 1292 Kisiluk, P., 1264 Kislitsina, G. 1, 503 Kiss, Z., 1260, 1261 Kistemaker, J., 182 Kittel, J. H., 247, 1405 Kitts, F. G., 529 Kiyoura, R., 260, 263 Kjanno, H. E., 1405 KJihne, E., 1460, 1555, 1556, 1557, 1558,

1594, 1598 Klaproth, M. H., 169 Klein, J. L., 247 Klein-Haneveld, A. J., 295, 297, 299 Kleinschmidt, P., 1077 Kleinschmidt, P. D., 969, 999, 1000, 1037,

1040, 1060, 1076, 1279, 1280, 1281, 1340, 1341, 1342, 1343, 1344

Klenze, R., 379, 1373, 1375, 1376, 1555 Klepfer, H. H., 229, 232 Kleppa, O. J., 1316 Kleykamp, H., 460, 667 Klimov, V. C., 1450 Kline, K. R., 1488, 1489 Kline, R. J., 1482, 1534 Klinkenberg, P. F. A., 48, 578, 579, 1224,

1251 Kloepper, H. C., 226 Klopman, G., 1498 Kluge, E., 120 Klutz, R. Z., 1576 Klyuchnikov, V. M., 77 Kmetko, E. A., 900, 1152, 1152, 1389, 1390 Kmeto, E. A., 1389, 1390, 1392 Knacke, 0., 66, 71, 72, 74, 223 Knapp, J. A., 55 Knauer, J. D., 992, 993, 1012, 1031 Knight, F. W., 604, 606 Knight, G. C., 474 Knighton, J. D., 544, 546, 593, 594, 596, 649,

890, 899, 1033 Knott, H. W., 676 Knox, F. A., 177, 180 Knudsen, F. P., 270, 271 Ko, R., 485 Koch, C. W., 60, 61 Koch, G., 528, 533, 534, 1521 Koch, L., 459, 485, 713,717,905,909 Kochetkova, N. E., 982

Kock, L., 716 Koczy, F. F., 111 Kodenskaya, V. S., 1504 Koehler, W. C., 456, 1006, 1041 Koehly, G., 538, 892, 913, 917, 918, 926, 928 Koelling, D. D., 49, 1001, 1392, 1393, 1395,

1411, 1411, 1412 Kohl, E., 194 Kohler, E., 83, 1463, 1592 Kohlschiitter, V., 51, 61, 65 Koike, Y., 24, 34 Koiro, O. E., 919, 928 Kojic-Prodic, D., 81 Kolarich, R. T., 142, 145, 146 Kolarik, Z., 1523 Kolb, A., 76, 77, 78, 80 Kolb, J. R., 1169, 1558, 1578 Kolbe, W., 1260, 1376, 1382 Kolesnikov, N. N., 1110, 1630 Kolesov, 1 V., 1104, 1107 Kolesov, V. P., 1279 Kolin, V. V., 463, 967, 971 Kolitsch, W., 1440 Kolkenbeck, K., 311 Kolodney, M., 595 Kolokol'tsov, V. D., 931 Kolthoff, I. M., 339 Kolyadin, A. D., 383,384, 1457 Komarov, E. V., 1498, 1501 Komarov, Y. V., 484 Komkov, Ya. A., 1482 Komkov, Yu. A., 469 Komura, K., III Konev, V. N., 621, 641, 642, 643, 645, 647,

648,649,651,652,653,654,656 Konig, E., 1368, 1370, 1371 Konishi, K., III Konkina, L. F., 930, 934, 935, 937, 939, 940,

941,942 Konobeevsky, S. T., 588, 598, 599, 606, 614,

616. 621, 623, 641, 642, 643, 644, 645, 646,648,649,650,651,653,654,655, 656,660

Konovalova, N. A., 1091, 1095, 1345, 1481 Kooi, J., 410, 992, 1053 Kopf, J., 1460, 1556, 1557 Koppel. 1, 79 Koppel, M. J., 1187 Kopytin, L. M., 647, 653 Kopytov, V. V., 912, 913, 970, 971, 978, 979,

992, 1004, 1012, 1013, 1014, 1050, 1054, 1059, 1291

Korbitz, F. W., 57 Korkisch, J., 993 Korostyleva, L. A., 578, 1199 Korotin, Y. S., 1107, 1108 Korotkin, Y. S., 1106, 1108 Korotkin, Yu. S., 26, 912, 978, 1644

Author Index

Korpusov, G. V., 992 Korsakova, M. D., 1435 Korshunov, B. G., 72 Korst, W. L., 53, 54 Kortright, F. L., 75, 76 Koster, G. F., 1211 Kosyakov, V. N., 893, 903, 907, 911, 912,

913, 919, 920, 924, 927, 928, 971, 978, 992, 1010, 1012, 1013, 1014, 1050, 1054, 1059, 1074, 1291

Kotlar, A., 261 Kotlin, V. P., 463, 926, 967, 971 Koval, V. T., 75 Kova1enko, G. S., 487 Kova1eva, T. V., 364 Kova1skaya, M. P., 361, 540, 541 Koval'skaya, N. P., 364 Kovba, L. M., 60, 264, 267, 268 Koz'min, Yu. A., 1481 Kramer, G. F., 901 Krasny-Ergen, W., 304 Krastinat, V., 390 Krastinat, W., 390 Kratz, J. V., 1644 Kraus, H., 140, 141 Kraus, K. A., 25, 112, 120, 338, 339, 347, 399,

582, 1482, 1484, 1485, 1487, 1488, 1488, 1489, 1492, 1493, 1493, 1494, 1495, 1496, 1526, 1527, 1530

Kraus, L., 17 Krause, K. A., 1488 Krause, M. 0., 215 Kravchenko, E. A., 74 Krein, F. P., Jr, 26 Kremers, H. E., 30 Kressin, I. K., 68, 70,551 Krestov, G. A., 994, 1013, 1013, 1279 Krikorian, ~ H., 54, 56, 58, 1317, 1433 Kritchevsky, E. S., 396 Krivokhat-skii, A. S., 1033 Kroner, M., 83 Krot, N. N., 457, 458, 464, 469, 470, 484, 485,

487, 715, 911, 912, 914, 918, 929, 930, 935,936, 970, 971, 978, 979, 1482, 1513

Kruger, O. L., 295, 296, 297, 667, 668, 669, 676, 677, 678, 679, 680, 697, 699, 700, 705,706, 707, 708, 709, 710, 711, 712, 713, 1337, 1338, 1339

Krugiov, A. A., 641, 653 Krumpe1t, M., 455 Krupa, J. c., 1262, 1264 Krupka, M. C., 54, 57 Kruse, F. H., 135, 136, 137, 152,319,902,

903,904, 972, 973, 1440, 1441, 1444, 1445, 1482

Kriiss, G., 64, 65, 71, 72, 79, 80 Kruyt, H. R., 76 Kry1ov, V., 484

Kry1ov, V. N., 1498, 1501 Kubaschewski, 0., 223, 227, 306, 1279, 1318,

1319, 1321, 1323, 1324, 1325, 1328, 1329, 1330, 1331, 1339, 1340

Kubo, K., 57 Kubo, V., 1490 Kuchumova, A. N., 81 Kudo, H., 121 Kugel, R., 1264, 1272, 1272 Kiihl, H., 80 Ku1akov, V. M., 106 Kulkarni, D. K., 140, 141 Kulkarni, V. H., 84 KUllberg, L., 1501, 1503, 1514, 1514, 1515 Ku1yako, Yu. M., 932, 1012, 1013, 1014 Kumar, N., 75 Kumok, V. N., 34, 81 Kunin, R., 308 Kunze, K. R., 1589 Kuptsov, V. M., 503 Kurbatov, N. N., 71, 72 Kuroda, P. K., 505 Kuroda, R., 85 Kurodo, R., 125 Kurtchatov, B. V., 515 Kusch, W., 649 Kusumakumari, M., 932 Kutaitsev, V. 1.,621, 623, 641, 642, 643, 644,

645,64~ 648, 649, 650, 651, 652,653, 654, 655, 656, 660

Kuzhina, I. I., 263, 264 Kuz'micheva, E. U., 264, 267 Kuz'mina, E. A., 503 Kuzmina, M. A., 116 Kuznetsov, V. I., 1103 Kuznetsov, V. S., 992 Kuznetsova, L. K., 982 Kuznietz, M., 251, 253 Kuzovkina, E. V., 992 Kyi, R.-T., 125

La Gamma de Bastioni, A. M., 124 Labedev, I. A., 120 Labereau, P. G., 1048 LaBonville, P., 930 Labozin, V. P., 1228 LaChapelle, T. T., 6, 456, 465, 470, 471, 474 Lachenmeir, P., 306 Lachere, G., 215 Lacombe, P., 232, 233 Lad, R. A., 394, 395 Ladd, M. F. C., 1454 LaDuda1, R., 1333, 1340, 1343 Lafferty, J. M., 54, 56 Lagowski, J. J., 1293 Laidler, J. B., 456, 703, 903, 1430, 1446, 1447,

1452 Laing, M., 1442

Author Index

Laitinen, H. A., 1481 Lajunen, L. H., 1492 Lallement, R., 606, 607, 614, 615, 677,

1377 Lam, D. J., 62, 64, 216, 453, 460,580,676,

679,680,709,710,711,902,903,904, 907, 1004, 1035, 1151, 1366, 1377, 1378, 1390, 1394, 1395, 1396, 1399, 1407, 1417, 1433,1435

Lam, D. W., 232 LaMar, G. N., 1575 LaMar, L. E., 691, 895, 1530, 1536 Lambert, D., 1231 Lambertson, W. A., 270 Liimmermann, H., 585, 587 Land, C. c., 632, 640, 641, 642, 643, 646, 647,

648,649,651,652,653,654,655,656, 657, 65~ 659, 667, 670, 674, 675, 1433

Lander, G. H., 490, 676, 1372, 1378, 1395, 1396, 1403, 1406, 1409

Landgraf, G. W., 1556 Landrum, J. H., 963, 964, 1092, 1094, 1095,

1105, 1106, 1481, 1644 Landrum, L. H., 1095 Lane, J. A., 362 Lane, L. J., 1170 Lang, J. M., 270, 271 Lang, R. G., 1224 Lang, R. J., 29, 48, 212. 212 Lange, R. c., 106 Langer, S., 54, 56 Langhorst, A. L., Jr, 570, 705 Langsworth, L. G., 344 Lanz, R., 679 Lapage, R., 669, 677 Lapitskii, A. V., 149, 150 LaPlace, S. J., 255, 256, 258, 1432 Laquer, H. L., 612 Larkworthy, L. F., 336, 337, 347 Larsen, A., 538 Larsen, S. D., 1558 Larsh, A. E., 7, 1099 Larson, A. c., 71, 602, 606, 607, 632, 642,

644, 64~649, 651, 652,654, 656, 657, 670, 674, 1440, 1445

Larson, D. T., 681, 694, 909, 1294, 1423 Larson, E. A., 249, 250 Larson, R., 349, 351,352,353 Larson, R. G., 106, ll2, ll5 Larsson, R., 1514 Larsson, S. E., 1643 Lasarev, Y. A., 1104 Lataillade, F., 645 Latimer, R. M., 7,992, lOll, 1055, 1058,

1058, 1080, 1099 Latimer, W. M., 76, 344, 702, 1279, 1285,

1288, 1327 Latrous, H., 1080

Latta, R. E., 259 Lau, K. F., 55 Lau, K. H., 1323, 1324 Laubereau, P., 9ll, ll66, 1553, 1554, 1559,

1561 Laubereau, P. G., 83, 381,382, 9ll, 971, 977,

998, 1003, 1007, 1043, 1048, 1050, 1459, 1459, 1460, 1461, 1563, 1564

Laubscher, A. E., 75 Laud, K. R., 80, 81 Laugier, J., 282 Laiigt, F., 81 Lauke, H., 1591, 1616, 1620 Laun, D., 213 Laun, D. D., 212, 212 Launay, S., 1446 Laurelle, P., 60 Laurens, W., 106 Laviron, E., 1551, 1567 Lavut, E. G., 268 Lawaldt, D., 902, 903, 906 Lawrence, F. D., 1170 Lawrence, F. 0., 505 Lawrence, J. J., 123, 124 Lawroski, S., 513, 521, 544, 547, 746, 1517 Laws, R. B., 542 Lazarevic, M., 208 Lazarev, Y. A., 1107 Lazkhina, G. S., 116 Lea, K. R., 1364, 1368 Leader, W. M., 226 Leah, A. S., 304 Leang, C. F., 106 Leary, J. A., 570,570, 571, 574, 575,575, 576,

577, 578, 589, 595, 596, 597, 598, 598, 616, 641, 643, 645, 654, 655, 656, 667, 668, 668, 669, 672, 673, 674, 677, 687, 705, 721, 723, 728, 747, 750, 891, 1338, 1339,1340

Leask, J. M., 1364, 1368 Lebeau, P., 57, 284 Lebedev, I. A., 12,887,892, 9ll, 912, 913,

915,918,919, 926, 928, 932, 933, 934, 940, 965, 970, 978, 979, 980, 993, 1012, 1013, 1014, 1031, 1077, 1081, 1283,1431, 1452

Lebedev, I. G., 621, 641, 642, 643, 645, 647, 648, 649, 651, 652, 653, 654, 656

Lebedev, V. M., 980 Leber, A., 52 Leber, R. E., ll05 LeBerquier, F., 580 Leciewicz, L., 295, 296 LeCloarec, M. F., 140, 141, 146, 148, 149 Lecoin, M., 23 Lecoq-Robert, A., 261 Lederer, C. M., 16, 106, 172, 500, 554, 887,

963, 1028, 1071

Author Index

Lee, D., 993, 1644 Lee, J. A., 126, 308, 309, 452, 453, 588, 598,

606, 613, 614, 615, 616, 623, 641, 643, 654, 668, 671, 677, 1337, 1339, 1340

Lee, R., 1490 Lee, R. E., 85 Lee, T., 1458, 1461, 1555 Lee, T. S., 234, 238 Lee, T. Y., 380, 1430, 1457 Lee, Y., 1461 LeFlem, G., 59, 60, 82 Lefort, M., 10, 1105, 1633 Leger, J. M., 909, 1044 Legoux, Y., 30, 1005, 1046, 1077, 1313 Legre, J., 1231 Leibowitz, L., 1321 Leibowitz, M. G., 1315, 1321 Leicester, H. M., 15 Leid, R. C., 669 Leigh, R. M., 338, 349 Leikina, E. V., 465, 469 Leino, M., 1644 Leino, M. E., 7, 1630 Leipoldt, 1. G., 84, 1456 Leitmeier, H., 191 Leitnaker, J. M., 677 Leitner, L., 270, 276, 723, 724 Lejeune, R., 25 LeMarouille, J. Y., 334, 1443 Lemire, R. J., 338, 338, 344, 346, 350, 350,

1291 Lemmertz, P., 1644 Lemons, J. F., 1488, 1489 Lenner, M., 1455, 1456 Leong, 1., 1459 Leonov, M. R., 1554, 1577 Leontovich, A. M., 587, 697 Lerner, J., 505 Lesinsky, J., 74 Lesuer, D. R., 900, 1389 Leung, A. F., 1269,1269, 1271, 1273, 1371 Leuze, R. E., 183, 887, 965, 1091, 1518 Levakov, B. I., 990 LeVanda, c., 83, 1463, 1575, 1580 Levenson, M., 521, 548, 570 LeVert, F. E., 889 Levet, J. C., 334, 335, 1443 Levey, C. G., 1251 Levi, G. R., 1453 Levine, C. A., 446, 503, 504, 512 Levine, S., 1279 Levinson, M., 1517 Levitsky, B. M., 599, 606 Levy, H. A., 1445, 1452 Levy, J. H., 1439, 1441, 1443, 1448 Levy, W., 73 Lewis, R. S., 505 Lewis, W. B., 1258, 1271, 1368

Li, S.-c., 71, 72 Liang, W.-B., 1608 Libedev, I. G., 641, 653 Liberman, D. A., 1258 Liberman, S., 1231 Libowitz, G. G., 248, 249, 250, 252, 253, 255,

1432 Lidster, P., 1369, 1369 Lied, R. C., 270 Lieke, W., 1409 Lieser, K. H., 120 Liimatainen, R., 548, 570 Liljenzin, G., 122 Liljenzin, J., 1290 Liljenzin, J. 0., 142, 149, 151, 398, 407, 1489,

1511 Lilley, E. M., 900 Lilly, P. E., 1077 Lim, C. K., 344 Lima, F. W., 121 Lin, Z., 1567 Linck, I., 17 Lincoln, S. F., 1490 Lindau, I., 1037 Lindemann, F., 181 Lindemer, T. B., 1297, 1337 Lindenbaum, A., 1186 Lindgren, I., 1001 Lindner, R., 13, 588, 589, 621, 623, 641,643,

644, 646, 647, 649, 652, 659, 1154 Lindquist, 0., 1456 Lindsay, J. D. G., 126, 128 Linford, P. F. T., 608, 612, 613, 697 Lingjaerde, R. 0., 551 Lipis, L. V., 1430 Lipkind, H., 55, 61, 66, 67, 71, 73, 77 Lipp, A., 56 Lippard, S. J., 255, 256, 257, 258, 1432, 1445 Liptai, R. G., 1401 Litteral, E., 264 Littler, D. J., 504 Litvina, M. N., 911, 912, 919 Litz, L. M., 284 Litzen, U., 1224 Liu, J. Z., 1571 Liu, M., 77 Liu, X., 77 Liu, Y.-F., 992, 993, 994 Livingston, R. S., 181 Llewellyn, P. M., 1375 Ll'inov, A. S., 1108, 1110 Lloyd, M. H., 574, 578, 686, 703, 704, 791,

792, 887, 904, 976, 1518 Loadier, F. D., 667 Loasby, R. G., 599, 609, 610, 614, 650, 652,

656 Lobanov, Y. V., 1103, 1104, 1107 Lobikov, E. A., 1199, 1228

Author Index

Loeb, D. B., 599, 606 Lofgren, N. A., 265, 293, 329 Lofgren, N. L., 59, 64, 65, 398, 462, 697, 700 Lohr, H. R., 228, 251,306,903,909, 9Il,

1316, 1323 Lo-Long-Jun, 534 Lombard, L., 288 Lombardi, c., 247 Lonadier, F. D., 576, 577, 621 Long, J. L., 544, 546 Long, J. T., 506, 529 Long, K. A., 615, 1321, 1328 Long, W., 216, 216 Longheed, R. W., 1042, 1046, 1047, 1050 Lonsdale, H. K., 1328 Loopstra, B. 0., 267, 270, 272 Lord, W. B. H., 588, 589, 598, 614, 621, 623,

628,629,630, 631, 631, 632, 641, 645, 649, 653, 661

Lord, W. P. H., 1405 Loree, T. R., 615 Lorenz, R., 1320 Lorenzelli, R., 459, 669, 673, 677, 1333, 1340,

1343 Loriers, J., 65, 909, 1044 Los, J., 182 Lou, c., 992, 993, 994 Lougheed, R., 995, 996 Lougheed, R. W., 7,963,964,996,997, 1034,

1075, 1076, 1092, 1094, 1095, 1105, 1106, 1108, 1229, 1260, 1441, 1481, 1483, 1630, 1644

Louis, R. A., 74 Louwrier, K. P., 686, 904 Love, J., 903 Love, L. 0., 503 Loveland, W., 1629 Lowe, J. T., 895, 896 Lowenstein, E., 361 Lowe, W. W., 540, 567 Lowrie, R. S., 359 Loye, 0., 60 Lu, C. C., 994 Lu, T. H., 1430, 1457 Luc, P., 1224, 1226 Lucas, J., 337 Lucas, R. L., 620 Luce, M., 1327 Luckyanov, A. S., 648, 650, 651, 652 Lueze, R. E., 893 Lugli, G., 378, 1169, 1459, 1460, 1463, 1548,

1548, 1549, 1549, 1572, 1593, 1593, 1596 Lukasiak, A., 1643 Luke, H., 1047 Luke, W. D., 1463, 1576, 1578 Luk'yanenko, N. G., 77 Lundgren, G., 80, 81, 1452, 1489, 1493 Lundquist, R. F. D., 1092, 1094, 1095

Lundqvist, I., 1530 Lundqvist, R., 931, 1487 Lundqvist, R. D., 1080 Lundqvist, R. F., 152, 153 Lundqvist, R. F. D., 1481 Lungu, G., 361 Lux, F., 136, 138, 140, 141, 219, 325, 327,

383,911, 1264, 1269, 1362, 1369, 1370, 1457

Lyalyushkin, N. V., 974 Lychev, A. A., 1457 Lyle, S. J., 124,979, 980, 981, 1498,

1507 Lynch, R. W., 897 Lynch, V. J., 195 Lynton, H., 361,414, 1452 Lyon, W. G., 1332 Lyon, W. L., 589, 598, 623, 643, 690, 728,

728, 729, 891 Lyon, W. S., 106, 110

Maatta, E. A., 83, 381, 1548, 1565, 1567, 1571, 1598, 1602, 1603, 1614, 1616

Maayer, P. de, 82 McBeth, R. L., 77, 218, 219, 220, 462, 1262,

1269, 1270 McBride, J. P., 686 McCart, B., 1378 McClure, D. S., 1260, 1261 McCoy, J. D., 106 McCreary, W. J., 589, 598, 643 McCue, M. c., 76, 1283, 1293, 1315,

1317 McCurdy, H. c., 181 McDonald, B. J., 643, 669, 673 McDonald, G. J. F., 188 McDonald, R. A., 60, 61, 284, 289 McDonald, R. 0., 202 McDonald, W. S., 1458 Mcdougal, J. R., 700 McDowell, J. D., 898, 899, 1292, 1293 McDowell, J. F., 29 McDowell, W. c., 407, 413 McDowell, W. J., 77, 892, 979, 1011, 1031,

1054, 1056, 1057, 1080, 1098, 1099, 1283, 1337, 1346, 1483, 1499

MacDuffee, W. T., 184, 186 McElroy, D., 668, 671, 1339 McElroy, D. L., 1340 Macfarlane, R. D., 1093, 1190 McGill, R. M., 304 McGlashan, M. L., 1092 McGlynn, S. P., 218, 344,345, 1367 McGowan, F. K., 217 McGuire, S. c., 990, 1028 MacInnes, D. A., 344, 1321 Mcisaac, L. D., 892

Author Index

McKay, H. A. C., 104, 112, /l3, 114, 117, /l8, 120,407,410, 4/l, 412, 506, 525, 527, 1057, 1502, 1521, 1522, 1522, 1523, 1523

Mackey, D. J., 1264 Mackey, D. R., 1517 McKinley, L. c., 686 Mclane, C. K., 784, 800, 802 Mclaughlin, R., 967, 1058, 1058, 1260, 1379,

1382 Mclaughlin, R. D., 585, 587 Macleod, A. c., 1328 McMillan, E. M., 4, 6, 443, 444, 499, 643,

644,645,648,652,653 McMillan, T. S., 311 McNally, J. R., 211, 212, 212, 213, 578, 579 McNally, J. R., Jr, 1227 McNeese, W. D., 593, 656 McNeille, S. M., 177 McNeilly, C. E., 643, 680, 683, 690, 697, 904,

909 McTaggart, F. K., 65 McVey, T., 320 McVey, T. N., 320 McVey, W. H., 582, 584, 585, 586, 704, 784,

799,819 McWhan, D. B., 897, 900 Maddock, A. G., 102, 104, /l3, 114, 117, /l8,

119,120,121,124,142,145,149,151, 658,701,774,817

Madic, C., 930, 1504, 1538 Maeda, M., 1492 Maekawa, S., 1411 Magel, T. S., 590, 591,643 Magette, M., 463, 1447 Magill, J., 1321, 1328 Magini, M., 85 Magnani, N. J., 1319 Magnon, L., 1431 Magnusson, D. W., 313 Magnusson, L. B., 6, 456, 465, 470, 471, 474,

475 Magon, L., 484, 795, 796, 799, 807, 808, 1492,

1493, 1493, 1507, 1508, 1509, 1510, 1516, 1516, 1517

Mahlum, D. D., 1181 Mahmoudi, S., 344, 345 Mailen,1. c., 891, 1033, 1053, 1323 Maillard, J. P., 212, 212 Mainland, E. W., 687 Maino, F., 969, 975, 976 Majer, V., 1130, 1162 Makarova, T., 931 Makarova, T. P., 812, 814, 1010 Malcic, S. S., 1431, 1450 Malevich, V. M., 1331 Malik, F. B., 994 Malikov, D. A., 992, 1012

Mallet, M. W., 284, 287 Mallett, M. W., 248, 289 Mallory, M. L., 1097, 1098 Maim, J., 103, 134 Maim, J. G., 112, 115, 452, 461, 697, 700,

702, 737, 738, 739, 741, 742, 742, 743, 745, 746, 1264, 1272, 1272, 1324, 1331, 1337, 1338, 1440

Mal'tsev, Yu. G., 334 Maly, J., 1012, 1052, 1091, 1095, 1096, 1098,

1285, 1481, 1483 Malyshev, N. A., 25 Malysheva, L. P., 1033 Mamantov, G., 971, 1052 Mandleberg, C. J., 731, 733, 734, 736, 737,

742, 746, 748, 774, 775, 799, 802 Manes, L., 1378 Manescu, I., 215, 580 Manev, I. N., 149, 150 Manier, M., 151, 152 Mann, I. B., 612 Mann, J. B., 488, 489, 898, 1035, 1080, 1101,

1258, 1633, 1635 Mann, J. P., 218 Manning, W. M., 6, 12,499, 500, 643, 644,

645,648,652,653, 658, 1071, 1086, 1098, 1101,1135,1278,1483,1484

Manriquez, J. M., 83, 381, 1460, 1548, 1565, 1566, 1567, 1568, 1568, 1571, 1588, 1598, 1600, 1602, 1603, 1607, 1614,1615, 1616

Manson, S. T., 995 Mansouri, I., 1446 Manuelli, c., 80 Maple, M. B., 51 Maples, c., 22 Maraman, W. J., 516, 516, 540, 550, 553, 554,

558, 559, 561, 566, 567, 568, 570, 570, 571,576,577,595,596,597,618,619, 621,661,674,687, 700,705

Marangoni, G., 1431, 1452 Marckwald, W., 16 Marcon, J. P., 294, 295, 296, 460, 677, 705,

706, 707, 708, 709, 710, 725, 728, 908, 1321, 1337

Marconi, W., 378, 1463, 1548, 1548, 1572 Marcus, J. A., 232 Marcus, R. A., 480 Marcus, R. J., 480 Marcus, Y., 85, 481, 799, 799,800,802,803,

893, 903, 908, 912, 918, 919, 926, 930, 931,932,943,1030,1506,1517,1518, 1519, 1521, 1523

Marden, J. W., 52, 67 Mardon, P. G., 452, 453, 606, 613, 623, 641,

643, 645, 646, 650, 654, 673, 1397 Marei, S. A., 969, 971, 974 Maresca, L., 1507

Author Index

Margherita, S., 85 Margorian, M. N., 487 Margrave, J. L., 1589 Maria, R., 19 Marinis, J., 730, 730, 731, 736 Marinsky, J. A., 304 Mark, R., 994, 1034 Markin, T. L., 680, 683, 695, 696, 696, 698,

725,779,780,907,911,928,1321 Markov, B., 1110 Markov, B. N., 1630 Markowski, P. J., 66 Marks, T. J., 83, 84, 381, 384, 385, 386, 1166,

1169, 1367, 1459, 1460, 1461, 1548, 1551, 1552, 1553, lSS5, 1558, 1559, 1560, 1561, 1562, 1565, 1566, 1567, 1568, 1568, 1569, 1571, 1571, 1578, 1588, 1590, 1591, 1593, 1594, 1598, 1599, 1599, 1600, 1601, 1602, 1603, 1603, 1605, 1605, 1607, 1608, 1608, 1609, 1610, 1610, 1614, 1614, 1615, 1616, 1617, 1618, 1618, 1619, 1620,1621, 1622, 1622, 1623

Marlein, J., 27 Marorina, N. N., 811 Marov, I. N., 810 Marov, N., 804 Marples, J. A. C., 126, 128, 453, 456, 606,

613, 623, 641, 643, 650, 653, 654, 655, 673,674, 714

Marquart, R., 355, 687, 690, 703, 727, 762, 765, 765, 766, 784, 907

Marquet-Ellis, R., 308, 1373, 1579, 1594, 1596, 1598

Marrus, R., 125 Marshall, W. L., 362 Marteau, M., 465, 470, 1335 Martell, A. E., 798, 816, 817, 930, 1499, 1504,

1508, 1509, 1513, 1514 Martensson, N., 1395 Martin, A., 259, 260, 673 Martin, A. E., 599, 606 Martin, D., 1123 Martin, D. B., 644 Martin, D. J., 677, 1339 Martin, F. S., 506 Martin, G. A., Jr, 335, 387, 389, 394, 395 Martin, G. R., 124 Martin, J. F., 1327, 1328, 1329 Martinot, L., 457, 458, 469, 783, 818, 915,

979, 1014, 1280, 1285, 1290, 1335 Martin, P. E., 799 Martin, W. C., 1033, 1094, 1098, 1103, 1292,

1293 Martinsen, M., 65, 66, 67, 71, 72, 73, 74 Marty, N., 124 Martynova, N. S., 334 Marzano, C., 227 Mashirov, G., 344, 345

Masino, A. P., 1559 Maslov, O. D., 1106 Mason, E. A., 506, 570 Mason, G. W., 22, 86, lll, 112, 115, 116,

446,450,503,505,893,931,933,991, 1012

Mason,J. T.,69, 72, 74, 234, 238,1440,1441 Mason, T., 109, 124 Massalski, T. B., 1403 Massei, A., 1460 Masson, J. P., 319, 1324 Masters, B. J., 801 Mastick, D. F., 540, 567 Mathers, W. G., 803 Mathesen, R., 389 Mathew, K. A., 33, 34 Mathieson, A. R., 410, 411 Mathieson, W. A., 528, 529,529,531,532,

534, 553 Mathur, J. N., 979, 980, 992, 1056, 1499 Matignon, C. A., 51, 52, 53, 61, 71, 73 Matkovic, B., 81, 1453 Matlack, G. M., 1344 Matorima, N. N., 810 Matson, L. K., 295, 297 Matsui, T., 1321 Matta, E. A., 1588 Mattern, K. L., 186 Matthews, J. M., 71, 73, 74 Matthias, B. T., 29, 126, 128, 1389 Mattraw, R. C., 742, 743 Matuzenko, M. Yu., 456, 465, 469 Matyashchuk, I. V., 470 Matz, J. J., 745, 749, 752 Maucher, A., 188, 191, 194 Mauermann, R., 1616 Maulden, J. J., 124 Maurette, M., 1171 Maurice, V., 1317, 1318 Mauson, S. T., 1035 Maximov, V., 282 Maxwell, E., 540, 567 May, A. N., 43 May, C. A., 1231 Mayankutty, P. C., 85 Mayer, P. C., 541 Mayerle, J. J., 255, 256, 257, 258, 1432 Mayfield, R. M., 618, 661 Maynard, R. B., 1460, 1596, 1597, 1597 Mayrath, J. E., 1291 Mazumdar, A. S. G., 801 Mazzei, A., 378, 1169, 1458, 1459, 1548, 1548,

1549, 1549, 1573 Mazzi, U., 1507 Mazzochin, G. A., 1510 Mead, F. C., Jr, 26 Meaden, G. A., 614 Meaden, G. D., 614, 616

Author Index

Meaden, G. T., 615 Mealli, c., 1442 Mech, H., 1071 Mech, J. F., 6, 22, III, 446, 450, 503, 505,

1086 Mecham, W. A., 548, 570 Mecham, W. J., 548, 570 Mecrouici, B., 251, 253 Medfod'eva, M. P., 930, 935, 941 Medical Research Council, 661 Medvedovskii, V. 1.,818, 819, 822 Meeker, R. D., 217, 217 Meerwein, H., 390 Mefodeva, M. D., 774, 795, 797, 802, 806,

807,808,810, 812 Mefod'eva, M. P., 13,458,464,469,484,485,

715,784 Mefodiyeva, M. P., 781, 783, 1482 Meggers, W. F., 27, 28, 212, 212, 213, 214,

1224 Mehlhorn, R. J., 994, 995, 1378 Meinke, W. W., 106, 124 Meisel, K., 52, 66 Meissner, K. W., 212, 212, 213 Meitner, L., 4, 15, 103, 106, 110, 112, 115 Mellor, J. W., 80 Melzer, G., 77, 78, 80 Menchikova, T. S., 621, 623, 641,642,643,

644,645,64~ 648,649,650,651,652, 653,654,655,656,660

Mende1eev, D., 103 Mendelsohn, L. B., 1035 Mendelson, A., 227 Mendelssohn, K., 308, 453, 614 Menovsky, A. A., 1409 Menzel, E. R., 1264 Merckle, A., 77, 78, 80 Merill, J. J., 580 Merinis, J., 1046, 1077, 1313 Merinis, J. K., 1005 Merk1, I., 551 Merkusheva, S. A., 81 Merrill, E. T., 521, 523 Merritt, R. C., 187, 191, 192, 197, 198,201,

202, 203, 204, 205, 206, 207, 208 Merz, M. D., 1405 Merz, R., 761, 762 Meschede, D., 1409 Mesmer, R. E., 788, 979, 1141, 1287, 1289,

1289, 1291, 1483, 1485 Messier, D. R., 693 Metiver, H., 791, 792 Metivier, H., 1172, 1178, 1182, 1183, 1184,

1185, 1187 Metta, D., 505 Metta, D. N., 503 Metz, C. F., 661, 764 Metz, Ch. F., 701

Metzger, F. J., 81, 82 Meunier-Piret, J., 1564, 1565, 1565 Mewherter, J. L., 505, 1170 Meyer, F. G., 544, 546 Meyer, G., 910 Meyer, N. J., 85, 1484, 1485, 1486, 1487,

1492, 1495, 1496, 1497 Meyer, R. E., 1099,1346 Meyer, R. J., 52, 71, 78, 80 Meyer, W., 335 Meyerson, G. A., 53 Michalski, T. J., 1190 Michel, G., 212, 212, 1564 Michel, M. C., 505 Michels, R. K., 352 Miedema, A. R., 55, 635, 636, 637 Miedena, A. R., 628, 635, 636, 638, 639 Miessner, W., 51 Mignanelli, M. A., 1332, 1337 Miihling, G., 727 Mikhailichenko, A. I., 25 Mikhailov, V. A., 116, 485 Mikhailov, V. M., 919, 928, 970, 978 Mikhailova, M. A., 22 Mikheev, N. B., 1002, 1009, 1034, 1053, 1081,

1091, 1095, 1139, 1140, 1285, 1290, 1344, 1345,1481

Mikul'skii, Va., 1095 Milanova, A. S., 826, 827 Milazzo, G., 398 Miles, F. T., 544 Miles, G. L., 124, 506, 534, 535 Miles, J. H., 979 Miley, F., 619, 621 Milford, R. P., 548, 570 Milie, N. A., 85 Milic, N. B., 1484, 1485, 1492, 1495, 1497 Miliyukova, M. S., 814 Miller, D. C., 650, 652, 656 Miller, J. F., 53 Miller, J. T., 1574 Milligan, W.O., 13,904,976,1289 Mills, K. C., 289, 294, 297, 1327 Milner, G. W. c., 701 Milner, W. T., 217 Milot, C., 674 Milstead, J., 1096 Milsted, J., 505 Milton, H. T., 313 Milyukova, M. A., 919 Milyukova, M. S., 12,485,795,820,824,887,

892,911,912,913,915,918,926,982, 992, 993, 1012, 1031

Milyukova, S., 1080 Miner, F. J., 755, 759, 784, 826 Miner, W. N., 282, 290, 500, 588, 589, 590,

591,598, 599, 605, 606, 607, 607, 608, 612, 613, 621, 623, 641, 642, 643, 644,

Author Index

Miner, W. N. (Contd.) 645,646,647,648,649,650,651,652, 653, 654, 656, 656, 657, 657, 658, 659, 660, 661, 662, 674, 680, 681, 699

Mintz, E. A., 83, 1551, 1552, 1569, 1571, 1593, 1594, 1605, 1609, 1610, 1614, 1620, 1623

Mintz, M. H., 1335 Misciatelli, P., 76, 77 Mishin, V. Ya., 911 Mitchell, A. W., 460, 667, 671, 673, 676, 679,

680, 710, 902, 904, 907, 1433 Mitchell, M. I., 1504 Mitchell, M. L., 930 Mitchell, R. F., 485 Mitius, A., 56 Mitsugashira, T., 25, 34 Mitsuji, T., 142, 146, 151, 152, 153 Miyake, c., 1368, 1371, 1373, 1375, 1507 Mize, J. P., 106,551 Mkeunier, G., 1431 Moak, D. P., 677 Moeller, R. D., 643 Moeller, T., 13, 30, 966, 967, 1101 Moeller, Th., 211 Moffatt, W. G., 1389 Mogilevskii, A. N., 1012, 1013, 1014 Mohanty, S. R., 121 Moise, C., 1596, 1604, 1623 Moissan, H., 52, 56, 57, 64, 65, 66, 67, 71, 72,

73,74 Molen, G. F., 746 Moline, S. W., 991, 1012 Moller, P., 1643 Molochnikova, A. P., 119 Molochnikova, N. P., 121, 122, 124 Molodkin, A. K., 78, 79, 80, 81, 1452,

1454 Moloy, K. G., 83, 1548, 1569, 1571, 1588,

1603, 1605, 1610, 1616, 1617, 1618 Monard, J. A., 489 Mondange, H., 60 Monet, G. P., 85 Money, R. K., 25, 29 Monk, A. W., 177, 180 Monsecour, M., 16, 23, 25 Montag, T., 1536 Montag, T. A., 924 Monti, H., 606, 623 Montignie, E., 66, 295, 297 Montoloy, F., 319 Moodenbaugh, A. R., 51, 65 Moody, C. D., 1623 Moody, D. c., 385, 386, 387, 1550, 1551,

1551, 1555 Moody, J. 8., 212, 212, 213, 214 Moody, J. W., 295, 297 Moody, K. J., 993, 1644

Moon, K. A., 340 Mooney, R. B., 304 Mooney, R. C. L., 69, 72, 85, 681, 1453 Mooney, R. W., 81 Moore, C. B., 1293 Moore, C. E., 29 Moore, D. A., 1288, 1289, 1289 Moore, F. H., 761, 762 Moore, F. L., 121, 122, 124, 894, 896, 943,

992, 1030 Moore, F. S., 122 Moore, G. E., 120, 582, 795, 911, 1321 Moore, J. E., 311 Moore, J. G., 125,918 Moore, R. H., 891 Moore, R. L., 106 Moore, R. W., 23 Morandi, G., 247 Moreland, P. E., 503 Moreton-Smith, M. J., 673 Morgan, A. N., 570, 571, 574, 575,575, 576,

577, 578, 593, 595, 596, 597, 616, 687, 705, 721, 723, 733, 747, 750

Morgan, A. N., Jr, 593 Morgan, A. R., 104 Morgan, H. W., 250 Morgan, 1. R., 599, 612, 1405 Morgan, L. 0., 6, 887 Morin, 1. K., 232, 233 Morinaga, H., 106 Morisseau, J. C., 1504, 1538 Morosin, 8., 365 Morrell, D. G., 1374, 1577 Morrilon, c., 214 Morris, D. F. C., 103 Morris, G. 0., 304 Morrison, B. H., 234 Morrison, G. H., 410 Morrison, J. c., 1245 Morrissey, D. J., 1629, 1644 Morrow, R. J., 1033, 1034 Morss, L., 270, 272, 277, 587, 759 Morss, L. R., 29, 76, 84, 457, 458, 459, 695,

717, 909, 915, 917, 974, 1000, 1003, 1005, 1010, 1012, 1037, 1040, 1045, 1052, 1053, 1058,1076,1137,1139,1154,1162,1163, 1271, 1281, 1282, 1283, 1291, 1292, 1293, 1294, 1294, 1296, 1297, 1297, 1298, 1298, 1299, 1302, 1303, 1303, 1305, 1306, 1309, 1310, 1311, 1315, 1317, 1321, 1331, 1334, 1335, 1336, 1340, 1341, 1343, 1344, 1379, 1397, 1446, 1447, 1593, 1600, 1602, 1603

Morterat, J. P., 288 Mortimer, M. J., 308, 309, 609, 613, 668, 671,

677, 1320, 1334, 1337, 1339, 1340 Mosdzelewski, K., 30, 817, 911, 935, 938, 982,

1520 Moseley, 1., 544, 546

Author Index

Moseley, P. T., 69, 74, 77, 463, 1440, 1441, 1444, 1444, 1455, 1458

Moseley, R. D., 746 Moser, J. B., 295, 296, 297, 676, 677, 678,

679,680,705, 706, 707,708,709, 710, 711,712,713,1338,1339

Moskalev, P. N., 911 Moskowitz, D., 54,56, 1432 Moskvichev, E. P., 82, 1431, 1452 Moskvin, A., 1315 Moskvin, A. I., 149, 150,350,351,767,774,

795, 796, 797, 802,805, 806, 807,808, 810,811,812,813,814,815,930,932, 934,935,940, 941, 942, 943, 947, 1289, 1289, 1296, 1306, 1507

Moskvin, L. N., 22 Mosley, W. c., 905, 909, 972, 974, 976 Moss, F. A. J., 966, 967 Moss, J. H., 488 Mott, B. W., 632 Moulin, J. P., 1504, 1538 Moulton, G. H., 574, 575, 578, 687, 690, 733 Mound Laboratory, 618,619, 686 Mrazek, F. c., 1330 Muccigrosso, A. T., 270, 276 Mucker, K., 69, 72, 1440 Mudge, L. K., 687 Mueller, M. H., 53, 54, 76, 270, 676, 1430,

1452 Mueller, W., 29, 102, 127, 128 Mueller, W. M., 1432 Muenstermann, E., 74 Mughabghab, S. F., 887 Mugnier, Y., 1551, 1567 Muis, R. P., 1332 Mukaibo, T., 1327 Mulac, W. A., 911, 912, 926, 970, 979, 1137,

1139,1260,1481 Mulak, J., 13,464,468, 1373 Mulay, L. N., 1366 Mulford, R. N. R., 61, 251, 251, 455, 459,

610,611, 621, 623, 662, 663, 665,665, 666, 667, 668, 669, 670, 672, 676, 680, 681, 683, 690, 691, 694, 699, 700, 700, 724, 725, 902, 904, 910, 1006, 1335, 1336, 1339, 1341, 1426, 1432, 1433

Muller-Westerhoff, U., 1462 Miiller, A., 76 Miiller, B., 270, 270, 271 Miiller, F., 66, 71, 72 Muller, U., 1440 Miiller, W., 13,891,897,900,901,902,904,

907,908,911, 915, 965, 968, 969, 970, 972, 973, 975, 976, 979, 993, 1031, 1091, 1153, 1154,1320, 1340, 1379, 1395, 1397, 1401, 1435, 1518

Miiller-Westerhoff, U., 382,1168,1374,1548, 1573

Mullins, L. J., 516, 544, 546, 567, 570, 574, 575, 576, 589, 593, 594, 595, 596, 598, 598,616,643,677,697,721,723,747, 749, 751, 891, 1338, 1339

Mulokozi, A. M., 761,762 Mundy, R. J., 410 Miinzenberg, G., 7, 1110, 1112, 1630, 1644 Murad, E., 48, 60 Murase, T., 1526, 1527 Murasik, A., 295, 296 Muray, P. G., 969 Murayama, Y., 1192 Murbach, E. W., 128 Murmann, R. K., 1537 Murphree, E. V., 182 Murphy, G. F. M., 174, 176 Murphy, G. M., 183 Murphy, W. F., 226, 227, 229, 230, 231, 232,

740 Murray, A. F., 1407 Murray, C. N., 1170 Murray, Ch., 173 Murray, J. R., 59, 65 Murthy, M. S., 49 Murthy, P. R., 78 Murty, A. S. R., 73 Musikas, c., 142, 151,457,464,465,470,

893, 930, 1012, 1013, /052, 1053, 1335, 1337

Musikas, M. C., 464 Muxart, R .. 102, 104, 106, 116, 122, 129, 130,

131, 132, 133, 134, 142, 145, 146, 148, 151, 152, 153, 1482, 1489

Myasoedov, B., 1007 Myasoedov, B. F., 12, 25, 102, 119, 121, 122,

124, 125, 142, 151, 152,487,887,892, 911,911,912,913,915,918,919,926, 928, 932, 933, 965, 970, 976, 978, 982, 992, 993, 1012, 1013, 1014, 1031, 1052, 1053, 1057, 1059, 1060, 1080

Myasoedev, B. T., 102 Mydlarz, T., 295, 297 Mydosh, J. A., 1409 Myers, M. N., 582, 583, 584, 764, 784 Myers, R. J., 1366

Naefe, P., 270, 270, 271 Nagarajan, G., 742 Nagarajan, K., 1317, 1323 Nair, G. M., 788, 804, 806, 1483 Nairn, J. S., 104, 113, 114, 117, 118, 120 Naito, K., 267, 1321 Nakamura, A., 1593, 1596, 1603 Nakamura, J., 1315, 1321 Nakamura, R., 1616 Nakamura, T., 59, 60 Nakayama, Y., 727 Nance, R. L., 567

Author Index

Nann, E., 182 Nannie, C. A., 890, 899 Naqvi, S.l., 1507 Naray-Szabo, L., 60 Narayanan, K., 61 Narayanankutty, P., 1499, 1503 Narten, A., 1538 Narten, A. n., 484 Nash, K. L., 893 Naslain, R., 56 Nassimbeni, L. R., 1442 Natarajan, P. R., 784 Nater, K. A., 1528 Nathan, 0., 15, 19 National Academy of Sciences, 1131 National Committee on Radiation Protection

and ~easurement, 27 National Nuclear Energy Series, 42 National Research Council, 1126, 1136 Naud, C., 1264 Naumann, D., 336 Navaza, A., 1456, 1458 Nave, S. E., 969, 973, 974, tOoo, 1008, 1008,

1009, 1009, 1013, 1013, 1038, 1379, 1380, 1381, 1382, 1406

Navratail, 1. D., 735 Navratil, 1. D., 13, 506, 544, 546, 593, 746,

762, 764, 765, 1328 Naylor, A., 407 Nazarenko, O. ~., 22 Nazarev, V. K., 802 Nazarov, P. P., 120 Nazarova, I. I., 981, 982 Nebel, D., 807, 808, 809, 810, 811 Nectoux, F., 713, 714, 716, 783 Neely, W. C., 344, 345 Neher, C., 53 Neil, G. R., 215 Neilson, O. B., 106 Neish, A. C., 82 Nekrasova, V. V., 25, 102, 122 Nellis, W. 1., 615, 1366, 1379 Nelson, D. E., 992, 1030 Nelson, F., 25, 120, 338, 339, 399, 788, 790,

791,806,811, 1482,1485, 1487, 1488, 1488, 1489, 1495, 1496, 1526, 1527, 1530

Nelson, G. c., 580 Nelson, n. R., 284, 287 Nelson, R. D., 1403, 1405 Nenot, 1. C., 661, 1172, 1178, 1182, 1183,

1184, 1185, 1187 Nereson, N. G., 56, 667, 1433 Nervik, W. E., 15, 24 Nesper, R., 66 Nestasi, ~. 1. C., 121 Nestor, C. W., 1292, 1293 Nestor, C. W., Jr, 29, 898, 899, 994, 995,

1034, 1088, 1090, 1092, 1098, 1635, 1636, 1641

Neubert, A., 60 Neufeldt, S., 270, 272 Neufeldt, S. J., 459 Neumann, F., 56 Nevitt, ~. V., 62, 64, 667,671,673, 1151,

1390, 1399, 1417, 1435 Newman, D. J., 1236, 1245, 1271, 1371 Newman, F. K., 800 Newton, A. S., 51, 53,54, 55, 61, 66, 67, 71,

73, 77, 225, 326, 327 Newton, T. W., 398, 399,471,475, 787,801,

804,806,817,818,820,828,830,831, 833, 834, 921, 922, 923, 1141, 1291, 1532, 1533, 1534, 1536, 1537, 1538

Nguyen-Nghi, n., 308 Nichols, J. L., 644, 645, 656, 673, 674 Nicholson, E. L., 186 Niedrach, C. W., 227 Nielsen, n. S., 106, 109, 124 Nielsen, O. B., 19, 25, 106, 124 Nielson, C. W., 1211 Nier, A. 0., 171 Nierenberg, W. A., 125 Niessen, G., 270 Nieuwenhuys, G. J., 1409 Nigalagevsky, V. B., 935, 936 Nigon, J. P., 902, 903, 913, 926 Niitsurna, N., 66 Nikaev, A. K., 911, 914, 929, 930 Nikolaev, G. N., 599, 606 Nikolaev, N. S., 757 Nikolaev, V. M., 896, 980 Nikolaevskii, V. B., 783, 911, 912, 914, 918,

929,930 Nikolayev, N. S., 753, 1430 Nikolotova, Z. I., 77, 932 Nikol'skaya, N. A., 813,815 Nikol'skii, V. D., 766, 767, 795, 796, 798 Nilson, L. F., 52, 64, 71, 72, 73, 74, 79, 80 Nininger, R. D., 191, 192, 194 Nishanov, D., 551 Nishina, Y., 106 Nitsche, n., 361 Nitschke, J. ~., 7,964, 1105, 1106, 1108,

1630, 1644 Nix, 1. R., 1643, 1644 Njugent, L. 1., 1553 Nobis, J. F., 394, 395 Noe, ~., 969, 970, 972, 974, 999, tOOO, 1035,

1036, 1036, 1037, 1038, 1046, 1047, 1048, 1050, 1078, 1079, 1382, 1441, 1450

NOel, n., 65, 335 Noland, R. A., 227 Nordenskjold, A. E., 60 Nordling, C., 49 Noren, B., 800,802,1498,1501

Author Index

Normand, C. E., 177, 180 Norreys, J. J., 56 Norris, J. O. W., 218, 221, 784, 1273, 1367 Norvell, V. E., 971, 1052 Nosttorf, R., 326 Noth, H., 56 Nothaft, P. C., 599, 606 Nottorf, R., 298 Nottorf, R. W., 51, 53, 54, 55 Novakov, T., 994 Noverack, J. R., 662 Novikov, G. I., 71, 72 Novikov, Yu, P., 125, 487 Novikova, G. I., 16,21 Novion, C. H. de, 62, 64, 64, 259, 677, 708,

709, 710, 729, 902, 904, 9O~ 908, 970, 972, 975, 976, 1372

Nowak, E. J., 897 Nowikow, J., 145, 146 Nowotny, H., 54, 56 Nuclear Power Fuel Reprocessing Technology

and Economics Conference, 506 Nugent, L. J., 29, 470, 911, 913, 915, 917,

918, 966, 976, 979, 994, 995, 1000, 1012, lOB, 1013, 1014, 1037, 1038, 1040, 1045, 1052, 1052, 1053, 1058, 1076, 1077, 1080, 1081, 1091, 1092, 1095, 1l0l, 1I02, 1206, 1280, 1281, 1282, 1297, 1301, 1315, 1345, 1397, 1447, 1481

Nurmia, M., 7, 16, 1097, 1098, 1100, 1101, 1I02, 1l04, 1l05, 1I07, ll08, 1481, 1630

Nurmia, M. J., 1630 Nurmia, N., 7 Niimberg, H. W., 1507 Nuttall, R. L., 29, 1279, 1315, 1316, 1317,

1318, 1319, 1321, 1322, 1323, 1324, 1326, 132~ 1328, 1329, 1330, 1331, 1332, 1347

Oak Ridge National Laboratory, 104,270, 287

Oak Ridge Operations Office, 308, 311 Oberkirch, W., 83 O'Boyle, D. R., 588, 598, 621, 623, 641, 642,

643,644,645,646,64~648,649,650, 651,652,653,654,656,657,657,658, 659,660,661,662,680,681,699

Ochs, L., 332 Ochsenfeld, W., 528, 533, 534, 784 Ockenden, D. W., 794,816, 1531 Ockenden, H. M., 662, 663, 669, 673, 675 O'Connor, P. R., 795, 797 O'Daniel, A., 327 O'Dean, P. J., 173 Odie, M. D., 232, 233 Odintsova, N. K., 1199, 1228 Odom, J. D., 386, 1550

O'Donnell, T. A., 306, 730 Oelsen, W., 631 Oesterreicher, H., 55 Oetting, F. H., 223, 227, 228, 231 Oetting, F. L., 50, 51, 72, 74, 265, 306, 312,

332, 397, 452, 599, 601, 608, 610, 610, 612,662,663,665,666,668,671,677, 742, 743, 749, 753, 899, 900, 901, 915, 973, 1009, 1014, 1279, 1280, 1282, 1283, 1284, 1285, 1300, 1304, 1306, 1307, 1308, 1309, 1310, 1311, 1312, 1313, 1314, 1315, 1316, 1317, 1319, 1320, 1321, 1323, 1324, 1325, 132~ 1328, 1329, 1332, 1333, 1334, 1335, 1336, 133~ 1338, 1339, 1340, 1341, 1342, 1347, 1389, 1390, 1397

orelt, G. S., 1254 Offer, S., 581 Ofte, D., 612, 686, 688, 728 Oganessian, Yu. Ts., 1644. Oganesyan, Y. T., 1103, 1104, 1107, 1108,

IllO Oganesyan, Yu. Ts., 1630 Ogard, A. E., 574, 575, 575, 576, 578, 616,

667,669, 721, 723, 728, 733, 747, 750, 1337

Ogden, A. J., 1589 Ogden, J. S., 677 Ogle, P. R., 319 Oguchi, T., 1411 O'Hare, P. A., 1332 O'Hare, P. A. G., 1279, 1302, 1308, 1315,

1317, 1318, 1322, 1323, 1324, 1326, 132~ 1329, 1330, 1331, 1332, 1333, 1335, 1336, 1339,1347

Ohnesorge, W. E., 84 Ohse, R. W., 728,969, 1281, 1321, 1328,

1337,1341 Ohta, T., 60 Ohwada, K., 318 Oishi, J., 1306 O'Kelley, G. D., 1095 O'Kelly, G. D. D., 1095 Oklo Phenomenon Symposium, 194,505 Okuhara, T., 61 Oliver, G. D., 313 Oliver, J., 1080 Ollendorff, W., 761, 762, 911, 1454 Olofsson, U., 1290 Olofsson, V., 1170, 1171, lI72, 1172, 1173,

1173, 1174, 1175 Olsen, C. E., 126,128,604,606,614,649,

1372 Olson, C. J., 1412, 1412 Olson, W. M., 61, 459, 668, 672, 676, 683,

684,728,904,910, 1336, 1339, 1341, 1432 000, F., 1327 Ooosov, V. N., 85 Orban, E., 26, 368

Author Index

Orlandini, F., 799,800,801 Orlandini, K. A., 897 Orlemann, E. F., 399 Orlova, O. A., 1644 Orr, P. B., 992, 993, 993, 1031 Ortega, D., 340 Orth, D. A., 562, 563, 572, 573, 593, 687 Osborne, D. R., 228 Osborne, D. W., 53, 251, 306, 461, 697, 700,

1315, 1316, 1322, 1323, 1326, 1330, 1332, 1333, 1335, 1336, 133~ 1338

Oshima, K., 267 Osika, L. M., 270, 276 Osten, H., 390 Ott, H. R., 1409, 1411 Otto, G. W., 599, 610 Otto, K., 251, 252 Otto, R. J., 1644 Ouvrard, L., 60, 81 Ouweltjes, W., 1324, 1325, 1326, 1328, 1331,

1332, 1333, 1337, 1338 Overman, R. F., 992, 1012 Overman, R. T., 123 Oyamada, R., 73

Padiou, J., 294, 295, 296 Pages, M., 67, 68, 71, 81, 82, 85, 463, 490,

710,713, 714, 716, 719, 721, 723, 756, 757, 783, 827, 903, 904, 908, 917, 925, 970, 978, 1446

Pagni, R. M., 1577 Paine, R. T., 893, 981, 1440, 1623 Paine, S. H., 247 Paisner, J. A., 1231 Palache, C., 191, 1453 Paladino, N., 1548, 1548 Palei, P. N., 122, 125, 149, 150,800,

814 Palenzona, A., 1318 Paley, P. N., 813 Palisaar, A.-P., 62 Palladino, N., 378 Palmer, B. A., 214, 1224, 1225, 1226 Palmer, C., 81 Palmy, C., 51 PaI'shin, E. S., 102, 119, 121, 124, 125, 139,

142, 149 Palstra, T. T. M., 1409 Panchanatheswaren, K., 1597 Paolucci, G., 1596 Pape, B. L., 578, 579 Pappalardo, R., 911 Pappalardo, R. G., 902, 903, 911 Paprocki, S. J., 691, 700, 701 Pardue, W. M., 674, 677, 678, 679, 691, 697,

699,700,701,718 Parhi, S., 1492 Parker, V. B., 29, 72, 74, 306, 312, 332, 742,

743, 749, 753, 1279, 1306, 1309, 1310, 1311, 1313, 1315, 1316, 1317, 1318, 1319, 1321, 1322, 1323, 1324, 1326, 1327, 1328, 1329, 1330, 1331, 1332, 1347

Parks, R. D., 51 Parrot, R., 1264 Parsons, B. I., 106, 124 Parsons, R., 396 Parsons, T. C., 83, 969, 970, 1035, 1036, 1037,

1038, 1052, 1053, 1078, 1080, 1382, 1440, 1443, 1462, 1573

Partington, J. R., IS Pascal, J., 232, 233 Pascard, R., 599, 667, 669, 693, 705, 706, 707,

708, 709 Pascual, J., 120, 124 Pasquali, M., 1455 Pastor, R. C., 67 Pasze, A. P., 1362 Paszek, A., 9%, 1034 Paszek, A. P., 218, 1050, 1247, 1251 Patel, C. C., 78 Patel, S. K., 121 Patil, S. K., 488, 779, 780, 932, 979, 980,

1498, 1499, 1503 Patrassi, E., 725, 726 Patrusheva, E. N., 992 Patterson, J. A., 193 Patterson, S. D., 1514 Patton, F. S., 224 Patton, R. L., 702, 737, 776,817 Pattoret, A., 228, 265 Pauh, E. G., 610, 611 Paul, A. D., 800 Paul, M. T., 809, 810, 1513 Paul, R., 270, 276 Paulikas, A. P., 580 Pauling, L., 630 Pauson, P. L., 1164 Pavlova-Verevkina, A. I., 335 Pavone, D., 223 Paw, J. C., 1596, 1597, 1597 Pawlowa, V. K., 816 Paxton, H. C., 502, 502 Peacock, R. D., 461, 730 Peak, S., 1490 Pearce, J. C., 650 Pearce, J. H., 452, 453, 645, 646, 1397 Pearlman, H., 177 Pearson, J. M., 1503 Pearson, R. G., 1497, 1498 Pearson, W., 1623 Pecoraro, L. V., 394 Pecoraro, V. L., 1187 Pedregosa, J. C., 82 Pedretti, U., 378, 1463, 1548, 1548 Peekema, R. M., 482 Peetz, U., 270, 276

Author Index

Pegilot, E., 399 Pekarek, V., 1505, 1507 Peker, L. K., 887 Peligot, E., 169,292, 358, 1517 Pelle, J. P., 270, 271 Pellizetti, E., 481 Pendretti, U., 1572 Peng, Q., 77 Penionzhkevich, Yu. E., 1630 Pennell, R. G., 1306 Penneman, R. A., 67, 68, 70, 71, 82, 135, 136,

137, 152, 318, 319, 380, 385, 386, 387, 756, 757, 784, 786, 804, 806, 887, 891, 892,895,898,902,903,904,910,911, 912,913,914,915,917,918,919,920, 922,926,927,928,928,929,962,971, 973, 976, 978, 1005, 1105, 1108, 1110, 1112, 11 13, 1125, 1127, 1144, 1439, 1440, 1444, 1445, 1446, 1446, 1458, 1459, 1481, 1482, 1530, 1536, 1556, 1635

Peppard, D. F., 22, 77, 86, lll, 112, liS, 116, 407,446,450,503,505,893,931,933, 991, 1012

Perego, G., 1455, 1458, 1459, 1460, 1549, 1549, 1593, 1593, 1596

Perelygin, V. P., 1103 Pererson, J., 106, 109 Peretrukhin, V. F., 470, 783, 784, 911, 912,

914,918,919,930, 970, 979 Peretz, M., 55 Perey, M., 16, 23 Pereyra, R. A., 1403 Perez-Bustamante, J. A., 702 Perezy Jorba, M., 60 Perkins, R. H., 619, 621 Perlman, I., 6, 21, 106, 500, 503, 513, 554,

887,926,962, 963, 1026, 1028, 1123, 1127 Perlman, J., 106 Perlman, M. L., 446, 503 Perret, W. R., 177, 180 Perrin, A., 1430, 1493 Perrin, D. D., 1513 Perrin, J. S., 728 Perrot, P., 1331 Perry, C. C., 544, 546 Perry, D. L., 1431, 1452 Pershina, V. G., 1054 Persson, G., 122 Petcher, T. J., 1441, 1443, 1444 Peterson, D. A., 208, 210 Peterson, D. E., 651, 652, 656, 657, 1341 Peterson, D. T., 23, 50, 50, 51, 53, 54, 55, 65 Peterson, J. R., 747, 748,897,902,903,911,

912,913,917,917,918,926,928,962, 968,969,971,972,973,974,975,976, 979,981,991,995,996,997,998,998, 999, 1000, 1001, 1002, 1003, 1004, 1005, 1006, 1009, lOll, 1012, 1013, 1013, 1014,

1035, 1036, 1036, 1037, 1038, 1041, 1042, 1043, 1046, 1047, 1048, 1050, 1051, 1052, 1052, 1053, 1057, 1058, 1059, 1059, 1060, 1060, 1061, 1078, 1079, 1080, 1080, 1260, 1265, 1290, 1291, 1340, 1341, 1342, 1343, 1379, 1380, 1381, 1382, 1406, 1432, 1435, 1439, 1440, 1441, 1442, 1442, 1443, 1447, 1448, 1450, 1499

Peterson, R. J., 969, 970 Peterson, S., 23, 506,520 Peterson, S. W., 1453 Petrov, K. I., 81 Petrov, P. N., 641,653 Petrukhin, O. M., 1519 Petryna, T., 1095 Petrzhak, G. I., 350,351 Pettit, L. E., 1517 Petty, W. G., 226 Petukhova, I. V., 982 Peyronel, G., 1453 Peurat, H., 129, 130, 131, 145 Pfeil, P. C. L., 233 Pfrepper, G., 145, 146 Philips, B. A., 668, 672 Phillips, G. M., 104, 114, 117, 120,456 Phillips, L., 6 Phillips, M. V., 212, 212, 213, 214 Phillips, S. L., 1291 Phipps, K. D., 686, 688, 690, 728 Phipps, T. E., 610, 611, 691, 731, 733, 734,

1338 Picard, A., 104 Picard, c., 1316, 1321 Picon, M., 294, 295, 296 Pietri, C. E., 769 Pijanovski, S. W., 690 Pilcher, G., 1593 Pilgenrother, A., 227 Pillai, C. N., 61 Pillinger, W. L., 125, 489 Piltz, G., 328 Pinamont, C. J., 659 Pinard, J., 1231 Pinke, A. G. de, 106 Pinkerton, R. C., 399 Pinnick, H. T., 615 Piret-Meunier, J., 83 Pirozhkov, S. V., 106, 120, 9ll, 932, 933, 940,

979,980, 982, 992, 1010, 1057, 1081 Piskunov, E. M., 980 Pissarshewski, L., 60, 61 Pitman, D. T., 56 Pittman, F. K., 516, 540, 567, 773

. Pitzer, K. S., 1291, 1327, 1636 Pitzer, S., 344 Plaisance, M., 146, 147, 149 Planattoni, C., 1430, 1452 Plessy, L., 538, 539

Author Index

Plettinger, H. A., 1506, 1517 Pleve, A. A., 1108, 1630 Plews, M. J., 1556, 1557 Ploetz, G. L., 270, 276 Ploger, F., 227 Plotco, U. M., 1630 Plotko, V. M., 1103, 1104, 1108, 1110 Plowtow, H. E., 250, 251 Pluchet, E., 1482 PlUddemann, W., 80 Plurien, P., 319, 1327, 1368, 1458 Plutonium-238 and Polonium-21O Data

Sheets, 501 Plutonium Chemistry Symposium, 500 Plutonium Ion Exchange Processes, 507, 550,

554,555,556,556,557,560,563 Plymale, D. L., 779, 780 Plyushcheva, N. A., 25 Pocev, S., 1489 Podorozhnyi, A. M., 1091, 1345, 1481 Poggio, S., 1549 Poitreau, J., 677 Polissar, M. J., 326 Poluboyarinov, Y. V., 1104 Polyukhov, V. G., 963, 970, 979 Polyukov, V. G., 990 Pomytkin, V. F., 1228 Pons, F., 645, 657 Poole, D. M., 606, 613, 644, 645, 653, 656 Poole, O. M., 623, 641,643,654 Poon, Y., 1371 Poon, Y. M., 1236, 1245, 1269, 1269, 1271 Popov, D. K., 930, 934, 935, 937, 939, 940,

941,942 Popov, M. M., 700 Popovic, S., 81 Poppensieker, K., 7, 1112, 1630, 1644 Popplewell, D. S., 1180, 1181 Porai-Koshits, M. A., 1452 Poranova, R., 1507 Portanova, R., 484, 795, 796, 807,808, 1492,

1493, 1493, 150~ 1508, 1509, 1510, 1516 Porter, F. T., 216, 1088, 1090 Porter, J. A., 774, 911, 976 Porter, P. E., 1527 Posey, J. C., 308 Poshanskii, B. G., 748, 751 Poskanzer, A. M., 24 Poskin, M., 27 Post, B., 54, 56, 1432 Potel, M., 65, 334, 1443 Potol, 294, 295, 296 Potter, P. E., 289, 670, 673, 674, 1317, 1327,

1328, 1329, 1332, 1337, 1339 Poulsen, 0.,1226 Povey, D. C., 1454 Powell, E. W., 304, 308 Powell, J., 326

Powell, J. E., 51, 53, 54, 55, 1527 Powell, J. R., 544 Powell, R. W., 1077 Powell, T., 298 Powers, J. A., 667 Powers, R. M., 351,352 Pozharskii, B. G., 766, 767, 795, 796, 798,

802, 803, 806 Prasad, R., 1325, 1329 Prater, W. K., 503 Pratt, K. F., 1005 Prawitz, J., 506 Prehaska, C. A., 501 Prescott, C. H., 227 Prewitt, C. T., 1002 Prgystawa, J., 1372 Price, C. E., 63 Price, D. E., 677 Priceman, S., 229, 229, 232 Priest, H. F., 308 Prigent, J., 325, 326, 327, 334 Prince, M. J., 632 Prins, G., 1324, 1325, 1329, 1337, 1338 Pritchard, W. C., 669 Privalova, P. A., 963 Probst, H., 74 Proc. Plutonium Information, 661 Proc. Rocky Flats Symp., 618, 661 Proctor, S. G., 891, 896 Prodic, B., 78, 81, 1452, 1453 Propst, R. c., 1012, 1013, 1481 Propst, R. L., 1053 Prosser, D. L., 502, 686 Prpic, I., 121 Prusakov, V. N., 903, 910, 914 Pruskin, S. L., 1597 Pryce, M. H. L., 1264, 1267, 1367, 1369, 1370 Puechl, K. H., 687 Pugh, R. A., 589, 598, 643 Pugh, W., 120 Pullen, F., 81 Pulliam, B. V., 1227 Purex Technical Manual, 288, 506, 525, 528,

529 Pushlenkov, M. F., 484, 801, 892 Pushlenkov, M. S., 800 Pyle, G. L., 6, 1071, 1086 Pyzhova, Z. I., 25

Quarton, M., 82 Quill, L. L., 443, 1527

Rabardel, L., 59, 60 Rabideau, S., 802, 818, 819,820, 822, 827,

834 Rabideau, S. W., 790, 791, 802, 804, 806, 819,

822, 827, 1482, 1488, 1489, 1534, 1536, 1537, 1538

Author Index

Rabideau, Sh., 800,806,818,820 Rabideau, Sh. W., 801, 803, 818, 819 Rabinovich, I. B., 1554, 1577 Rabinovitch, V. A., 1641 Rabinowitch, E., 12, 170,223,248,249,301,

303, 310, 338, 1324 Racah, G., 48, 1209, 1210, 1217,1224, 1229 Rachev, V. V., 335 Riide, D., 59, 60 Radiation Safety, 661 Radionova, G. N., 992 Radke, J. H., 687 Radzewitz, H., 60, 906, 909 Radziemski, L. J., 1267 Radziemsky, L. J., Jr, 212, 212. 213, 214,

215, 1225, 1226 Rae, A. D., 1430, 1452 Rae, H. K., 736, 737, 742, 746 Raetsky, V. M., 232, 233 Rahman, H. U., 1372 Rai, D., 1288, 1289, 1289 Raich, 8., 224 Rainey, R. H., 125, 529, 701, 791 Rajan, K. S., 1508, 1509 Rajendra Prasad, 1317, 1323 Rajnak, K., 587, 748, 1076, 1200, 1219, 1223,

1226, 1241, 1251, 1254, 1255, 1256, 1262, 1293

Ramadan, A., 121 Ramakrishna, V. V., 121, 1498, 1499, 1503,

1514 Raman, V., 60, 61 Ramaniah, M. V., 33, 34 Ramaswami, D., 741 Ramme1sberg, c., 60 Ramos Alonso, V., 74 Ramsey, W. J., 650, 651 Rana, R. S., 1251 Rand, F. H., 691, 697, 699 Rand, M. H., 42, 50, 51, 56, 57, 58, 66, 223,

227, 228, 231, 234, 234, 236, 237, 238, 239, 240, 241, 242, 243, 251, 265, 281, 282, 283, 283, 288, 288, 329, 452, 455, 599,601,608, 610, 610, 612, 641, 657, 659,660, 665, 667, 668, 669, 671, 672, 677, 683, 693, 696, 697, 697, 698, 700, 705,723,724,731, 734, 741, 742, 753, 899,900,901,973, 1279,1280, 1282, 1315, 1317, 1318, 1320, 1321, 1323, 1328, 1329, 1330, 1331, 1334, 1336, 1337, 1338, 1339,1340, 1341, 1347, 1389, 1390, 1397

Rand, M. W., 1328, 1329, 1339 Randrup, I., 1643 Rao, C. L., 33, 34 Rao, G. L., 804, 806 Rao, G. S., 687, 764 Rao, P. R. V., 1503 Rao, V. K., 33, 34

Raphael, G., 677, 708, 709, 1377 Rapp, K. E., 308 Rappin, M., 645 Raschella, D. L., 979, 1038, 1052, 1060, 1341 Rasmussen, J. J., 904, 909 Rasmussen, M. J., 574, 575, 576, 747 Raspopin, S. P., 71, 72 Raub, E., 51 Rauchle, R. F., 53 Raue, D. J., 740 Rauh, E. G., 48, 51, 52, 59, 60, 228, 456,

1315, 1321, 1335 Rawley, E. I., 774 Rawley, E. L., 658, 817 Raymond, K. N., 83, 382, 383, 394, 775, 779,

816, 1178, 1179, 1183, 1187, 1187, 1458, 1459, 1460, 1461, 1462, 1462, 1463, 1513, 1566, 1566, 1573,1574, 1579

Raymond, N., 1555 Razbitnoi, V. L., 907 Razbitnoi, V. M., 911, 940 Reader, J., 1033, 1094, 1098, 1103, 1199,

1292,1293 Ready, G. T., 678 Reas, W. H., 528, 529, 549, 567, 569, 570,

573,574, 591,687, 810 Reavis, J. G., 574, 575, 575, 578, 667, 668,

673, 677, 733, 747, 750, 758 Rebizant, J., 1377, 1378, 1564 Rechtien, J. J., 1403 Recosio, A., 679 Recovery of Uranium, Proc. Symp. Sao Paulo,

197 Reddy, A. S., 121 Reddy, J. F., 676 Reddy, S. K., 121 Redhead, P. A., 49 Redman, J. D., 754, 758 Redon, A., 764 Redox Technical Manual, 506, 521 Reeb, P., 1567 Reedy, G. T., 1321 Reents, W. D., Jr, 481 Reetz, T., 1090, 1091, 1644 Regge, P. de, 16, 23, 25 Regnaut, P., 746, 764 Rehner, T., 75 Reichlin, R., 1389, 1390 Reichlin, R. L., 968, 969, 970 Reid, A. F., 83, 1554 Reid, J. c., 394, 534, 535 Reid, M. F., 1264 Reihl, B., 1395 Rei11y, J. J., 548, 570 Rei11y, V. J., 918 Rein, 1. E., 570, 705 Reisberg, W., 1630, 1644 Reisdorf, K. H., 7

Author Index

Reisdorf, W., 7,1110,1112,1630,1644 Reisfeld, M., 319 Reisfeld, M. J., 218, 587, 926, 968, 1077,

1080 Reisfield, M. J., 996, 1033, 1242, 1258, 1269,

1271 Reishus, J. W., 691, 691, 692, 693, 694 Reitz, R., 306 Reitz, R. R., 463 Rekas, M., 982 Rembold, F. A., 613 Renkin, J. M., 1564 Rentschler, H. C., 52, 67 Reprocessing of Irradiated Fuels symposium,

506, 569, 570 Reul, J., 29, 891, 900, 965, 968, 969, 970, 972,

973, 979 Reui, R., 969, 1281, 1341 Reuter, H., 289 Rexer, J., 53, 54 Reymond, F., 112 Reynolds, C. T., 1444,1444 Reynolds, F. L., 227 Reynolds, J. G., 1430, 1452, 1458 Reynolds, J. H., 505 Reynolds, L. T., 368, 380, 1166, 1548, 1555 Reynolds, M. B., 306 Reynolds, R. W., 1008, 1077, 1379, 1382 Reynolds, S. A., 106, 110 Reznikova, V. E., 751 Reznutskij, L. R., 1279 Rheingold, A. L., 1623 Rhinehammer, T. B., 317 Rhyne, L. D., 1573 Ribas Bernat, J. G., 74 Rice, O. K., 85 Richards, E. W. T., 125, 577 Richards, R. B., 184, 506, 513, 514, 519, 521,

522, 528, 529, 541 Richardson, A. E., 23 Richardson, G. L., 541 Richardson, M. F., 1264 Richardson, R. P., 1376 Richman, I., 1264 Rickard, C. E. F., 78, 84, 136, 138,779,780,

902, 1441, 1442, 1448, 1455, 1456, 1458, 1561

Ridgeley, A., 577 Ridgway, K. H., 502, 502 Riedel, H. J., 551 Rieke, R. D., 1573 Rietschel, A., 53 Rietz, R. R., 760, 1432 Rigny, P., 1327, 1368, 1373, 1458, 1579 Riha, J., 757 Riley, B., 680, 690 Riley, B. F., 690 Rimmer, B., 84

Rimsky, A., 60, 81, 1446 Rimsky, H., 82 Rin, E. A., 1050 Ringbom, A., 820, 824 Riou, M., 23 Ritcey, G. M., 1518 Ritchey, J. M., 1623 Rittenberg, D., 182 Ritter, G. L., 893 Rizzarelli, E., 1517 Robel, W., 809, 810, 911 Robert, J., 106 Roberts, A. M., 304 Roberts, C. E., 85, 1484, 1485, 1486, 1487,

1495, 1496, 1497 Roberts, F., 679 Roberts, F. P., 551, 674, 889, 896 Roberts, J. T., 192, 304, 529 Roberts, L. E. J., 129, 130, 131, 262, 263, 270,

456, 683, 1322, 1337 Robertson, D. S., 187, 189 Robertson, J. A. L., 588, 598 Robins, B. N., 619, 621 Robinson, A. C., 612, 1403 Robinson, H. P., 747, 752 Robinson, J. M., 12 Robinson, P., 340 Robinson, P. S., 779, 780 Robinson, R. A., 344 Robinson, R. L., 217 Robinson, W. R., 1447 Roche, M. F., 106 Roddy, J. W., 902, 907, 909, 910 Rodger, W. A., 548, 570 Rodinov, Yu. F., 106 Rodionov, V. F., 22 Rodionova, J., 122 Rodionova, L. M., 25, 992 Roell, E., 51, 53 Roesch, D. L., 644 Rogers, A. L., 1442 Rogers, D. R., 701 Rogers, F. J. G., 104, 106, 114, 120 Rogers, J. J. W., 187 Rogers, N. E., 317 Rog!, P., 56, 58 Rogozina, E. M., 930, 934, 935, 937, 939, 940,

941,942 Rohmer, R., 334 Rohr, W. G., 612 Rojas, R. M., 1431 Rokop, D. J., 503 Roll, W., 43 Rollefson, G. K., 80, 577, 578, 579, 585, 1498,

1500 Romero, J. W., 619, 621 Roncari, E., 1507 Ronchi, C., 686

Author Index

Roof, R. B., 647, 651, 652, 656, 657, 670, 674, 900, 1153, 1389, 1390, 1440

Roof, R. B., Jr, 607, 644, 649, 697 Roozeboom, H. W. B., 79 Rosch, N., 1371, 1577 Rose, R. L., 619, 621, 900, 1389 Rosen, A., 974 Rosen, N., 181 Rosen, S., 667, 671, 673 Rosengren, A., 51, 1000, 1034, 1035, 1090 Rosenheim, A., 67, 71, 72, 73, 74, 75, 79, 80 Rosenkevich, N. A., 1053 Rosenthal, M. W., 317, 325, 1186 Rosenzweig, A., 67,68, 70, 136, 137, 887, 910,

962,971,973, 1005, 1144, 1439, 1444, 1445, 1446, 1448

Rosha1t, 1. N., 111 Ross, J. W., 232, 1377 Ross, L. E., 409, 409 Ross, R. G., 993, 1031 Rossetto, G., 1550 Rossetto, R., 1596 Rossi, R., 1560, 1561, 1562 Rossignol, D., 677 Rossini, F., 697, 7(}() Rossini, F. D., 1279 Rossotti, F. J. c., 1499, 1500 Roth, R. S., 270, 271 Roth, W., 977, 1553 Rothschild, B. F., 77 Rothwarf, F., 51 Rough, F. A., 230, 232, 233, 234, 234, 236,

237, 238, 239, 240, 241, 290, 678 Rough, F. H., 233, 234, 234, 236, 237, 238,

239,241 Rourke, F. M., 505, 1170 Rouse, P. E., Jr, 213 Roux, C., 645, 657 Roveri, N., 1431 Rowley, E. L., 701 Roybal, J. C., 567 Roy, K. N., 1325 Roy, R., 60 Rozanov, I. A., 295, 297, 300 Rozen, A. M., 77, 932 Rozenkevich, N. A., 1053, 1081, 1095, 1344 Ruben, H., 1431, 1452 Ruben, H. W., 1432 Rubin, B., 534, 536 Ruby, S. L., 217, 217, 488,899 Ruch, W. c., 208, 210 Rud, V. I., 1107 Rudenko, T. I., 764 Rudigier, H., 1409 Ruedorff, W., 270, 276 Ruff, 0., 52, 308 Ru1fs, C. L., 485 Rumer, I. A., 1053, 1081, 1091, 1095, 1481

Runciman, W. A., 1264, 1372 Rundle, R. E., 51, 53,54, 55, 56, 60, 61, 251,

284,289, 1426, 1427 Runnalls, O. J. C., 299, 453, 621, 623, 624,

642, 643, 645, 646, 649, 650, 674 Runna1s, O. J. C., 900, 902, 902 Runner, I. A., 1344 Rupert, G. N., 61, 63 Rush, R. M., 1492, 1493, 1494 Russ, B. 1., 1445 Russell, A. S., 103, 124 Russell, L. E., 683, 690,717,718,720,722,725 Rustichelli, F., 1378 Ruston, C. L., 1455 Rutherford, E., 15, 16 Rutledge, G. P., 316, 316 Ryabova, A. A., 826, 827 Ryan, A. D., 206 Ryan, 1. L., 204, 205, 550, 554, 700, 755, 773,

803,807,894,896,902,903,913,915,917, 918,943,979, 1012, 1013, 1013, 1045, 1052, 1052, 1053, 1058, 1077, 1269, 1271, 1280, 1288, 1289, 1289, 1481, 1526, 1531

Ryan, R. R., 67, 68, 70, 71, 380, 887, 910, 962, 971, 973, 1005, 1144, 1439, 1440, 1445, 1446, 1446, 1459, 1550, 1551, 1551, 1555, 1556, 1623

Ryan, V. A., 142, 145, 146 Rydberg, 8., 394 Rydberg, J., 142, 149, 151,394,398,407,506,

508, 509, 515,816, 817, 1125, 1127, 1128, 1171, 1176, 1290, 1489, 1511, 1511

Rykov, A. G., 827, 912, 913, 919, 920, 922, 923, 924, 925, 926, 970, 979, 1013, 1050, 1054, 1054, 1291, 1538

Ry1e, 8. G., 186 Ryzhova, L. V., 982 Ryzhov, M. N., 892, 934, 980

Sabatier, R., 1446 Sabine, T. M., 1431, 1452, 1517 Sabine, W. K., 505 Sabol, W. W., 742, 743 Sacconi, L., 351 Sachs, A., 78 Sackett, W. M., 103 Saddington, K., 520,536,1517 Sadowski, G. S., 521 Sahrn, C. c., 1110, 1112, 1630, 1644 Saiki, M., 121 St John, D. S., 21 Saito, E., 1579 Saito, S., 1398, 1398 Saito, Y., 261, 262 Sakairi, M., 24, 33, 34 Sakakibara, T., 66 Sakangue, M., 1049 Sakanoue, M., Ill, 125, 911

Author Index

Salazar, K. V., 306, 385, 386, 387, 1550, 1551, 1551, 1555, 1623

Salem, S. I., 580 Saller, H. A., 230, 232, 233, 234, 234, 236,

237,238,239,241 Salm, C. c., 7 Salman, P., 711 Salmon, P., 295, 297 Salutsky, M. L., 15, 19,27,29, 102, 112, 117 Salvatore, F., 1504 Salzer, M., 69, 71, 757, 1446 Samhoun, K., 29,32,912,913,915,917,917,

918,926,928,971, 1000, 10\3, 1013, 1014, 1038, 1040, 1045, 1046, 1052, 1052, 1053, 1054, 1058, 1059, 1059, 1060, 1077, 1081, 1090, 1091, 1092, 1095, 1099, 1102, 1280, 1281, 1282, 1290, 1291, 1297, 1315, 1320, 1334, 1340, 1343, 1344, 1345, 1346, 1397

Samilov, P. S., 106 Samter, V., 67, 71, 72, 73, 74, 75, 79, 80 Samuel, A. J., 177, 180 Sancier, K. M., 218 Sandenaw, T. A., 599, 604, 606, 606, 607, 608,

610,613,613,614,668,697,699,700, 1336,1339

Sanderson, S. W., 77 Santhamma, M. T., 61 Saprykin, A. S., 912, 918, 971, 978 Sarconi, A., 247 Sari, C., 680, 684, 725, 725, 900 Sarkisov, E. S., 999 Sarup, R., 1251, 1260, 1362 Sasaki, N., 57 Sata, T., 60, 260, 263 Sathe, R. M., 85 Sato, A., 34 Sattelberger, A. P., 1623 Satten, R., 219, 223 Satten, R. A., 1262, 1264, 1362 Satterthwaite, C. B., 53, 54, 55 Satyanarayana, S., 340 Saunders, B. G., 580 Sauro, L. J., 894, 1030 Savage, A. W., 1500 Savage, H., 668, 697, 699, 1337, 1339 Savage, H. W., 177, 180 Savchenko, P., 628, 630 Savnicar, S., 78 Savolainen, J. E., 184, 186 Savoskina, G. P., 892, 1033 Savvin, S. B., 125,487 Sawyer, D. L., 56 Saylor, H. W., 308 Scanlan, J. P., 1504 Scargell, D., 117, 121,123 Scargill, D., 144, 149, 1522, 1523, 1523 Scarife, D. E., 69, 75

Scavinl:!ar, S., 1517 Scavnicar, S., 1452 Schaber, P. M., 1190 Schadel, M., 1644 Schaeffer, J. B., 808, 809, 810 Schafer, H., 72, 73, 85 Schafer, J., 1409 Schaffer, H. J., 226 Schaffer, R., 516, 567 Schaifer, J. B., 1507 Schedin, U., 1492, 1493, 1493 Schegolev, V. A., 1106 ScheIman, G. J., 684 Schelmann, G. J., 697 Schenk, H. J., 196, 1367, 1501, 1507 Schenck-Van den Berg, M., 578, 579 Schenkel, R., 969, 1340 Scherer, V., 133, 135,911, 974, 976, 1454 Scherff, H. L., 121, 142, 146, 1320 Scherrer, V., 1441 Schertz, L. D., 83, 1571, 1609, 1614, 1620 Schickel, R., 673 Schiferl, D., 900, 1389, 1390 Schilling, G., 1555 Schilling, J., 72, 73, 74, 75 Schirber, J. E., 232, 1395 Schlapmann, H., 326 Schlea, C. S., 964 Schlechter, M., 688-Schlesinger, H., 255, 256 Schlesinger, H. I., 394, 395, 755 Schlyter, K., 512, 1495, 1496 Schmets, J. J .. 1314 Schmid, W. F., 81 Schmidt, F. A., 51, 53 Schmidt, H. E., 1340 Schmidt, H. G., 53 Schmidt, K.-H., 1630, 1644 Schmidt, K. H., 7,481, 1110, 1112, 1137,

1139, 1260, 1481, 1630, 1644 Schmidt, K. M., 911, 912, 926, 970, 979 Schmidt, V. S., 447 Schmieder, H., 534, 784 Schmieder, M., 528, 533, 534 Schmitt, J. M., 359 Schmitz, J., 1501 Schmitz-Dumont, 0., 291 Schmorak, M. R., 107\ Schmutz, H., 756, 757, 903 Schneider, A., 284, 534 Schneider, J. H. R., 7, 1112, 1630, 1644 Schneider, J. K., lOll, 1054, 1507, 1510 Schneider, J. R. H., 7, 1630, 1644 Schneider, 0., 293 Schneider, W. F. W., 7, 1112, 1630, 1644 Schneiders, H., 291 Schnidt, K.-H., 1630, 1644 Schoebrechts, J. P., 1334, 1336, 1341

Author Index

Scholder, R., 59, 60 SchomaKer, V., 1439 Schonfeld, F. W., 588, 598, 599, 606, 607,

607, 612, 620, 621, 623, 641, 642, 643, 644,645,646,647,648,649,650,651, 652,653,654,656,657,657,658,659, 660,661,662,674,680,681,687,699

Schonfeld, S. W., 621 Schott, H. J., 7 Schott, H.-J., 1630, 1644 Schrader, R. J., 177,325,326 Schreck, H., 33, 981, 982, 1055 Schreiber, C. L., 1262, 1264, 1362 Schreiber, D. S., 55 Schreiner, F., 461 Schreyer, J. M., 362, 368, 1505 Schrock, H., 911, 934, 939, 942 Schroebrechts, J. P., 1292 Schubert, J., 551, 563, 572, 1186 Schuch, A. F., 607 Schuler, F. W., 52 Schiiler, H., 125 Schull, C. G., 53, 54 Schultz, A. J., 1460, 1598, 1602, 1605, 1614,

1615 Schulz, N., 17 Schulz, W., 501, 513, 554 Schulz, W. W., 12, 13, 125,447,450, 506,

538, 546, 547, 887, 890, 892, 895, 896, 901,915,917,926, 933, 942

Schumann, H., 1616 Schuman, R. P., 106, 109, 110, 124, 142, 145,

146 Schumm, R. H., 29, 1279, 1315, 1316, 1317,

1318, 1319, 1321, 1322, 1323, 1324, 1326, 1327, 1328, 1329, 1330, 1331, 1332, 1347

Schuske, C. L., 548 Schuster, R. E., 85, 1490 Schuurmans, P., 48, 213 Schuurmans, Ph., 212, 212, 213 Schuutmans, Ph., 1251 Schwab, M., 968, 969, 970, 1389, 1390 Schwabe, K., 807, 808 Schwalbe, L., 900 Schwalbe, L. A., 1389, 1390 Schwartz, D. F., 227 Schwartz, M. A., 621 Schwarz, H., 59, 60 Schwarz, R., 60, 80 Schwarzenbach, G., 1498, 1499 Schweiger, J. S., 120 Schwetz, K., 56 Schwiesow, R. L., 1249 Schwochau, K., 196 Schwochau, K., 82, 398, 1367, 1501, 1507 Scibona, G., 482, 483, 799,800,801 Scofield, J. H., 995, 1035 Scoppa, P., 1170, 1174, 1175

Scott, A., 1321 Scott, D. M., 599, 610 Scott, F. A., 482, 687 Scott, R. B., 1323 Scott, R. L., 632 Scott, T. E., 50, 50 Scott, T. R., 410 Scribner, B. F., 214 Scrieffer, J. R., 51 Seaborg, G. T., 4, 5,6, 7, 10, 12, 15, 21, 42,

43, 102, 106, 111, 170, 399, 444, 446, 465, 499, 500, 503,504, 51 I, 512, 513, 521, 550, 552, 554, 643, 644, 645, 648, 652, 653, 658, 802, 818, 819, 887, 889, 904, 911, 962, 990, 992, 993, 994, 1012, 1013, 1026, 1028, 1030, 1056, 1071, 1074, 1086, 1088, 1091, 1092, 1093, 1094, 1096, 1098, 1101, 1102, 1105, 1108, 1110, III 2, 1123, 1127, 1135, 1278, 1527, 1530, 1629, 1630, 1633, 1635, 1636, 1637, 1644

Sears, D. R., 67 Sears, G. W., 691, 731, 733, 734, 1338 Secaur, C. A., 1461, 1569, 1571, 1608 Secoy, C. H., 368, 378 Secoy, G. H., 362 Sedlet, J., 15,32,102,112,121 Seed, J. R., 826 Seefeldt, W. B., 548, 570 Sege, G., 541 Segischer, G., 1055 Segre, E., 4, 6, 106, 500 Seguin, M., 614 Seibold, K., 358 Seidel, W., 1644 Seifert, G. W., 1338 Seifert, R. L., 610, 611, 691, 731, 733, 734 Seiffert, H., 457, 713, 716 Seitz, T., 52 Sekhina, L. D., 810 Sekine, T., 24, 33, 34, 817, 1507, 1511, 1512 Selbin,340 Selbin, J., 83, 219, 220, 381, 1563 Se1chenkov, L. I., 551 Selle, J. E., 644, 700 Sellers, P. A., 126, 127, 128, 129, 130, 131,

1427 Sellers, P.O., 112, 115 Sellman, P. G., 59, 65 Selmanoff, G. D., 599, 606 Selwood, P. W., 270 Semenaud, C., 215 Semochkin, V. M., 120 Seng, W. T., 1030 Sentyurin, I. G., 12, 485, 795, 814, 820, 824 Serebrennikov, V. V., 81 Sergeev, G. M., 981 Serik, V. F., 461, 903, 910, 914 Serpan, C. Z., 604, 607

Author Index

Settle, J. L., 1317, 1326, 1330 Seufzer, P., 548, 570 Sevast'yanov, V. G., 295, 297 Seyam, A. M., 83, 381, 1169, 1459, 1548,

1555, 1559, 1565, 1567, 1571, 1578, 1588, 1590, 1592, 1598, 1614, 1616

Shabana, R., 116, 121, 122 Shabena, R., 116 Shacklett, R. L., 580 Shacter, J., 174 Shafiev, A. I., 896, 992 Shah, A. H., 992 Shahani, C. J., 33, 34 Shalaevskii, M. R., 1090, 1091, 1098, 1102,

1106,1107,1108 Shalek, P. D., 59, 64, 293, 294, 295, 296 ShalimotT, G. M., 1343 ShalimotT, G. V., 1362 Shalinets, A. B., 912, 931, 936, 937, 943, 982 Shanker Das, M., 85 Shannon, R. D., 84, 85, 898,981, 1002, 1154,

1164,1283,1284,1289,1295,1447, 1448

Shanon, R. D., 1041 Sharma, H. D., 779, 780, 1318, 1329, 1336,

1339, 1507 Sharma, V. K., 398 Shatinskii, V. M., 106 Shatokhina, O. B., 783 Shaver, K., 112, 117 Shaw, J. L., 670, 673 Shchegolev, V. A., 1107, 1108 Shchukarev, A. S., 335 Shchukarev, S. A., 334 Sheft, I., 208, 211, 298, 303, 459, 460, 547,

548,570,731, 732,733, 734, 749, 750, 751, 752, 753, 971

Sheline, G. E., 582, 584, 585, 586, 784, 826, 827

Sheline, R. K., 19,25, 1589 Shelton, R. N., 65 Shenoy, G. K., 453, 488, 489, 490, 491, 582,

899, 902, 903, 904, 907, 1407, 1407 Sheppard, J. c., 1526 Sherry, E., 268 Shestakov, B. I., 25, 931 Shestakova, I. A., 25, 32, 33, 1289 Shesterikov, V. N., 447, 982 Shetty, S. Y., 85 Shevchenko, V. B., 116, 527, 767, 800, 802,

805, 806, 1525, 1525 Shi, M., 77 Shikua Huang, 1251 Shilin, I. V., 802 Shiloh, M., 481, 799, 799,800, 802, 903, 926,

930,931,932,943 Shilov, B. V., 1106 Shilov, V. P., 469, 781, 783, 784, 911, 912,

914,918,919,929,930,935,936,971, 978, 1482

Shim, W. A., 691, 691, 692, 693, 694, 728 Shimbarev, E. V., 974, 1004 Shimokawa, J., 673, 674 Shinn, W. A., 671, 738, 740, 742, 746 Shiraldi, D. A., 1569 Shirane, G., 1372 Shirley, V. S., 16, 500, 554, 1071 Shirley, V. W., 172 Shiryaeva, L. V., 263, 264 Shock, R. N., 1389, 1390 Shore, B. W., 1076, 1293 Short, I. F. G., 218, 221 Short, I. G., 784, 1273, 1367 Short, J. F., 104, 114, 120,551 Shortley, G. H., 1207, 1209, 1253 Shoun, R. R., 77, 407, 413,892,904, 1031,

1057 Shuck, A. B., 618, 661 Shui T. Lai, 1251 Shul'gin, L. P., 1481 Shull, C. G., 1427 Shults, W. D., 1012, 1013, 1014 Shunk, F. A., 233, 234, 236, 237, 238, 239,

288, 290, 291 Shupe, M. W., 576, 677, 721, 723 Shupe, W., 616 Shvetsov, I. K., 892, 934, 1010, 1074 Sibieude, F., 60 Sibrina, G. F., 82 Siekierski, S., 1447 Sidall, T. H., 448, 1366 Siddall, T. H., 111,892 Siddham, S., 61 Siegal, M., 1005, 1447 Siegal, S., 1042, 1043, 1046 Siegel, S., 69, 72, 259, 263, 263, 264, 265, 266,

267,268, 269, 1003, 1006, 1441, 1443, 1446 Sienel, G. R., 1555, 1556, 1558, 1560 Sienko, M. J., 1375, 1376 Sierk, A. J., 1644 Sierkierski, S., 125 Sievers, R., 62 Sievers, W., 16 Sieverts, A., 51, 53 Sigurdson, E. R., 1590 Sikkeland, T., 7,551, 1096, 1098, 1099, 1101,

1102, 1285, 1481 Sillen, L. G., 81, 85, 338, 347, 509, 512, 798,

930, 1484, 1485, 1487, 1488, 1491, 1492, 1495, 1499, 1504, 1508, 1509, 1513, 1514

Silva, R., 1105, 1285, 1481 Silva, R. J., 1074, 1088, 1090, 1096, 1097,

1099, 1101, 1101, 1102, 1105, 1107, 1283, 1337, 1346, 1630, 1644

Silva, T., 1096, 1097, 1098, 1104

Author Index

Silver, G. L., 793, 820, 821, 822, 823, 824, 825, 826, 827, 1290

Silveria, E. F. de, 106 Silverton, J. V., 1445 Silvestre, J. P., 82, 721, 723 Simakin, G. A., 470, 912, 971, 978, 1012,

1013, 1014, 1050 Simon, D. M., 364, 408 Simon, S. L., 599, 606 Simonsen, S. H., 1430, 1452 Simpson, F. B., 106 Simpson, O. C., 610, 611, 691, 731, 733, 734,

1338 Simpson, O. C., Jr, 691 S"nnpson, S. J., 1612, 1622 Sims, T. M., 990, 1028 Singer, N., 84 Singer, J., 759 Singh, R. N., 1318, 1329, 1336, 1339 Singh, Z., 1317, 1323, 1325 Sinha, D. N., 76, 77 Sinitsyna, G. S., 25 Sironen, R. J., 677, 893, 931, 933 Sivarakrishna, C. K., 801 Sivaramakrishnan, C. K., 714, 715, 717 Sixoo, G. J., 106, 124 Sjlukic, M., 81 Sjoblom, R., 465, 469, 471, 481, 811, 91I, 912,

926, 970, 979, 1260, 1481 Sjoblom, R. F., 1137 Sjoblom, R. K., 996, 1030, 1050, 1081 Skavdahl, R. E., 643, 671, 680, 681, 683, 685,

690,697 Skelton, W. H., 1319 Skinner, J. A., 1593 Sklyarenko, I. S., 12, 485, 795, 814, 820, 824 Skobelev, N. K., 1107 Skorik, N. A., 81 Skriver, H. L., 999, 1395 Slater, J. C., 1207 Slater, J. L., 1589 Slatin, H., 227 Slee, L. J., 551 Sleight, N. R., 511 Slivnik, J., 71, 319 Sljukiv, M., 1453 Slovyanskikh, V. K., 295, 297, 300, 1435 Smales, A. A., 551 Smiley, S. H., 309 Smimova, E., 648, 650, 651, 652 Smimova, E. A., 1033 Smimova, I. V., 469, 484, 485,781,783, 1482 Smimova, N. D., 813, 815 Smimova, T. V., 715 Smith, A. J., 151, 152, 1441, 1443, 1444, 1446,

1454 Smith, C., 701 Smith, C. M., 662, 663, 665, 666, 1337

Smith, C. S., 588, 598 Smith, D. J., 185, 186 Smith, D. W., 1439 Smith, E. A., 319 Smith, E. F., 71 Smith, E. R., 389, 398 Smith, F. J., 891, 1323 Smith, G. M., 1598, 1599, 1599, 1602, 1605 Smith, G. P., 1638 Smith, G. S., 69,72,654,968,969,970, 1389,

1390, 1440, 1443 Smith, H. E., 551 Smith, H. L., 6, 106, 1071, 1086 Smith, J. A., 964 Smith, J. F., 50, 50, 1319 Smith, J. K., 218, 344, 345, 1367 Smith, J. L., 102, 127, 128, 251, 253, 254, 900,

1040, 1I52, 1152, 1I53, 1340, 1389, 1390, 1392, 1393, 1409, 1410, 1410, 1411, 1412, 1412

Smith, K. A., 1576 Smith, K. D., 1460 Smith, P. K., 968, 1341 Smith, R., 774, 775, 799, 802 Smith, R. A., 674, 677, 678, 679 Smith, R. c., 589, 598, 643 Smith, R. J., 500 Smith, T. D., 812, 813, 814, 815, 1513 Smith, V. H., 1I86 Smith, W. C., 775, 779, 816 Smith, W. L., 775, 816, 1I78, 1I83, 1I87,

1187, 1513 Smithells, C. J., 52, 61 Smoes, S., 228 Smotritskaya, E. S., 641,653 Smutz, H., 1446 Sneider, J. R. H., 1110 Snellgrave, T. R., 218, 784, 802 Snellgrove, T. R., 1273, 1367 Snijders, J. G., 1273 Snoddy, L. B., 182 Snow, A. I., 284 Sobiczewski, A., 1643 Sobolev, Yu. P., 924 Sobolov, Yu. P., 919 Sochina, L. P., 764 Soddy, F., 15, 103 Sofen, S. R., 775, 779, 816 Sofranova, P. M., 270, 271 Sokolov, A. P., 361, 1430, 1452 Sokolov, V. B., 461, 903, 910, 914 Sokursky, Y. N., 599, 606 Solar, J. P., 1377, 1575, 1580 Solar, J. R., 83, 1580 Solarz, R. W., 1231 Sollman, T., 75, 79, 81 Solntsev, V. M., 456 Solov'eva, G. V., 1554, 1577

Author Index

Solt, G., 1377 Somerville, L. P., 1105, 1630 Sommartano, S., 1517 Sommerville, P., 1442 Sonneberger, D. C., 1297, 1341 Sonnenberger, D., 695 Sonnenberger, D. C, 1593, 1594, 1599, 1599,

1600, 1603 Sood, D. D., 1317, 1323, 1325 Sorantin, H., 511, 550, 551 Sorokin, P. P., 1253 Sosnovski, O. A, 826, 827 Sostero, S., 1454 Sotobayashi, T., 121 Souka, N., 116, 121, 122 Soulie, E., 1271, 1371, 1372, 1373 Sowden, R. G., 673 Spahiu, K., 1504 Spaunburgh, R. G., 534 Spear, K. E., 677, 1327, 1329 Specht, S., 551 Spedding, F. H., 53, 250, 250, 253, 326, 590,

591, 1527 Spence, R., 1505 Spence, R. W., 6, 1071, 1086 Spencer-Palmer, H., 300, 306 Spl!va~k0vl1, V., 116 Spiegal, A, 1574 Spiegl, A W., 1578 Spindler, W. C, 612 Spink, D. R., 1518 Spirlet, J. C, 29, 102, 127, 128,292,900,915,

968,969,970,972,1148,1151,1153, 1340, 1377, 1379, 1401

Spirlet, J. E., 1340 Spirlet, M. R., 1564 Spiro, T. G., 1577 Spitsyn, V. I., 120, 125, 142, 149, 264, 267,

469, 470, 781, 783, 784,911, 912, 914, 918,919,929,930,970,971,978,979, 1002, 1009, 1034, 1053, 1054, 1081, 1091, 1095, 1344, 1345, 1481, 1482

Spitz, J., 250 Springer, F. H., 964 Sryatha, U., 723, 724 Staats, P. A, 250 Stacey, R. J., 1403 Stackelberg, M. V., 56 Stafsudd, O. M., 1273 Stakemann, R., 1644 Stalinsky, B., 1327 Stambaugh, C K., 642 Standifer, R. L., 548, 549, 550, 570 Stanley, D. R., 1590 Stannard, J. N., 661 Stanner, J. W., 106 Stanton, H. E., 1076, 1088, 1229 Stapleton, H. J., 125

Starinski, E., 270 Staritzky, E., 585, 586, 687,701, 759, 760,

763, 766, 767, 769, 770, 902, 903, 907, 911, 913, 1452

Starks, D. F., 1462, 1573, 1574 Starks, D. V., 83 Starr, Ch., 177 Stary, I., 1091, 1091 Stary, J., 1011, 1030, 1054, 1055, 1511,1511,

1512,1517,1519,1519 Stather, J. W., 661 Stauffert, P., 1603 Staundenmann, J. L., 65 Stchouzkoy, T., 129, 130, 131, 145 Steahly, F. L., 52, 85 Stebunov, O. B., 931 Stecher, H. H., 1598, 1616 Stecher, P., 54, 56 Steele, B. C H., 1321, 1329 Steemers, T., 686 Steglich, F., 1409 Steidl, D. V., 737, 738, 739, 742, 743, 745 Steiglitz, L., 1553 Stein, L., 27, 120, 135, 139 Stein, P., 1577 Steinberg, E. P., 506, 507 Steindler, M., 548, 570 Steindler, M. J., 461, 662, 737, 738,739, 739,

741,742, 742, 743, 744,745, 746, 1336 Steinhaus, D. W., 212, 212, 213, 214, 1226 Steinhauser, M., 701, 767, 773 Steinitz, M. 0., 232 Steinkopff, H., 247 Steinriicke, E., 83 Ste!son, P. H., 217 Stenger, L., 1005, 1447 Stepanov, A. V., 912, 931, 936, 937, 943, 979,

1011, 1054, 1055 Stepenov, A V., 812,814 Stephanou, S. E., 891, 911, 913, 922, 926 Stephen, J., 125 Stephens, D. R., 453, 599,603, 612 Stephens, F. M., Jr, 202 Stephens, G. R., 900 Stephenson, R., 368 Sternal, R. S., 1569, 1605, 1606, 1620, 1623 Steunenberg, R. K., 334, 548, 570, 649, 737,

738, 739, 742, 1033 Stevens, eM., 503, 505 Stevens, 1. G., 488, 489 Stevens, 1. L., 489 Stevenson, C E., 506, 570 Stevenson, 1. N., 747, 748, 962, 968, 969, 971,

972,973,975,999, 1000, 1001, 1003, 1005, 1006, 1012,1042, 1044, 1439, 1440, 1441

Stevenson, M. 1., 1253 Stevenson, P. C, 15,24, 120, 1644

Author Index

Stevenson, R. L., 521,523 Stevenson, S. N., 1042, 1046 Stewart, D. c., 506, 662, 785, 786 Stewart, G. R., 251, 253, 254, 1279, 1340,

1409, 1410, 1410, 1411 Stewart, M. A. A., 779, 780,903, 1447 Stickland, G., 548, 570 Stieglitz, L., 977 Stiffler, G. L., 662, 666 Stites, J. G., Jr, 29 Stockmeyer, W. H., 338 Stojakovic, P. R., 384, 386 Stokeley, J. R., Jr, 911 Stokely, J. R., 465, 949, 996, 1009, 1012,

1013, 1014, 1052, 1448, 1449, 1456, 1481 Stoll, W., 727 Stollenwerk, A., 1373, 1375 Stollenwerk, A. H., 1376, 1555 Stoller, S. M., 184,506,513,514,519,521,

522, 528, 529, 541 Stone, B. D., 29 Stone, F. G. A., 1547, 1623 Stone, J. A., 125,489,780, 1008, 1364, 1365,

1367, 1367, 1374, 1375, 1376, 1376, 1377, 1378, 1380, 1462, 1463, 1550, 1552, 1559, 1560, 1563, 1573, 1579

Stone, P. L., 1329 Stone, R. E., 1092, 1095, 1481, 1483 Stone, R. S., 661 Storey, A. E., 1454 Storhoek, V. W., 674, 677, 678, 679, 718 Storms, E. K., 54, 57, 667, 668, 668, 669, 671,

673, 676, 677, 678, 1279, 1317, 1318, 1320, 1321, 1328, 1329, 1336, 1339, 1347

Stoughton, R. W., 24, 42, 52, 84,115,124 Stout, J. W., 616 Stout, N. D., 1318 Strassman, F., 106, 110 Strassmann, F., 4, 170, 332, 443 Straumanis, M. E., 50 Street, K., 802 Street, K., Jr, 6, 550, 552, 1025, 1030, 1074,

1088, 1527 Street, R. S., 667, 669, 680, 683, 725 Strehlow, R. A., 754, 758 Streitwieser, A., 382, 1462, 1463 Streitwieser, A., Jr, 83, 1168, 1374, 1377,

1548, 1573, 1574, 1575, 1576, 1577, 1578, 1579, 1580

Strickert, R. G., 1288, 1289, 1289 Strickland, G., 549 Strietwieser, A., Jr, 1573, 1577, 1578, 1578 Striganov, A. R., 578, 1199, 1227, 1228 Stringham, W. S., 27, 112 Strohecker, J. W., 177,325,326 Stroganov, E. V., 361, 1430, 1452 Stromatt, R. W., 482, 487 Stromberg, H. D., 900

Stronski, I., 982 Strotzer, E. F., 52, 64, 65, 66, 293 Strouse, C. E., 904, 910, 1260, 1441 Struebing, V. 0., 623, 639, 641, 643, 646, 647,

659,900 Struss, A. W., 75 Stuart, W. T., 643 Studd, B. F., 84 Studier, M., 184 Studier, M. H., 6, 43, 106, 112, 115, 446, 450,

503,505, 1071, 1086 Stukenbroker, G. L., 578, 579 Stumpp, E., 328 Sturch, E., 234 Sturdy, A. E., 662, 663, 665, 665, 666 Sturdy, G. E., 455 Sturgeon, G. D., 318, 319, 757, 1444, 1445 Subramanian, M. S., 687,764, 1318, 1329,

1336,1339 Subramanyam, V. B., 106 Sudakov, L. V., 456, 974, l()(k Sudarikov, B. N., 197, 806 Sugar, J., 29, 48, 215, 898, 993, 1033, 1076,

1094,1098,1103,1225,1251,1262,1292, 1293

Sugar, J. L., 1231 SugIobov, D. N., 344, 345 SugIobova, I. G., 1332, 1333, 1334, 1445 Suits, E., 1328 Sulerzhitsky, L. D., 503 Sullenger, D. B., 690 Sullivan, A. J., 173 Sullivan, C., 349, 349 Sullivan, J. c., 408, 410, 412, 446, 450, 465,

469,470,471,472,475,477,479,480, 481,482,483,484, 503, 505, 804, 911, 912, 924, 926, 930, 970, 979, 1137, 1139, 1260, 1290, 1291, 1481, 1482, 1487, 1488, 1489,1503, 1504, 1536, 1537, 1538

Siimmerer, K., 1644 Sundaram, S., 742 Sundaresan, M., 85 SUDer, A., 124 Sung-Ching-Yang, G. Y., 106 Sung-Yu, N. K., 1550, 1573 Sun-Tzin-Yan, G. Y., 1107 Suranji, T. M., 85, 1484. 1485, 1492 Surls, J. P., Jr, 895, 1030, 1527 Suskin, M. A., 1236, 1240, 1245 Suski, W., 13,294,295,296,297 Sutcliffe, P. W., 308, 453, 1339 Sutton, 344 Su Yin-Tsang, 761, 762 Suzuki, H., 1598, 1599, 1599, 1600, 1616 Suzuki, S., 25, 34, 120, 142, 146 Suzuki, T., 66, 12l Suzuki, Y., 673, 674 Svantesson, J., 122

Author Index

Swain, H. A., 1456 Swallow, A. G., 84 Swaney, I. R., 319 Swanson, J. L., 759 Swepston, P. N., 1591, 1608, 1620 Swiatecki, W. J., 1644 Swift, W. H., 533, 553 Sylva, R. N., 85 Szczepaniak, W., 1332 Szilard, B., 76 Szklarz, E. G., 57

Tabuteau, A., 719, 721, 723, 904, 908, 1446 Tachiki, M., 1411 Tacon, J., 1455, 1456 Tagawa, H., 1331 Taire, B., 1042, 1043, 1046 Takagi, S., 66 Takahashi, K., 106 Takahashi, Y., 289, 1318, 1326, 1327 Takashi, Y., 1315, 1321 Takats, J., 1559, 1560 Takegahara, K., 66 Tamhina, B., 121 Tanabe, K., 61 Tanaka, K., 61, 83 Tanaka, Y., 61 Tani, B., 1003, 1006, 1441, 1443 Tannenbaum, I. R., 737, 738, 739, 741, 742,

742,746 Tanner, J. P., 976 Tanner, S. P., 980, 982, 995 Tanner, S. R., 1081 Tanon, A., 641, 646, 647, 648, 659 Tarasova, A., 335 Tarrant, J. B., 1081 Tarrant, J. R., 976, 995, 1095, 1098, 1099,

1101, JIOl, 1107, 1283, 1337, 1346, 1483 Tarraut, J. R., 1630 Tate, R. E., 177, 325, 326, 595, 597, 621, 623 Tateno, J., 1331 Tatsumi, K., 344, 1589, 1593, 1596, 1603 Taube, M., 12, 500, 588, 598 Taylor, D. M., 1180, 1181, 1186 Taylor, G. N., 1186 Taylor, J. C., 67, 76, 608, 614, 697, 1430,

1431, 1439, 1440, 1441, 1443, 1448, 1452, 1517

Taylor, J. K., 389, 398 Taylor, K., 681, 683, 694 Taylor, S. R., 22, III Taylor, T. I., 389 Teaney, P. E., 700 Teatum, E. T., 633 Teillac, J., 23, 124 Teillas, J., 106 Tel'noi, V. I., 1554, 1577 Tempest, A. C., 1560, 1561, 1562

Templeton, C. C., 77 Templeton, D. H., 54, 56, 69, 74, 76, 83, 760,

904,909,1430,1431, 1432,1441, 1443, 1447, 1452, 1458, 1463, 1576, 1576, 1580, 1611

Templeton, L. K., 1432, 1458, 1463, 1576, 1576

TenBrink, B. 0., 106 Tenenbaum, M., 668, 672 Tepp, H. G., 208, 210 Ter-Akopian, G. M., 1644 Ter Haar, G. L., 83 ter Meer, N., 902, 911, 1454 Tetenbaum, M., 683, 694, 695, 1294, 1315,

1321, 1337 Teterin, E. G., 735 Tetzlaff, R. N., 501 Teufel, c., 77, 78, 80 Tevebaugh, R., 67, 73 Thakur, A. K., 1329 Thakur, L., 1329 Thamer, J., 352 Theilacker, J. S., 270, 273 Theisen, R., 727 Theison, R., 725, 726 Them, G. G., 122, 124 Thewlis, 1., 229 Thiele, K.-H., 83, 1463, 1592 Thirtle, J. R., 387, 389, 394, 395 Thode, H. G., 504 Thoma, R. E., 67, 70,317,317,320, 1005 Thomas, C. A., 590, 591, 643, 658 Thomas, J. L., 1374 Thomas, J. R., 534,535, 536, 538 Thomas, J. T., 502, 502 Thomas, L. H., 1241 Thomke, K., 71 Thompson, G. H., 965, 966 Thompson, J. 0., 489 Thompson, M. A., 548, 570 Thompson, M. C., 968 Thompson, R. c., 112, 115,474,481, 484,

1178 Thompson, S. G., 6, 7, 513, 990, 1012, 1013,

1025, 1030, 1071, 1086, 1088, 1091, 1092, 1094, 1527, 1528, 1530

Thomson, J., 111 Thomson, J. R., 1623 Thomson, M. C., 969 Thoret, J., 60, 81, 82 Thorium Fuel Cycle Symp., 186 Thorn, R. J., 456, 1321, 1335 Thornton, G., 1371 Thuma, B., 7, 1110, 1630, 1644 Thiimmler, F., 725, 726 Tiessler, R., 270, 276 Tikhomirova, G. S., 992 Timma, D. L., 23

Author Index

Timofeev, G. A., 912, 920, 922, 923, 924, 925, 963, 970, 971, 978, 979, 990, 1012, 1013, 1014, 1050, 1059, 1291

Timoshev, V. G., 527, 800, 802 Ting, G., 116, 125 Tipton, C. R., 620, 683, 684 TishkotT, G. H., 352 Tittel, G., 1644 Tiwari, R. N., 76, 77 Toepke, I. L., 53 Tofie1d, B. c., 271 Tolley, W. B., 747 Tom, S., 106, 124 Tomat, G., 484, 1431, 1492, 1493, 1493, 1507,

1508, 1509, 1510, 1516 Tomilin, S. V., 1291 Tomkins, F. S., 27, 28, 125,213,578,579,

897,1198,1224,1224,1226,1227 Toms, D. 1., 104, 114, 117, 119, 121 Tondello, E., 83, 795, 796, 1492, 1493, 1577 Tondon, V. K., 715, 717 Toops, E. c., 21 Tope, W. G., 669 Topic, M., 81 Topp, N. E., 1048 Topp, S. V., 1178 Torgerson, D. F., 1190 Toropchenova, G. A., 116 Torstenfe1t, B., 1170, 1171, 1172,1172,1173,

1173, 1174, 1175, 1290 Toscano, P. 1., 1616 Toth, K. S., 106 Toth, L. M., 465, 468, 1531 Tourssaint, J. Cl., 902 Toussaint, J. c., 29, 891, 965, 968, 970, 972 Tousset, 1., 23 Toye, R. H., 311 Trainor, R. J., 1407, 1407, 1408, 1408 Trauger, D. B., 42 Trautmann, N., 19, 106, 1644, 1644 Traverso, 0., 1454, 1510, 1550 Travnikov, S. S., 911, 932, 933, 967, 1007 Trees, R. E., 1236 Treiber, A., 83 Tremaine, P. R., 338, 338, 344, 346, 350, 350,

788, 789, 1291 Tretiakova, S. P., 1103, 1107 Tret'yakov, A. A., 1331 Tret'yakov, E. F., 16, 21 Tretyakov, Y. P., 1108 Tretyakova, S. P., 1104, 1108, 1110, 1630,

1644 Trevorrow, L. E., 461, 738, 740, 741, 742,

757,1336 Tridot, G., 279 Triebner, A., 1548, 1553 Tries, V. G., Jr, 541 Trifonov, I. I., 71, 72

Trimmer, J. D., 177 Trinkl, A., 602, 605 Tripathi, S. N., 1322 Troc, R., 13, 295, 296, 1327 Troelstra, S. A., 76 Troeltzsch, R. E., 659 Trofimov, A. S., 106 Trofimov, T. I., 1012, 1013, 1014 Tromp, R. L., 106, 124 Trond, S. S., 319 Troost, L., 56, 60, 81 Trotman-Dickenson, A. F., 13, 887, 910 Troxel, J. E., 62 Troyer, A. de, 25, 26, 27 TRU Operating Manual, 542,545 Truitt, A. L., 585, 586, 760, 766, 767, 769,

770,911 Trukchlayev, P. S., 892, 934 Trukhlyaev, P. S., 980 Trunov, V. K., 60, 82 Truswell, A. E., 304, 733, 735, 736 Trzebiatowski, W., 270 Trzeciak, M. J., 248 Tsang, T., 1368 Tsaryov, S. A., 116 Tschirne, G., 336 Tsigunov, A. N., 264, 267 Tsirlin, V. A., 25 Tso, T. C., 140, 141, 1148, 1430 Tsutsui, M., 1169, 1459, 1548, 1596 Tuck, D. G., 75, 1524,1524 Tucker, C. W., Jr, 229 Tucker, P. A., 644, 686, 688, 728 Tucker, T. C., 994 Tucker, W., 77 Tucotte, R. P., 1042, 1044 Tul'skii, M. N., 461 Turcotte, R. P., 456, 904, 909, 1003, 1004,

1004, 1045, 1341 Turnbull, A. G., 75 Turner, H. W., 1432, 1612, 1622 Turner, T. J., 1611 Tvoerdokhlebov, V. N., 80 Tynan, D. E., 208 Tyree, S. Y., Jr, 1485, 1487

Ueki, T., 76, 1452 Ueno, K., 79, 907 Ugaijn, M., 673, 674 Uistrup, J., 993 Unrein, P. J., 979, 980, 1011, 1054 Uranium Carbide Conf., 287 Uranium Dioxide and Related Phases, 256,

260, 261, 265,267 Uranium Exploration Geology, 191, 194 Urbain, G., 84 Urey, H. c., 182 Uriarte, A. L., 701

Author Index

USAEC, 559, 904 Ustinov, V. A., 1335, 1338

Vaan, J. P., 662 Vaezi-Nasr, F., 121 Vaidyanathan, S., 784 Valenta, E., 212, 212 Valentine, A. M., 576, 616, 721, 723 Valet, G., 270, 276 Valli, K., 19, 106 van Alphen, P. V., 51 van Arkel, A. E., 51, 53 Van den Berg, G. J., 213 van den Berg, J., 1409 van den Bosch, J. C., 212, 212, 213 Van Houten, R., 55 van Lierde, W., 261 Van Mal, H. H., 55 van Rensen, E., 71, 72 Van Winkle, Q., 112, 115 Vance, E. R., 1264 Vance, J. E., 170, 197 Vandegrift, G. F., 450 Vandegrift, R. A., 659 Vanderhooft, N. c., 1550 Vander Sluis, K. L., 29, 911, 966, 976, 994,

1047, 1050, 1101, 1553 Van Deurzen, C. H., 1251 Van Deventer, E. H., 1337, 1339 Van Ghemen, M., 133, 135, 1441 Vanhellemont, G., 697 Van Impe, J., 305, 306 van Meersche, M., 1564, 1565,1565 Van Nice, R., 1452 Vanstrum, P. R., 174 van Tets, A., 1431 van Vlaanderen, P., 1324 Van Vleck, J. H., 1361 Van Winkle, Q., 106, 112 Varga, L., 16 Varga, L. P., 218, 587, 926, 968, 996, 1033,

1077, 1080, 1242, 1258, 1271 Varlashkin, P. G., 1052, 1059, 1059, 1060,

1290, 1291 Varma, C. M., 1411 Varnell, L., 106 Vasil'ev, V. P., 1279 Vasil'ev, V. Ya., 78, 827, 970, 979, 992, 1004,

1012 Vasil'ev, V. Yu., 992 Vasil'kova, I. V., 334 Vasilyev, A. M., 362 Vasseur, C., 902 Vasudeva Rao, P. R., 932, 979, 980, 1514 Vaughan, R. W., 55 Vaughen, V. A. C., 183 Vaughen, V. C. A., 183 Vaughn, G. A., 452, 453

Vaughn, J., 1186 Vaugoyeau, H., 288 Vdovenko, V. M., 344, 345, 350, 350, 361,

364, 540, 541, 803, 931, 1430, 1452 Veal, B. W., 216, 580, 1004, 1035, 1395, 1396 Vedrine, A., 67, 85 Veigele, W. J., 1035 Velasquez-Lopez, 0., 779, 780 Veldhuyzen, E. J. J., 182 Venkatasetty, H., 779, 780 Venugopal, V., 1317, 1323, 1325 Vereshchaguin, Yu. I., 1010 Verges, J., 212, 212, 213, 995, 1034, 1050,

1224, 1226, 1227, 1228 Vermeulen, D., 7, 1112, 1630, 1644 Vermeulen, T., 534, 536 Vernadskii, V. J., 122 Verneuil, A., 76, 80 Vernois, J., 125 Vertes, P., 227 Vesely, V., 1505, 1507 Vidali, M., 78, 1450 Vidanskii, L. M., 268 Vietzke, H., 227 Vigato, P. A., 78, 1450 Villani, S., 173, 174,177, 182, 183 Vinogradov, A. P., 191,811,812 Viswanathan, R., 65 Visyashcheva, G. I., 902, 913, 915, 1291 Vita, O. A., 264 Vityutnev, V. M., 992, 1012, 1054 Vladimirova, M. V., 826, 827 Vladimirova, N. A., 470 Voegeli, R., 1567 Voelz, G. L., 1184 Vogel, G. J., 740 Vogel, R. C., 311, 315, 316, 409, 409, 548,

570,737 Vogl, A., 270, 276 Vogler, S., 548, 570 Vogt, 0., 292, 293, 294 Voight, A. F., 23 Voigt, A. F., 511 Vokhmyakov, A. N., 72 Volck, C., 64, 81, 82 Volkov, T. F., 902, 913, 915 Volkov, Yu. F., 78, 1291, 1431, 1452 Volkova, A. A., 527, 800, 802 Volkova, E. A., 16, 21 Vollmer, S. H., 1460, 1566, 1567, 1568, 1568,

1600, 1602, 1603, 1607, 1614 Voloitis, S., 79, 85 Volz, K., 1458 Volz, W. B., 968, 996, 1033 von Ammon, R., 1459, 1554, 1555, 1558 von Bolton, W., 52, 71, 73 Von Deventer, E. H., 677, 700 von Gunten H. R., 992, 993, 994, 1644

Author Index

Von Schnering, H. G., 66 von Wartenberg, H., 52, 64, 71 Vorob'er, S. P., 810 Vorob'ev, A. F., 1279 Vorob'eva, V. V., 1056 Voronov, N. M., 270, 271 Vyatkina, I. I., 919

Waber, J. T., 245, 282, 290, 620, 621, 623, 630, 632, 633, 633, 634, 1112, 1633

Wachter, P., 298, 1366, 1367, 1368, 1374, 1409 Wachter, W. A., 83, 84, 384, 385, 1367, 1460,

1551, 1552, 1555, 1559, 1591, 1593 Waggener, W. c., 465, 467 Wagman, D. D., 29, 1279, 1306, 1309, 1310,

1311, J3J5, 1316, J3J7, 1318, 1319, 1321, 1322, 1323, 1337

Wagner, D. D., 1324, 1326, 1327, 1328, 1329, 1330, 1331, 1332, 1347

Wagner, F., Jr, 996, 1033, 1034, 1047, 1050 Wagner, F. W., 996, 1034, 1050 Wagner, J. J., 1226 Wagner, R., 270, 276 Wagner, R. M., 918 Wagner, R. P., 746 Wahl, A., 499, 643, 644, 645, 648, 652, 653 Wahl, A. c., 4, 6, 444, 500, 511, 540, 567 Wahlig, B. G., 534 Wailes, P. C., 83 Wailes, R. D., 1554 Wain, A. G., 117, 121,123,894,1522,1523,

1523 Wait, E., 268, 270 Wakerling, R. K., 177 Waldron, M. B., 588, 589, 598, 606, 613, 621,

623, 641, 642, 643, 645, 646, 654, 658, 661,669

Walen, R. J., 106 Walenta, K., 191,373 Walker, A. J. W., 456, 459 Walker, C. R., 264 Walker, D. I., 907 Walker, F. W., 106 Walker, L. A., 1445 Walker, R., 1374, 1463, 1576, 1576, 1577 Wallace, P. L., 650, 651, 653 Wallace, T. c., 56, 1433 Walling, M. T., Jr, 528, 529, 1518 Wallmann,1. c., 6, 602,605, 731, 734, 735,

897, 900, 968, 969, 970, 972, 973, 974, 1449

Wallroth, K. A., 81 Walsh, K. A., 574, 575, 575, 578, 733, 747,

750, 758 Walter, A. J., 117, 119, 129,130,131,262,

263, 582, 683, 784, 1322 Walter, D., 83 Walter, K. H., 459, 713,716,717,718,719,

720, 721, 763, 768, 902, 905, 906, 908, 909, 976, 1453

Walters, R. L., 1170 Walters, R. R., 1326 Walton, A., 111 Walton, G. N., 661 Walton, J. R., 7, 1096 Wang, A., 77 Wang, H.-Y., 78 Wang, W., 77 Wang, Z., 77 Wangersky, P. J., 111 Wapstra, A. H., 16, 106, 172,173,174,175,

500, 554, 887 Ward, J., 969, 1077 Ward, J. W., 251, 253, 254, 901, 915, 999,

1000, 1037, 1040, 1045, 1060, 1076, 1279, 1280, 1281, 1315, 1340, 1341, 1342, 1343, 1344, 1345, 1346, 1395, 1397

Ward, M., 799, 802, 979, 980, 1499 Warden J., 1034 Ware, M. J., 72, 85 Warf, J. C., 67, 73, 77, 327 Warner, J. C., 170, 197, 223, 224, 236, 237,

238,239,240,241,590,591,643,658 Warner, R. K., 407, 407, 413 Warren, B. E., 229 Warren, I. H., 66 Warren, K. D., 1371, 1374, 1577 Wasserburg, G. T., 188 Wasserman, H. J., 1550, 1551, 1551, 1555 Wasserman, N., 29, 898, 899, 1292, 1293 Wassermann, H. J., 1623 Waterbury, G., 764 Waterbury, G. R., 487, 551, 701 Waterman, M. J., 687, 761, 762, 764 Waters, T. N., 1430, 1452 Watrous, R. M., 112, 115 Watson, C. D., 529 Watson, L. M., 216, 216 Watson, R. E., 1001 Watt, G. W., 84 Watts, 0., 1565 Way, R., 623 Weaver, B., 887, 892, 893, 904, 992, 1012,

1091, 1521 Weaver, B. S., 894, 1030 Weaver, C. F., 300 Weaver, E. E., 461, 742, 742, 1338, 1440 Weaver, 1. H., 55 Webb, G. W., 29, 1389 Weber, L. W., 1377, 1378 Weber, M. J., 1050, 1253 Webster, R. K., 551 Wede, U., 807, 809,813,814,815,900 Wedekind, E., 285 Weeks, J. L., 228, 229 Weeks, M. E., 15

Author Index

Weigel, A., 334 Weigel, F., 30, 31, 32, 133, 135, 191,270,272,

273, 276, 311, 334, 335, 336, 337, 344, 347, 355, 362, 365, 366, 367, 373, 602, 605,661,662,687,690,701,703,723, 724,727,735, 749, 751, 752, 753, 755, 759, 761, 762, 763, 765, 766, 767, 768, 769, 770, 773, 784, 803, 902, 903, 907, 911,973,976, 1338, 1341, 1441, 1453, 1454

Weill, F. L., 1187 Weinland, R. F., 80 Weinstock, B., 461,574,575,731,733, 734,

737, 738, 739, 741,742, 742, 743, 746, 1272, 1335, 1336, 1338, 1368, 1369, 1439, 1440

Weisberger, A., 662 Weiss, A., 1453 Weiss, A. R., 224 Weitl, F. L., 394, 775, 779, 816, 1187 Weitzenmiller, F., 621, 623, 642 WeIch, C. A., 685, 686, 687 WeIch, D. A., 669, 673 WeIch, G. A., 662, 663, 675, 687, 764, 794,

799, 802, 804, 806, 979, 980, 1499, 1531 WeIch, R. B., 1644 Welge, R. H., 182 Weller, S., 308 Wells, A. F., 1490 Wells, H. L., 71, 73 Wending, E., 344,345 Wendlandt, W. W., 77 Wendolkowski, W. S., 315 Wendt, H., 412 Wensch, G. W., 650, 656, 660 Wenz, D., 334 Wenzel, A. W., 769 Wenzel, U., 551 Werner, G. D., 340, 587, 588, 755, 759, 763,

767, 768, 803, 903, 906 Werner, G. K., 578, 579, 911, 976, 995, 1047,

1050, 1080, 1081, 1553 Werner, L. B., 6,500,511,512,926,962 Werter, D. W., 769 Wessels, G. F. S., 84, 1456 Wester, D. W., 464, 468, 995, 1255, 1290 Westgaard, L., 109, 124 Westlake, D. G., 53, 54 Westrum, E. F., 452, 731, 734 Westrum, E. F., Jr, 306, 589, 590, 591, 598,

643, 674, 675, 681, 687, 690, 705, 707, 747,751,752, 1279, 1304, 1315, 1316, 1317,1318, 1320, 1321, 1322, 1323, 1324, 1325, 1326, 1327, 1328, 1329, 1331, 1333, 1335, 1337, 1338, 1339, 1341, 1342, 1343, 1347

Westrum, E. F., Jr, 76, 1321 Wet, J. F. de, 1442, 1443

Wever, F., 631 Whatley, M. E., 186 Wheeler, V. J., 77, 1321 Wheelwright, E. J., 550, 554, 803, 889, 896,

1531 White, A. G., 799 White, A. H., 1455 White, D. B., 673 White, G. D., 320, 621, 669 White, G. M., 84 White, J., 295, 297 White, J. c., 206 White, J. F., 256 White, R., 585, 587 White, R. W., 57, 126, 128 Whitman, C. I., 53, 227 Whittaker, B., 122, 132, 135, 140, 141, 1148,

1267, 1269, 1320, 1369, 1369, 1442, 1455, 1456, 1458

Whyte, D. D., 650, 656, 660 Wick, G. c., 106 Wick, O. J., 13,500,513,516,588,598,600,

607,608,618,618,621,623,658,662, 663, 686, 698, 725, 728, 760, 838

Wicke, E., 251, 252 Wickman, H. H., 971 Wiedenheft, c., 1456 Wieliczka, D. M., 1412, 1412 Wienwandt, T. A., 455 Wiewandt, T. A., 1335, 1432 Wiggins, J. T., 1031 Wigley, D. A., 614 Wijkstra, J., 992 Wild, J. F., 963, 1042, 1046, 1047, 1050, 1092,

1094, 1095, 1105, 1106, 1260, 1441, 1481, 1644

Wilhelm, H. A., 52, 53, 56, 224, 225, 284 Wilhite, R. N., 349 Wilhite, R. W., 1503 Wilke, G., 83, 1548 Wilkins, R. G., 151, 152 Wilkinson, G., 368, 380, 1166, 1547, 1548,

1555, 1590 Wilkinson, W. D., 170, 191,201,206,223,

226,226,227,229,230,231,232,233, 244, 245, 246, 285, 286, 500, 574, 588. 598,599,606,612,614,618,621,623. 644, 656, 658, 660, 661

Willett, R. D., 81 Williams, c., 1264, 1272, 1272 Williams, C. W., 587, 717,995, 1050, 1271,

1272, 1298, 1302, 1331, 1336, 1340 Williams, E. H., 1490 Williams, J., 725 Williams, J. M., 1460, 1598, 1602, 1605, 1614,

1615 Williams, K. E., 1105 Williams, K. R., 1010, 1012, 1057

Author Index

Williams, P., 79 Williamson, G. K., 606, 613, 623, 641, 643,

653,654 Williams, R J., 1289 Willis, B. T. M., 260, 261, 261, 262, 264 Willis, J. D., 1153 Willis, J. M., 71, 73 Willis, J. 0., 1409, 1410, 1410 Wilmarth, P., 1644 Wilson, A. S., 51, 53,54, 55, 60, 61, 284, 289,

1526 Wilson, D. W., 63, 66, 67 Wilson, H. D., 1030 Wilson, J. R., 599, 606 Wilson, M., 125, 133, 1199, 1217 Wilson, P. W., 327, 1439, 1440, 1441, 1443,

1448 Wilson, W., 340 Winchester, R. S., 516, 516, 550, 567, 570 Wing, R. 0., 746 Wingchen, H., 72, 74 Wink, D. J., 1590 Winkler, C., 51, 52, 53 Winkler, J., 270, 276 Winocur, J., 125 Winslow, G. H., 267 Winslow, J. S., /321 Wirth, A., 325, 327 Wirth, F., 79, 80, 136,138 Wirth, G., 1644 Wischow, R. P., 186 Wise, H., 213 Wise, H. S., 125 Wish, L., 551 Wishnevsky, V., 749, 751, 752, 753, 902, 903,

1338, /341 Wiss, A., 365 Wiswall, R. H., Jr, 544 Witteman, W. G., /329 Wittenberg, L. J., 317,452,453,604,607,

612, 645, 654, 657, 686, 728 Wittman, W. G., 1433 Wittmann, F. D., 907 Wittmann, M., 66 Wittner, E., 325, 326 Wohleben, D., 1409 Wohler, L., 80 Wohler, P., 80 Wojakowski, A., 294, 295, 296, 297, 711, 902,

904,907,908,970,972,975,976,1435 Wojakowski, W., 972, 975 Wolf, A. S., 308 Wolf, G., 53 Wolf, L., 1456 Wolf, M., 902 Wolf, M. J., 77, 121, 124, 745, 749, 750,

752 Wolf, R. A., 502, 502

Wolf, W. P., 1364, 1368 Wolfe, D. L., 567 Wolfs, D. L., 516 Wollan, E. 0., 53,54, 1427 Wolter, F. J., 511, 774 Wolzak, G., 106 Wong, c., 1430, 1457, 1555 Wong, C. H., 1458, 1461 Wong, C.W., 380 Wong, E., 219, 223, 1375 Wong, E. Y., 1262, 1264, 1273, 1362 Wood, D. H., 650, 651, 654, 655 Wood, G. A., 352 Wood, J. H., 251, 253, 254 Wood, R. H., 1291 Woodhead, J. L., 527, 1502 Woodley, R. E., 287, 728, /321, /337 Woodmark, D. R., 1367 Woods, M., 481, 924, 1504 Woodward, L. A., 72, 85 Woodwark, D. R., 218, 784, 802, 1273 Woody, R. J., 199, 201 Woolard, D. C., 78, 1442, 1458 Woolatt, R., 30 Worbleski, D. A., 1623 Worden, E. F., 213, 994, 995, 1033, 1034,

1050, 1075, 1076, 1198, 1226, 1227, 1228, 1229, 1231, 1293

Wright, H. W., 106, 110 Wright, J. c., 587, 598 Wright, J. M., 511, 1527 Wrobleski, D. A., 1623 Wroblewska, J., 719 Wrona, B. J., 679 Wu, C. K., 340 Wu, S.-C., 125 Wyart, J. F., 214, 215, 1034, 1224, 1225, 1226,

1227, 1228, 1229, 1251, 1262 Wyatt, E. I., 106, 110 Wyboume, B. G., 784, 802, 926, 996, 1033,

1210, 1218, 1219, 1223, 1236, 1241, 1244, 1363, 1364

Wylie, A. W., 69, 75 Wymer, R. G., 186, 506, 520, 686, 688, 689 Wyrouboff, G., 60, 75, 76, 80, 359

Xiong, G., 1616 Xu, D., 77 Xu, J., 25 Xu, S., 77

Yacoubi, N., 909, 1044 Yaffe, L., 77 Yakalev, G. N., 120 Yaklovlev, G. N., 1056 Yakolev, G. N., 1431, 1452

Author Index

Yakovlev, G. N., 487,515,807,892,893,896, 902,903,907,9/1,913,915,919,920, 922, 923, 924, 927, 928, 932, 933, 934, 940,979,980,992

Yale, H. L., 394, 395 Yamana, H., 25 Yamauchi, S., 665, 697, 699, 705, 1279, 1316,

1323, 1325, 1337, 1341, 1347 Yanase, A., 66 Yanir, E., 84,912,918,919, 1506, 1517, 1518,

1519, 1521, 1523 Yarembash, E. I., 295, 297, 1435 Yasaki, T., 106 Yashin, M. M., 578 Yashita, S., 1644 Yatzimirskij, K. B., 1279 Yeh, S., 306, 461, 1440 Yen, K.-F., 71, 72 Yen, T., 1458, 1555 Yen, T. M., 380 Yen, W. M., 1257 Yen, W. N., 1251 Yeoman, F. A., 387, 394,395 Yerin, E. A., 1010 Y onco, R. M., 644 Yonts, O. c., 578, 579 Yoshida, N., 83, 1573 Yoshida, S., 73 Young, G. A., 197 Young, J. P., 968, 971, 991, 995, 997, 998,

998, 1003, 1005, 1006, 1007, 1014, 1042, 1046, 1047, 1050, 1051, 1052, 1078, 1079, 1260, 1265, 1440, 1441

Young, R. C., 74 Young, T. F., 347 Ythier, c., 19 Yu, M., 77 Yudina, K. S., 932 Yungman, V. S., 1279, 1293, 1300, 1316,

1317, 1323, 1324, 1325, 1338, 1346 Yiinlii, K., 1596, 1598

Zachariasen, W. H., 29, 30, 31, 53,54,59, 61, 62,63, 64, 65, 67, 68, 71, 75, 126, 127, 128, 129, 130, 131,251,251,287,294, 306, 308, 340, 452, 453, 456, 460, 599, 602, 604, 605, 606, 607, 647, 655, 667, 674, 681, 705, 706, 748, 751, 756, 757, 759, 762, 897, 898, 900, 902, 903, 904, 905, 908, 909, 911, 912, 972, 974, 975, 999, 1006, 1036, 1150, 1389, 1426, 1427, 1430, 1431, 1433, 1434, 1435, 1436, 1439, 1440, 1441, 1443, 1445, 1446, 1449, 1450, 1453, 1501, 1506, 1517

Zachariesen, W. H., 659 Zacharova, F. A., 1482 Zadneprovskii, G. M., 1442

Zager, B. A., 1107 Zagrai, V. D., 551 Zaimorsky, A. S., 599, 606 Zainel, H. A., 1331 Zaitsev, A. A., 919, 924, 980, 981, 1056 Zaitsev, L. M., 77, 764, 774, 795, 797, 802,

806, 807, 808, 810, 812, 930, 935, 941 Zaitseva, L. I., 751, 753, 755, 756, 757 Zaitseva, V. P., 703, 795, 796, 797, 806, 808,

8/1,914 Zakharkin, V. S., 1525, 1525 Zakharova, F. A., 350,351,469,485,781,783 Zakhvataev, B. B., 1106 Zaki, M. R., 1327, 1328 Zalkin, A., 54, 56, 69, 74, 76, 83, 382, 383,

760, 1430, 1431, 1432, 1441, 1452, 1458, 1462, 1462, 1463, 1573, 1574, 1576, 1580, 1605, 1606, 1611, 16/1, 1612

Zalubas, R., 47, 48, 1224, 1225 Zalubas, R. J., 1224 Zambonini, F., 81 Zamir, D., 55 Zamorani, E., 686 Zandin, V. N., 361 Zanella, P., 83, 1550, 1560, 1561, 1562, 1577,

1596 Zanella, R., 1596 Zanotti, G., 1560, 1561, 1562 Zarakhovap, F. A., 783, 784 Zarli, 8., 1430, 1452, 1508 Zastenker, E. E., 795, 798 Zastenker, Y. Y., 766, 767, 795, 796 Zavizziano, H., 115 Zazzetta, A., 1458, 1463 Zdanowicz, E., 66 Zebroski, E., 516,571 Zebroski, E. L., 521, 541, 800, 1503 Zebroski, W., 534, 536 Zeitsev, A. A., 982 Zeitseva, L. L., 1430 Zelenkov, A. G., 106 Zeller, P. G., 1440 Zemlyanukin, V. I., 892, 1525, 1525 Zener, c., 1389 Zenkova, R. A., 907 Zhakarova, F. A., 715 Zhang, Q.-X., 534 Zhou, M. L., 17, 77 Zhu, Y., 25 Zhuikov, B. L., 1090, 1091 Zhuk, M. I., 82 Zielen, A. J., 465, 469, 470, 484, 1335,

1482, 1503 Zielen, J. C., 1536, 1538 Zigan, F., 182 Zijp, W. L., 106, 124 Zimmerman, H., 83 Zimmermann, J. I. C., 169

Zingeno, R. A., 206 Ziomek, J. S., 1321 Zippe, G., 182 Ziv, D. M., 16,21, 32,33, 1289 Zivadinovic, M. S., 1431, 1452 2mbov, K. F., 60 Zolnierek, Z., 1377 Zolotov, Yu. A., 551, 816, 1519 Zolotulcha, S. I., 116 Zons, F. W., 81, 82 Zozoli, G. B., 247

Author Index

Zozulin. A. J., 385, 387, 1550, 1551, 1551, 1555, 1623

Zukas, E. G., 1403 Zumbusch, M., 64, 65 zur Nedden, P., 1517, 1519 Zvara, 1.,1090,1091,1098,1102,1106,1107,

1108, 1281, 1632, 1644 Zvarova, T. S., 1106 Zverev, V. L., 503 Zwolinski, B. J., 480 Zyagintsev, O. E., 806

SUBJECT INDEX Page numbers in italic refer to information in figures or tables.

Absorption spectra divalent actinide ions, 1260-2 higher-valent actinide ions, 1264-73, 1266,

1270, 1272, 1273 tetravalent actinide ions, 1262-4, 1263,

1265 trivalent actinide ions, 1239 see also under individual elements (by name)

Acetylacetonato complexes, 1147, 1511 extraction data for, 1519 stability of, 1511 see also under individual elements (by name)

Acid -base reactions, kinetics of, 1531-2 Actinide concept, 8-9, 1122 Actinide contraction, 1164, 1202, 1425 Actinide elements

antimonides, 62, 64 arsenides, 62, 64 divalent state, stability of, 1053, 1086, 1090 5f-electron effects on, 9, 1392-3 lanthanides compared with, 9; see also

Lanthanides nitrides, 62, 64 oxidation states, 507, 509 phosphides, 62, 64 pnictides, 62, 65 precipitation reactions of, 511 production of, 1122-7 solvent extraction behavior of, 510 un-named elements: see Element

104 ... 109; Superheavy elements Actinides, term discussed, 1388, 1389 Actinium

applications for, 14 atomic properties of, 27-9 bromide

crystal structure data for, 31, 1157, 1441 physical properties of, 1157 preparation of, 31 thermodynamic properties of, 1310

bromo complexes, 33 stability of, 1499

chloride crystal structure data for, 31,1157,1441 physical properties of, 1157 preparation of, 31 thermodynamic properties of, 1309, 1315

chloro complexes, 33 stability of, 1499

discovery of, 15 electron configurations of, 27, 1135, 1203,

1204, 1224, 1237-8, 1237 emission spectra of, 27, 28 fluoride

crystal structure data for, 31, 1157, 1440 physical properties of, 1157 preparation of, 31 thermodynamic properties of, 1306, 1315

global inventory of, 22 halides

crystal structure data for, 31,1157, 1440-1

preparation of, 31 thermodynamic properties of, 1306, 1309,

1310,1315 hydration enthalpy for, 1293 hydride, 1155 hydroxide

activity product of, 1289 solubility of, 32, 34 thermodynamic properties of, 1315

ionic radii of, 1165, 1284, 1289, 1448 ionization energies for, 27, 1293 ions in solution, 30, 32-4

complexation of, 33, 34 redox behavior, 30, 32 solubility of, 32, 33, 34 stability of, 33, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284,1315 isolation of gram quantities, 26-7 isotopes, 14, 16-22

decay properties of, 16-17, 1653-4, 1669 half-life values listed for, 16-17, 1653-4,

1669 production methods for, 16-17, 23, 1123,

1653-4 radiation energies listed for, 16-17,

1653-4 specific activities listed for, 1669

lanthanum compared with, 14 large-scale isolation of, 26-7 metal, 29-30

crystal structure data for, 29, 1150, 1391

Subject Index

Actinium (Contd.) physical properties of, 29, 1150, 1391 preparation of, 29, 1401 thermodynamic properties of, 29, 1150,

1280, 1281, 1315, 1396 metallic radius of, 29-30, 1150, 1450 naphthoyltrifiuoroacetonate complex, 33 naturally occurring isotopes, 22-3 nitrato complex, 33 nuclear properties of isotopes, 16-22, 16-

17, 1653-4, 1669 nuclear spins and moments of, 1648 occurrence in nature of, 22-3 origin of, 15, 103 oxalate, 31, 32,33 oxalato complex, 33 oxidation state of, 30, 1139 oxide

crystal structure data for, 31, 1155, 1421 physical properties of, 1155 preparation of, 31 thermodynamic properties of, 1315

oxyhalides, crystal structure data for, 31, 1443

phosphate, 31 phosphato complex, 33 production facility for, 27 production methods for, 16, 16-17, 23,

1123,1653 reduction potentials of, 32, 1142, 1286, 1287 separation/purification methods, 23--6

cation-exchange chromatography, 25--6 liquid-liquid extraction, 23-5 reverse-phase chromatography, 25--6

solution chemistry of, 30, 32-4 sulfato complexes, 33

stability of, 1503 sulfide, 31, 1437 thiocyanato complexes, 33

Actinium-225 natural occurrence of, 22-3 nuclear properties of, 17, 19,21, 22, 1654,

1669 production of, 17, 19, 1654

Actinium-227 alpha spectrum of, 19 decay products of, 23 gamma spectrum of, 20 nuclear properties of, 16, 17, 19, 1654, 1669 occurrence in nature of, 22 production of, 23, 106, 107, 1654

Actinium-228 gamma spectrum of, 21 nuclear properties of, 16,17, 19,21,1654,

1669 Actinouranium series (4n+3), 14,18,107 Actinyl complexes, structural chemistry of,

1424--6 Actinyl ions

formation of, 1141, 1143 hydrolytic behavior of, 1145--6, 1489-95 spectra of, 1264-7 see also Americyl; Neptunyl; Plutonyl;

Uranyl ions Alkylammonium extractants, 1524--6 Alloying relationships, 1397-9

see also under individual elements (by name) Alloys: see Intermetallic compounds Allyl complexes, 1460, 1548-50 Alpha coefficient, definition of, 824 Alpha decay processes, 1649-50 Alpha-particle spectroscopy, 1651 Americium

absorption spectra of, 926-30, 927, 928, 929, 1239, 1265

acetates, 913 acetato complexes, 934, 945

stability of, 1507 thermodynamics for formation of, 1510

acetylacetonato complexes, 911 aluminate, 902 aluminum alloys, 900, 902 amino-acid complexes, 934, 935, 937, 939,

940, 942, 945 aminocarboxylato complexes, 892, 935, 936,

93~ 938, 942, 944, 945 antimonides, 902, 1438 applications for, 889-90, 1189, 1190 arsenate, 902 arsenazo complexes, 934 arsenide, 902, 1438 atomic properties of, 897-9 autoreduction, 919-20 benzoyltrifiuoroacetonate, 911 benzoyltritluoroacetonato complex, 934 beryllide, 902 biological behavior of, 1174, 1179, 1180,

1181, 1183 bismuthides, 902, 1438 bond lengths of, 897-8 borate, 902 borides, 902, 1433 bromides, 902, 911

crystal structure data for, 902,1140-1, 1157,1158

physical properties of, 1157, 1158 thermodynamic properties of, 1310, 1341

bromo complex, 931 carbide, 902, 1433 carbonates, 902-3, 912-13 carbonato complexes, 913, 931 chlorides, 903, 911

crystal structure data for, 903, 1157, 1440,1442

physical properties of, 1157 thermodynamic properties of, 1299, 1303,

1305, 1309, 1341 chloro complexes, 931, 943, 1499

Subject Index

citrato complexes, 935 cobaltide, 902 complex halides, 910

crystal structure data for, 903 magnetic properties of, 1365, 1378-9 structures of, 1446, 1447 thermodynamic properties of, 1341

complex ions in solution, 930-47 with inorganic ligands, 930, 931-3, 943 with organic ligands, 934-42, 943-4, 944 thermodynamic properties of, 944, 945-6,

947 complex oxides, 905-6, 909

Am --0 bond length in, 898 crystal structure data for, 905-6

complex phosphates, 906 critical mass of, 899 curium complex oxides, 905 cyclo-octatetraenyl complex, 911, 1579 cyclopentadienyl complexes, 911, 1167, 1553 diglycolato complex, 936, 945, 947 dioxide, 909

Am --0 bond length in, 898 crystal structure data for, 1156 magnetic properties of, 1378 physical properties of, 1156 thermodynamic properties of, 1162, 1301,

1312, 1341 discovery of, 5, 6, 887 electron configurations of, 897, 1135, 1203,

1204, 1227 electron energy level scheme for divalent

ion, 1261 emission spectra of, 899 energy level parameters for, 1246 ethylenediaminetetraacetato complexes, 936,

944, 945, 947 thermodynamics of formation for, 1513

fluorides, 903, 910, 914 crystal structure data for, 903, 1157,

1159,1440 electron energy level structures for, 1271 physical properties of, 1157, 1159 thermodynamic properties of, 1306, 1312,

1341 fluoro complexes, 930, 931, 945, 947

stability of, 1498 fluoroacetonates, 911 fluoroacetonato complexes, 934, 939, 942 formate, 911 free-ion energy level structure for, 1249 germanate, 904 glycine complex, 937, 945, 947 g1ycolato complexes, 936, 937

stability of, 1507 hafnium complex oxide, 906 halides, 902, 903, 904, 910

crystal structure data for, 902, 903, 1157, 1158, 1159, 1440-1

physical properties of, 1157, 1158, 1159 thermodynamic properties of, 1305, 1306,

1309, 1312, 1341 halo complexes, 931 Hartree-Fock calculations for, 1221 hexafluoropentanedionato complex, 1456,

1457 8-hydroxyquinolinates, 911 8-hydroxyquinolinato complexes, 935, 938,

939 hydration enthalpy for, 1293 hydrides, 904, 910

crystal structure data for, 904, 910, 1432 physical properties of, 1155 thermodynamic properties of, 1341

hydroxide, 904, 914 thermodynamic properties of, 1288, 1289,

1341 hydroxo complexes, 931 hydroxyisobutyrato complexes, 938 iminodiacetato complexes, 937, 938, 939,

945 iodides, 904, 911


physical properties of, 1157, 1158 thermodynamic properties of, HI 1

ion-exchange separation of, 894-7, 1089, 1528, 1529

ionic radii of, 897, 1165, 1284, 1289, 1448 ionization energies for, 898-9, 1293 ions in solution, 910-47

absorption spectra for, 926-30, 927, 928, 929, 1239, 1265

autoreduction of, 919-20 complexes of, 930-47 disproportionation reactions of, 920-1,

921 electrode potentials of, 915, 917-19, 917 oxidation states of, 910-14, 916, 1139 oxidation-reduction kinetics for, 921-6 preparation of, 916 Raman spectra for, 930 solvent extraction data for, 1519, 1520 stability of, 930-42, 1144, 1288, 1481 thermodynamic properties of, 915, 916,

1280, 1281, 1284, 1299, 1312, 1340 iridium compound, 904 iron compound, 904 isotopes, 8, 887,888

decay properties of, 888, 1172, 1660, 1671 half-life values listed for, 888, 1172, 1660,

1671 production methods for, 888-9, 888,

1124-5, 1660 radiation energies listed for, 888, 1660 specific activities listed for, 1671

lactato complexes, 911 magnetic data for, 1365, 1378-9

Subject Index

Americium (Con/d.) marine organisms affected by, Il74 metal, 899-900

alloys, 900 crystal structure data for, 900, 901, 1150,

1391 hardness of, 901 intermetallic compounds, 900 magnetic properties of, 901 physical properties of, 900, 901,1150,

1391 preparation of, 899-900, 1401 pressure effects on, 900, 90 1 reactivity of, 900 single crystals, 140 I superconductivity of, 900, 1153, 1394 thermal properties of, 901 thermodynamic properties of, 901,1150,

1280, 1281, 1340, 1396 vapor-pressure relationships for, 901

metallic radius of, 897, 901, 1105, 1450 molybdates, 904 monoxide, 904, 909 Mossbauer spectra of, 899 nickel compound, 904 nitrato complexes, 930, 932 nitride, 904, 1438 nitrilo-acid complexes, 939-40, 944, 945,

947 nitrito complex, 932 nuclear properties of isotopes, 887, 888,

1660, 1671 nuclear spins and moments of, 1648 organic compounds, 910, 911, 934-42,

943-4 osmium compound, 904 oxalates, 911, 1454 oxalato complexes, 940, 1507 oxidation states of, 910-14, 1139, 1139 oxidation-reduction reactions in solution,

921-6 hydrogen peroxide reduction, 924-5 neptunium reduction, 924, 925 peroxydisulfate oxidation, 922-4, 922 uranium reduction, 925-6 water reduction, 926

oxides, 904-6, 909 crystal structure data for, 904-6, 1155,

1156 physical properties of, 1155, 1156 thermodynamic properties of, 1162, 1296,

1301, 1312, 1341 see also Americium, complex oxides; ... ,

dioxide; ... , monoxide; ... ; sesquioxide

oxybismuthide, 902, 1438 oxyhalides

crystal structure data for, 903, 1443 thermodynamic properties of, 1341

oxysulfide, 908, 1438 palladium compound, 906 perchlorates, 913 perchiorato complex, 932 phosphates, 906, 912 phosphato complexes, 932 phosphide, 907, 1438 phospho-organic complexes, 935, 936, 937,

938, 939, 941 platinum compounds, 907 plutonium alloys, 900 production methods for, 888-9, 888, 1124-

5, 1660 pyrazolone complexes, 940 pyruvato complex, 941 radioactive decay of, 890, 965, 1172 Raman spectra for, 930 redox kinetics of, 921-6 reduction potentials of, 915, 917-19, 917,

1142, 1286, 1287 in carbonate media, 917, 918 in hydroxide solutions, 917, 918-19 in perchloric acid, 915, 917-18, 917 in phosphoric acid, 917, 918

rhodium compounds, 907 ruthenium compound, 907 salicylate, 911 salicylato complexes, 941, 1455 scandate, 907 selenides, 907, 1438 separation/purification methods, 890-7

amine extraction processes, 893-4 anion-exchange processes, 894-5 cation-exchange processes, 895-7 chromatographic elution schemes, 896 ion-exchange processes, 894-7 molten-salt extraction process, 546, 546,

547,890-1 organophosphorus extraction processes,

892-3 precipitation processes, 891 pyrochemical processes, 890-1 reversed-phase partition chromatographic

procedures, 897 solvent extraction processes, 891-4 TBP process, 892 zirconium phosphate ion-exchange pro

cesses, 896-7 sesquioxide, 909

crystal structure data for, 904, 1155, 1422 physical properties of, 1155 thermodynamic properties of, 1162, 1295,

1296, 1299, 1341 silicate, 907 silicide, 907 sulfates, 908, 913, 1453, 1454 sulfato complexes, 930, 932, 946, 1503 sulfides, 908, 1437, 1438 tartrato complexes, 941

Subject Index

tellurides, 908, 1435, 1436, 1437, 1438 tetramethylheptane-3,5-dionato complex,

1456 thenoyltritluoroacetonate, 911 thenoyltritluoroacetonato complexes,

942 thiocyanato complexes, 894-5, 933, 943,

946, 1514 thiodigiycolato complex, 942, 946 thiogiycolato complexes, 942 toluenesulfonato complexes, 942 trimetaphosphato complex, 933 tropolonato complexes, 939, 942 tungstate, 908 vanadates, 908 x-ray spectra of, 899 xenate,908 zirconium complex oxide, 906

Americium-24I applications for, 889-90 production of, 889

Americium-243 applications for, 890 production of, 889

Americyl acetate, 911 Americyl carbonato complex, 913 Americyl ions

disproportionation of, 1538 stability in solution of, 1144, 1288 thermodynamic properties of, 1340

Americyl pyridine compounds, 911 Ames process, uranium metal manufacture,

224, 226 Applications of actinides, 1188-92

medical applications, 1190-2 neutron sources, 1189-90 nuclear power, 1188-9 portable power sources, 501-2, 1189,

1190-1 see also under individual elements (by name)

Aquatluor process, 549, 550 Arene complexes, 1463, 1572-3 Arsenates, structural chemistry of, 1453

see also under individual elements (by name) Atmosphere, transuranium elements released

into, 1172, 1173 Atomic spectroscopy, 1134, 1196-1231

configuration systematics, 1201-6 empirical analysis, 1199-1201 experimental details, 1197-9 lowest-level lines listed, 1223-9 number of spectral lines in, 1198, 1199 parameter calculations, 1220-3 parameter fitting, 1216-20 term analysis, 1206-16 see also under individual elements (by name)

Atomic vapor laser isotope separation (A VLlS) process, 173, 174

Atomic weights, 1127

Aufbau principle, 1631 Autunite (mineral), 190, 190

Bardeen-Cooper-Schrieffer theory, 51 Beaverlodge (Canada), uranium ore deposits,

193,202 Benzoylacetonato complexes, extraction data

for, 1519 Berkelium

absorption spectra of, 995-8, 997, 998, 1239, 1265

acetato complexes, 1011 stability of, 1507 thermodynamics for formation of, 1510

aminocarboxylato complexes, 1011 antimonide, 1003, 1438 arsenide, 1003, 1438 atomic properties of, 993-8 bromide, 1003, 1005-6


physical properties of, 1158 thermodynamic properties of, 1310, 1343

carbonato complex, 1014 chalcogenides, 1001, 1003, 1006, 1007 chlorides, 1003, 1005


physical properties of, 1157 solid-state absorption spectra of, 998 thermodynamic properties of, 1305, 1309,

1343 chIoro complexes, 1011, 1499 citrato complexes, 1011 complex halides, 1003, 1005

crystal structure data for, 1003 magnetic properties of, 1365, 1380 structure of, 1446, 1447

complexes listed for, 1011 compounds, 1002-9

californium, effect of, 1002 crystal structure data for, 1003 magnetic susceptibility of, 990, 1007-9

cyclopentadienyl complexes, 1003, 1007, 1167, 1460, 1553

1,3-diketonato compound, 1007 dioxide, 1002, 1003, 1004


magnetic properties of, 1008, 1008, 1009, 1379

physical properties of, 1156 thermal expansion properties of, 1004 thermodynamic properties of, 1301, 1312,

1342 discovery of, 5, 6, 990 electron configurations for, 993, 1135, 1203,

1204, 1228 electronic energies of, 993-5, 1204

Subject Index

Berkelium (Contd.) emission spectra of, 995 energy level parameters for trivalent ion,

1246 energy level scheme for divalent ion, 1261 ethylenediaminetetraacetato complexes,

1011,1513 fluorides, 1003, 1005


physical properties of, 1157, 1159 thermodynamic properties of, 1306, 1312,

1342-3 see also Berkelium, tetrafluoride; ... ,

trifluoride fluoro complexes, 1011 free-ion energy level structure for, 1249 glycolate complexes, 1011 halides, 1003, 1004--6

crystal structure data for, 1003, 1157, 1158, 1159, 1440-1


1309,1310,1311,13121342-3 Hartree-Fock calculations for, 1221 hydration enthalpy for, 1293 hydrides, 1003, 1006-7


physical properties of, 1155 hydroxide, activity products of, 1289 hydroxo complexes, 1011 hydroxyisobutyrato complexes, 1011 iodide, 1003, 1006

crystal structure data for, 1003, ll58, 1441

physical properties of, 1158 thermodynamic properties of, 1311

ion-exchange separation of, 992, 993, 1089, 1528, 1529

ionic radii of, 1002, 1165, 1284, 1289, 1448 ionization energies for, 993, 1293 ions in solution, 1009-14

absorption spectra of, 995--6, 1239, 1265 complexes of, 1010, 1011 oxidation states of, 1009, 1139 oxidation-reduction behavior of, 1012-

14 reaction rates of, 1010, 1012 redox potentials for, 1012-14, 1013 solubility of, 10 12 stability of, 1010, lOll, ll44, 1288 thermodynamic properties of, 1009-10,

1280, 1281, 1284, 1342 isotopes, 8, 991

decay properties of, 991, 1662, 1672 production methods for, 990, 991,1662

lactato complexes, 1011 luminescence spectra of, 995

magnetic data for, 990, 1000-1, 1007-9, 1049, 1365, 1379, 1380, 1381

malato complexes, lOll metal

chemical properties of, 1001 crystal structure data for, 999, 1003,

ll50, 1391 electronic configuration of, 1001 magnetic data for, 1000-1, 1380, 1381 physical properties of, 999-1001, 1150,

1391 preparation of, 998-9, 1401 thermodynamic properties of, 1000, 1001,

1150,1280,1281,1342,1396 vapor-pressure relationships for, 1000

metallic radii for, 999, 1150, 1450 nitride, 1003, 1006, 1438 nuclear properties of isotopes, 990, 991,

1662,1672 nuclear spins and moments of, 1648 orthophosphate, 1007 oxalato complexes, lOll oxidation states of, 1002, 1139, ll39 oxides, 1002, 1003, 1004

crystal structure data for, 1003, 1155, ll56

physical properties of, ll55, ll56 thermodynamic properties of, 1296, 1301,

1342 see also Berkelium, dioxide; ... ,

sesquioxide oxyhalides, 1003, 1006, 1443 oxysulfate, 1003, 1007 oxysulfide, 1003, 1007 phosphide, 1003, 1438 pnictides, 1001, 1003, 1006 production capacity for, ll26 production methods for, 990, 991, 1662 radiative relaxation for, 1257 reduction potentials of, 1000, 1143, 1286 selenides, 1003 separation/purification methods, 991-3

chromatographic procedures, 992-3, 994 ion-exchange procedures, 992, 993 redox procedures, 991-2

sesquioxide, 1003, 1004 crystal structure data for, 1003, 1155-6,

1422 physical properties of, 1155-6 thermodynamic properties of, 1296, 1342

sulfato complexes, lOll sulfides, 1003, 1006, 1437 tartrato complexes, lOll tellurides, 1003 tetrafluoride

crystal structure data for, 1003, 1005, ll59

magnetic susceptibility of, 1008, 1008, 1009

Subject Index


thiocyanato complexes, 1011 trifluoride, 1003, 1005

crystal structure data for, 1003, 1157 physical properties of, 1157 thermodynamic properties of, 1306, 1342

x-ray photoelectron spectroscopic studies for, 1004

Beta decay processes, 1650 Biological behavior, 1178-82

body fluids, 1179-80 bone tissues, 1181-2 liver, 1180

Blood, actinide elements in, 1179 Body fluids, state of actinide elements in,

1179-80 Bone tissues, uptake of actinide elements by,

1181-2 Borides, structural chemistry of, 1432-3,

1433,1434 see also under individual elements (by name)

Borohydride compounds, 1167 see also under individual elements (by name)

Bromate oxidation reactions, neptunium, 473, 474

Bromo complexes, 1447, 1499 see also under individual elements (by name)

Butex process, 536 advantages/disadvantages of, 536 extractant used in, 517, 1517,1523 solvent used in, 517

Californium absorption spectra for, 1033, 1051, 1058-

60, 1059, 1239 acetato complexes, 1054


aminocarboxylato complexes, 1055, 1056 antimonide, 1043, 1048, 1438 applications for, 1028-9, 1130, 1189-90,

1192 arsenide, 1043, 1048, 1438 bromides, 1042, 1046, 1047

crystal structure data for, 1042, 1157, 1440-1


carbonato complex, 1052 chalcogenides, 1048 chlorides, 1042, 1046, 1047

absorption spectra for, 1050, 1051 crystal structure data for, 1042, 1157,

1440 physical properties of, 1157 thermodynamic properties of, 1303, 1305,

1309, 1343

chloro complexes, stability of, 1499 citrato complexes, 1055 co-precipitation behavior of, 1053, 1054 comparison with lanthanides, 1039, 1041,

1049, 1051, 1053 complex halides

magnetic properties of, 1382 thermodynamic properties of, 1343

complexes, stability of, 1054-6 compounds, 1040-50

crystal structure data for, 1042-3 magnetic behavior of, 1049-50

cyclopentadienyl complexes, 1043, 1048, 1167

dioxide, 1042, 1044-5 crystal structure data for, 1042, 1156 physical properties of, 1156 thermodynamic properties of, 1301, 1312,

1343 dipivaloylmethanato complex, 1048-9 discovery of,S, 6, 1025 electron configurations for, 1040, 1135,

1203, 1204, 1228 electron energy level scheme for divalent

ion, 1261 electronic properties of, 1033-4 emission spectra for, 1034 energy level parameters for, 1246 ethylenediaminetetraacetato complexes,

1055, 1513 fluorides, 1042, 1045, 1045, 1046



1343 fluoro complexes, 1054, 1498 free-ion energy level structure for, 1249 future studies proposed for, 1060-1 glycolate complex, 1055 halides, 1045-7

crystal structure data for, 1042, 1157, 1158, 1159, 1440-1

hygroscopic nature of, 1047 mixed-valence compounds, 1047 physical properties of, 1046, 1157, 1158,

1159 preparation methods for, 1045, 1046,

1047 thermodynamic properties of, 1305, 1306,

1309, 1310, 1312 Hartree-Fock calculations for, 1221 hydration enthalpy for, 1293 hydride, 1043, 1048 hydroxide, activity products of, 1289 hydroxo complex, 1054 hydroxyisobutyrate complex, 1055 8-hydroxyquinolinato complex, 1056 iminodiacetato complexes, 1056

Subject Index

Californium (Contd.) iodides, 1042, 1046, 1047



ion-exchange separation of, 1030-1, 1032-3, 1032, 1089, 1528, 1529

ionic radii of, 1040, 1041, 1165, 1284, 1289, 1448

ionization energies for, 1293 ions in solution, 1050--60

absorption spectra of, 1058--60, 1239 complexation of, 1054-7 exchange kinetics of, 1057 oxidation states of, 1050, 1053--4, 1139,

1139 oxidation-reduction reactions of, 1052--4 stability of, 1054-7, 1144, 1288 thermodynamic properties of, 1057 -8,

1280, 1281, 1284, 1312, 1343 isotopes, 8, 1027

decay properties of, 1025, 1027, 1028, 1129, 1130, 1663, 1672

production methods for, 1025-8, 1027, 1125, 1126, 1663

lactate complexes, 1055 magnetic properties of, 1049, 1382 malato complex, 1055 marine organisms affected by, 1175 medical applications of, 1192 metal, 1035--40

alloys, 1039 chemical properties of, 1039 crystal structure data for, 1036, 1036,

1037-8,1150, 1391 magnetic properties of, 1038-9, 1040,

1382 physical properties of, 1036-9, 1150,

1391 preparation of, 1035, 1405 thermodynamic properties of, 1038, 1105,

1280, 1281, 1343, 1396 vapor-pressure relationships, 1038 volatility of, 1035, 1038

metallic radii of, 1036, 1037, 1150, 1450 metallic valences of, 1037 neutron emission data for (Cf-252), 1029 nitride, 1043, 1048 nitrilo-acid complexes, 1055 nuclear properties of isotopes, 1027, 1663,

1672 nuclear spins and moments of, 1648 oxalato complexes, 1054 oxidation states of, 1050, 1053--4, 1139,

1139 oxides, 1041, 1042, 1044-5


intermediate-composition species, 1042, 1044

non-stoichiometric, 1163 physical properties of, 1044, 1156 thermodynamic properties of, 1296, 1301,

1312, 1343 see also Californium, dioxide; ... ,

sesquioxide oxyhalides, 1043, 1045, 1443 oxysulfate, 1043, 1048 oxysulfide, 1043, 1048, 1438 phospho-organic complexes, 1056 phosphotungstate complexes, 1050, 1052,

1059--60 pnictides

crystal structure data for, 1043 preparation methods for, 1047-8

production capability for, 1028, 1126 production methods for, 1025-8, 1027,

1125, 1126, 1663 pyrozolin-complexes, 1056 radiative relaxation for, 1257 reduction potentials of, 1038, 1052, 1143,

1286 se1enides, 1048 separation/purification methods, 1029 -33

fused salt-molten metal process, 1033 ion-exchange procedures, 1030-1, 1032-

3, 1032 ultra-purification process, 1033

sesquioxide, 1044-5 crystal modifications, 1044 crystal structure data for, 1037, 1042,

1044, 1156, 1422 physical properties of, 1044, 1156 thermodynamic properties of, 1295, 1296,

1299, 1343 solid-state absorption spectra for, 1050,

1051 sulfato complexes, 1054, 1056

stability of, 1503 thermodynamic data for, 1058 thermodynamics for formation of, 1503

sulfides, 1048 crystal structure data for, 1437

tartrate complexes, 1055 tellurides, 1048 thenoyltrifiuoroacetonato complexes, 1055,

1056,1057 thiocyanato complexes, 1054, 1056, 1514 trifiuoroacetonato complexes, 1055, 1056,

1057 x-ray emission spectra for, 1034-5 x-ray photoelectron spectroscopic studies

for, 1035 Calutrons, 177, 180,325 Cancer, treatment of by 2s2Cf , 1192 Cancer incidence, effect of actinide elements,

1185

Subject Index

Carbides, structural chemistry of, 1432--4, 1433 see also under individual elements (by name)

Carbonates, structural chemistry of, 1449-50 see also under individual elements (by name)

Carbonato complexes, formation and stability of, 1502, 1504

Carbonyls, 1169, 1589 Carboxylates, structural chemistry of, 1454-5

see also under individual elements (by name), acetates; ... , formates; ... , oxalates

Carboxylato complexes, formation and stability of, 1505-9

Carnotite (mineral) chemical composition of, 190, 191 plutonium content of, 504, 505 uranium content of, 504

Casimir operators, 1244 Catechoy1amido chelates, 775, 779, 1513 Chalcogen complexes, formation and stability

of,1501-6 Chalcogenides, structural chemistry of, 1435-

6, 1437--8 see also under individual elements (by name)

Chelate complexes formation and stability of, 1509-13 structural chemistry of, 1455-8

Chelating ligands, 1147 Chemical identification, heavy elements,

1630-1, 1633 Chloro complexes

stability of, 1499 structural chemistry of, 1446-7 see also under individual elements (by name)

Chromatographic methods, 450-1, 1133 CODATA thermodynamic compilations, 1347 Coffinite (mineral), 190, 191, 339 Cold fusion reactions, 1630, 1644 Complex halides

magnetic data for, 1365 thermodynamic properties of, 1314, 1347 see also under individual elements (by name)

Complex ions: see under individual elements (by name)

Complex oxides thermodynamic properties of, 1298 -1300,

1302, 1303, 1304 see also under individual elements (by name)

Complexes formation in aqueous solution, 1146-7,

1497-1516 with carboxylate ligands, 1506-9 with chelating agents, 1509-13 condition necessary for, 1497 with halide ions, 1498-1501 with nitrogen-coordinating ligands, 1514 with oxygen-coordinating ligands, 1501-6 thermodynamics of, 1501, 1509,1510,

1515, 1517

hard/soft acceptors/donors for, 1497-8 stability of, 1497-8 structural chemistry of, 1424-6, 1446-7 see also under individual elements (by name)

Condensed-phase spectra, 1238-9 and free-ion emission spectra, 1251-2 interpretation for trivalent actinide ions,

1240-57 Configuration interaction (CI), 1218-19, 1236 Controlled potential coulometry, neptunium,

470,487 Cotter (nuclear fuel reprocessing) concentrate,

114 enrichment of, 115 typical analysis of, 113

Coupling schemes, electron interaction, 1216 Critical masses

americium, 899 plutonium, 502

Crown ether complexes, 1457-8 Crystal field Hamiltonian, 1245-51 Crystal field splittings, 1363--4, 1364, 1365 Crystal spectra, 1196-7, 1245-53, 1260, 1273 Crystal structure

compounds, 1154, 1155-60, 1164, 1417-63 metals, 1149-51, 1150, 1389, 1391

melting point affected by, 1390, 1392 pressure effects on, 603, 900-01, 999,

1037-8, 1152-3, 1390 Curie-Weiss law, 1365-6, 1406 Curium

absorption spectra for, 966-8, 966, 967, 1239, 1256, 1265

acetato complexes, 980, 1507, 1510 acetylacetonato complexes, 977 alloys, 972 aluminate, 972, 976 antimonide, 972, 975-6, 1438 applications for, 964 arsenide, 972, 975-6, 1438 atomic properties of, 966-8 biological behavior of, 1179, 1180, 1183 bromide, 972, 973

crystal structure data for, 972, 1158, 1441 physical properties of, 1158 thermodynamic properties of, 1310, 1342

carbonate, 976 carbonato complex, 976 chalcogenides, 972, 975 chlorides, 972, 973


1342 chloro complexes, 980, 1499 citrato complex, 980 comparison with lanthanides, 966, 967, 969,

970 complex halides, 972, 973

Subject Index

Curium (Contd.) magnetic data for, 1365

complex sulfates, 976 cyclopentadienyl complexes, 977, 1167, 1553 1,3-diketone complexes, 982 dioxide, 972, 974

crystal structure data for, 972, 1156 magnetic properties of, 1379 physical properties of, 1156 thermodynamic properties of, 1162, 1301,

1312, 1341 discovery of, 5, 6, 962 electron configurations of, 966, 1135, 1203,

1204, 1227-8 electron energy level scheme for divalent

ion, 1261 energy level parameters for, 1246 ethylenediaminetetraacetato complexes, 980,

1513 fluorides, 971, 972, 973



1342 fluoro complexes, 978, 980, 1498 free-ion energy level structure for, 1249 g1ycinato complexes, 980, 982 g1ycolato complexes, 1507 halides, 971, 972, 973--4

crystal structure data for, 972, 1157, 1158,1159,1440-1


1310,1311,1312,1342-3 handling techniques for, 964 Hartree-Fock calculations for, 1221, 1223 hydration enthalpy of, 1293 hydrides, 1155, 1432 hydroxide, 976

thermodynamic properties of, 1289, 1341 hydroxyisobutyrato complex, 980 8-hydroxyquinolinato complexes, 982 iodide, 972, 973

crystal structure data for, 972, 1158, 1441 physical properties of, 1158 thermodynamic properties of, 1311

ion-exchange separation of, 1089, 1528, 1529

ionic radii of, 1165, 1284, 1289, 1448 ionization energies for, 1293 ions in solution, 978-82

absorption spectra of, 966-7, 966, 967, 979, 981, 1239, 1256, 1265

with inorganic ligands, 978-9, 980, 981 with organic ligands, 980-1, 981-2 oxidation states of, 970, 1139 oxidation-reduction reactions, 978-9 solvent extraction data for, 1520

stability of, 979, 980-1, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284, 1312, 1341 isotopes, 963--4, 963, 1129

decay properties of, 963,1661,1671-2 production methods for, 963, 964, 965,

1125,1125,1126,1661 lactato complex, 980 magnetic data for, 1049, 1365, 1379, 1406,

1406 marine organisms affected by, 1175 metal,968-70

chemical reactions of, 970 crystal structure data for, 968, 972, 1150,

1391 magnetic properties of, 969 physical properties of, 968-9, 1150, 1391 preparation of, 969-70, 1401 single crystals, 140 I thermodynamic properties of, 969, 1150,

1280, 1281, 1341, 1396 vapor-pressure relationships for, 969

metallic radii of, 1150, 1450 niobate, 976 nitrato complex, 980 nitride, 972, 975-6, 1438 nitrilotriacetato complex, 981 nitrito complex, 980 nuclear spins and moments of, 1648 organometallic compounds, 977 oxalate, 972, 974, 976 oxalato complexes, 980, 1507 oxidation states of, 970. 1139, 1139 oxidation-reduction reactions, 978-9 oxides, 972, 974


non-stoichiometric, 1163 physical properties of, 1155, 1156 thermodynamic properties of, 1162, 1296,

1301,1341 see also Curium, dioxide; ... , sesquioxide

oxyantimonide, 972, 1438 oxybismuthide, 972, 1438 oxychloride, 972, 973--4


oxysulfate, 972, 974-5 oxysulfide, 972, 975, 1438 oxytelluride, 972, 975, 1438 phosphates, 976 phosphide, 972, 975-6, 1438 organophosphorus complex, 981 pnictides, 972, 975-6 production capacity for, 1126 production methods for, 963, 964, 965,

1125, 1125, 1126, 1661 radiative relaxation for, 1257 radioactive decay of, 1172

Subject Index

reduction potentials of, 979, 1143, 1286, 1287

selenides, 972, 975 crystal structure data for, 972, 1437, 1438

self-irradiation effects of, 970, 971 separation/purification methods for, 964-6 sesquioxide, 972, 974


1296, 1299, 1341 solid-state spectra for, 967-8 solution chemistry of, 978-82 sulfato complexes, 980, 1503 sulfides, 972, 975, 1437, 1438 tantalate, 976 as target material for superheavy element

synthesis, 1644-5 tellurides, 972, 975, 1437, 1438 thenoyltrifluoroacetone complexes, 981 thiocyanato complexes, 979, 980, 1514 trimetaphosphato complexes, 980 weighable amount first isolated, 6, 962

Curium-242 applications for, 889-90 production of, 890

Cyc1o-octatetraene complexes, 1168, 1462, 1573-80

chemical reactivity of, 1576-7 Cyc10pentadienyl complexes, 1164, 1165-7,

1167, 1550-63 bis(cyc1opentadienyl) chloro compounds,

1167, 1460, 1553 bis(cyc1opentadienyl) derivatives, 1560-1 preparation methods for, 1166, 1550-63 structural chemistry of, 1458-9, 1551, 1554,

1555, 1556, 1561 tetrakis(cyclopentadienyl) compounds, 1167,

1553-5 tris(cyclopentadienyl) compounds, 1167,

1461, 1550-3 tris(cyc1opentadienyl) derivatives, 1167,

1458-60, 1461-2, 1555-60 see also under individual elements (by name)

Cyc10pentadienyl hydrocarbyl complexes, 1592-8

Czerny -Turner spectrograph, 213

Dapex process, 1521 Darken-Gurry solubility prediction (alloys),

632-3, 633, 634 Darmstadt Laboratory (Germany), 10, 1110 De Haas-van Alphen effect, 232, 295 Decay modes

definition of, 1649-50, 1674 (footnote) heavy elements, 1630 (listed), 1653-74 see also individual elements (by name),

isotopes ...

Decay series (4n+ I), 19,22,43 (4n+2),171 (4n + 3), 14, 18, 42, 107, 171

Diethylenetriaminepentaacetato complexes, 1513

Diffusion separation methods: see Gas diffusion .. .

Dioxoneptunium ... : see Neptunyl ... Dioxouranium ... : see Uranyl ... Discovery criteria/guidelines, 1105, 1633 Divalent ions

in aqueous solution, 1481 hydrolytic behavior of, 1483 spectra of, 1260-2

Dubna Laboratory (USSR), 7, 10, 1104, 1108, 1632

EGT (external gelation of thorium) process, 270,270

EGU (external gelation of uranium) process, 270,271

Einstein (fluorescence) expression, 1255 Einsteinium

absorption spectral data for, 1078, 1079, 1080, 1239

aminocarboxylato complex, 1080 atomic properties of, 1075, 1076 bromides

absorption spectra for, 1079 crystal structure data for, 1078, 1158,

1441 physical properties of, 1158

chlorides absorption spectra for, 1079 crystal structure data for, 1078, 1157,

1440 physical properties of, 1157 thermodynamic properties of, 1305, 1309,

1344 chloro complex, 1080 citrato complex, 1080 complexes, stability constants of, 1080 discovery of, 5,6, 1071, 1127 electron configurations of, 1075, 1076, 1135,


ion, 1261 energy level parameters for, 1246 ethylenediaminetetraacetato complex, lOBO fluorides, 1077, 1078

absorption spectral bands for, 1078 thermodynamic properties of, 1306, 1312,

1344 free-ion energy level structure for, 1249 halides, 1077, 1078, 1079

absorption spectra for, 1079 crystal structure data for, 1078, 1157,

1158, 1440-1

Subject Index

Einsteinium (Contd.) physical properties of, 1157, 1158 thermodynamic properties of, 1305, 1306,

1309, 1312, 1344 Hartree-Fock calculations for, 1221 hydration enthalpy for, 1293 hydroxide, activity products of, 1289 hydroxo complex, lOBO hydroxyisobutyrato complex, lOBO iodides, 1078, 1079

absorption spectra for, 1078, 1079 crystal structure data for, 1078, 1158 physical properties of, 1158 thermodynamic properties of, 1311

ion-exchange separation of, 1074, IOB9, 1529

ionic radii of, 1079, 1080-1, 1165, 1284, 1289, 1448

ionization energies of, 1076, 1293 ions in solution, 1079-81

absorption spectra of, 1239 divalent ion, 1081 stability of, 1080, 1080, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284, 1312, 1344 trivalent ion, 1079-81

isotopes decay properties of, 1072, 1129-30, 1664,

1672-3 production methods for, 1072, 1073,

1125, 1126, 1127, 1664 limitations on study of, 1072-3 magnetic data for, 1049, 1382 malato complex, lOBO metal, 1075-7


divalencyof, 1076 physical properties of, 1076, 1150, 1391 preparation of, 1401 thermal conductivity of, 1077 thermodynamic properties of, 1076-7,

1150,1280, 1281, 1344 metallic radius of, 1150 nuclear spins and moments of, 1648 oxidation states of, 1080, 1139 oxides

crystal structure data for, 1078, 1156 physical properties of, 1156 thermodynamic properties of, 1296, 1301,

1312, 1344 oxyhalides, 1078, 1443 production methods fdr, 1072, 1073, 1125,

1126, 1127, 1664 radiative relaxation for, 1257 reduction potentials of, 1081, 1103, 1143,

1286 separation/purification methods, 1073-5

separation factors for, 1075

sulfato complex, lOBO as target material for superheavy element

synthesis, 1644 tartrato complex, lOBO thiocyanato complex, lOBO

Eisenstein-Pryce model, best-fit parameters for, 1362, 1370, 1371

Eka-actinium: see Element 121 Eka-astatine: see Element 117 Eka-bismuth: see Element liS Eka-gold: see Element III Eka-hafnium: see Element 104 Eka-iridium: see Element 109 Eka-lead: see Element 114 Eka-mercury: see Element 112 Eka-osmium: see Element 108 Eka-platinium: see Element 110 Eka-polonium: see Element 116 Eka-radon: see Element 118 Eka-rhenium: see Element 107 Eka-tantalum: see Element lOS Eka-thallium: see Element 113 Eka-tungsten: see Element 106 Electrode potentials: see Reduction potentials Electron configurations, 1133-7, 1201-6

experimental techniques for, 1134 heavy elements, 1631-2 (listed), 1135 metals, 1151-3, 1390, 1392 relative energies of, 1136,1136, 1201-6,

1203, 1204, 1236-9, 1237 summary of, 1223-31 superheavy elements, 1633-5 see also Under individual elements (by 1IQme)

Electron nuclear double resonance (ENDOR) measurements, 1369

Electron paramagnetic resonance (EPR) measurements, 1362--4, 1368-9

Electron radial distribution functions, 1202, 1205, 1207, 1243

Electron radial integrals, 1210-11, 1210 Electron spin-orbit coupling, in magnetic

studies, 1364, 1369-70 from spectroscopy, 1241-52

Electron stability, Sf-electrons, 1388, 1393 Electron structures: see Electron

configurations Electrostatic interactions

energy calculations for, 1208-11 in magnetic studies, 1364 open-shell electrons, 1207 -14

Element 104 chemical properties predicted for, 1105,

1111, 1637 discovery of, 7, 1103, 1104 electron configurations of, 11 OS, 1111, 1135 ion-exchange behavior of, 1105-6 ionic radius of, 1111, 1637 ionization energy of, 1111, 1637

Subject Index

isotopes decay properties of, 1104, 1668, 1674 production methods for, 1I03--4, ll04,

1668 naming of, 11 04, 11 05 oxidation states of, 1I05, llll, 1637 reduction potential of, 1111, 1637

Element lOS chemical properties predicted for, 1108,

llll, 1637 chloride, volatility of, I 107 discovery of, 7, 1I06, 1I07 electronic configuration of, 1108, IIII ionic radius of, llll, 1637 ionization energy of, 1111, 1637 isotopes

decay properties of, 1109, 1668, 1674 production methods for, 1I06-7, 1l09,

1668 naming of, 1107 oxidation states of, 1I08, llll, 1637 reduction potential of, 1111, 1637

Element 106 chemical properties predicted for, 1109-10,

llll, 1637 discovery of, 7, 1108 electronic configuration of, 1I09, llll ionic radius of, llll, 1637 ionization energy of, llll, 1637 isotopes

decay properties of, 1109, 1668, 1674 production methods for, 1108-9, 1109,

1668 oxidation states of, 1110, llll, 1637 reduction potential of, 1111, 1637

Element 107 chemical properties predicted for, Illl,

1112, 1637 discovery of, 7, II 10 electronic configuration of, llll, 1112 ionic radius of, llll, 1637 ionization energy of, llll, 1637 isotopes

decay properties of, 1109, 1668, 1674 production methods for, 1109, 1110, 1668

oxidation states of, III I, 11I2, 1637 reduction potential of, llll, 1637

Element 108 chemical properties predicted for, 11 11 ,

1112, 1637 discovery of, 7, 1112 electronic configuration of, 1111, 1112 ionic radius of, ll11, 1637 ionization energy of, 1111, 1637 oxidation states of, 11 11, 1I12, 1637 reduction potential of, 1111, 1637

Element 109 chemical properties predicted for, 1111,

1113, 1635, 1637

discovery of, 7, 1I12 electronic configuration of, 1111, 1113 ionic radius of, 11 11, 1637 ionization energy of, 1111, 1637 isotopes

decay properties of, 1109, 1668, 1674 half-life value listed for, 1109, 1668, 1674 production method for, 1109, 1I12-13,

1668 oxidation states of, III I, lI13, 1635, 1637 reduction potential of, 1111, 1637

Element 110, 1635, 1637 Element 111, 1635, 1637 Element 112, 1635-6, 1637 Element 113, 1636, 1637, 1638, 1639, 1641 Element 114, 1636, 1637, 1639, 1639, 1641 Element 115

chemical properties predicted for, 1637, 1641-2

compared with antimony and bismuth, 1616, 1638, 1640

Element 116, 1637, 1642 Element 117, 1637, 1642 Element 118, 1637, 1642 Element 119, 1637, 1642 Element 120, 1637 Element 121, 1637, 1642 Emission spectra, 1134-5

term analysis of, 212-13, 578-90, 1198-9 see also Atomic spectroscopy; and under in

dividual elements (by name) Engel-Brewer (alloy) theory, 633-5 Entropies

compounds (listed), 1315-46 jons in solution, 1280, 1282--3, 1284 metals, 1280, 1281, 1397

Environmental aspects, 1169-78 man-made synthesis, 1171-3 marine transfer mechanisms, 1173-5 natural sources, 1170-1 nuclear waste disposal, 1176-8 sorption/mobility processes, 1175-6

Ethereal sludge (nuclear fuel reprocessing), 104,114

enrichment of, 116-18, ll8 typical analysis of, 113

Ethylenediaminetetraacetato complexes, 1147, 1512-13

stability of, 1513 see also under individual elements (by name)

Excer (UF 4 production) process, 304

Feces, actinide elements in, 1179-80 Fergusonite (mineral)

chemical composition of, 190 plutonium content of, 504, 505 uranium content of, 504

Fermi energy, metals, 1388

Subject Index

Fermi level electron related properties, metals, 1392-3, 1394

Fermium atomic properties of, 1088-9, 1090 chlorides, thermodynamic properties of,

1305, 1309, 1345 complexes, 1091 discovery of, 5, 6, 1086, 1127 electron binding energies for, 1089, 1090 electron configurations of, 1088, 1103, 1135,

1203, 1204, 1229 free-ion energy level structure for, 1249 Hartree-Fock calculations for, 1221 hydration enthalpy for, 1293 ion-exchange separation of, 1088, 1089,

1528 ionic radii of, 1091, 1103, 1284 ionization energy of, 1103, 1293 ions in solution, 1091-2

complexes, 1091 coordination number of, 1091 stability of, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284,1345 isotopes, 8, 1086-7, 1087

decay properties of, 1087, 1665, 1673 production methods for, 1086-7, 1087,

1088, 1125, 1127, 1665 metal

predictions for, 1090 thermodynamic properties of, 1280, 1281,

1345 metallic radius for, 1090 organic complexes, 1091 oxidation states of, 1103, 1139 production methods for, 1086-7, 1088,

1097, 1125, 1126, 1127, 1665 reduction potentials of, 1091-2, 1103, 1143,

1287 separation/purification of, 1088, 1089 sesquioxide, thermodynamic properties of,

1296, 1345 solution chemistry of, 1091-2 x-ray energies for, 1089, 1090

Fission isomers, 1650 Fission-product elements, 506, 507

distribution coefficients listed for various solvents, 520

half-life values listed for, 507 radioactivity of, 507, 508

Fluorescence lifetimes, 1255, 1257 Fluoro complexes

stability of, 1498 structural chemistry of, 1444---6 thermodynamics of formation of, 1501

Fluorox (UF 6 production) process, 311 Food chain, actinide elements in, 1175 Formation enthalpies

halides, 1305--6, 1309-12

ions in solutions, 1280, 1281, 1282, 1312 metals, 1280; see also Sublimation

enthalpies oxides, 1296, 1297,1301,1302,1303,1312

Fourier-transform spectroscopy, 579, 579, 1198

Free-ion emission spectra and condensed-phase spectra, 1251-2 see also Emission spectra

Free-ion models, 1240-1 Free-ion states, 1238-9

media effects on, 1239

Gamma-particle spectroscopy, 1651-2 Gas centrifuge separation processes, 181-2

efficiency of, 181-2 plants listed, 182

Gas diffusion process, 174-7 plant design difficulties, 176 plants in USA, 174, 176-7,178-9,180 porous barrier characteristics for, 176, 177 separation efficiency for, 175---6

Gas jet (transeinsteinium element separation) method, 1093, 1097, 1101

Gaseous atoms/ions thermodynamic properties of, 1292 see also Free-ion spectra; Vapor-phase

spectra Goldanskii-Karyagin effect, 491

Hahnium: see Element 105 Halex process, 541 Half-life values

(listed), 1129, 1653-74 see also under individual elements (by

name), isotopes, half-life values ... Half-sandwich complexes, 83, 1580 Halides

magnetic properties of, 1367, 1376 structural chemistry of, 1436, 1439, 1440-1,

1442-3 thermodynamic properties of, 1300, 1303-

14, 1347 see also under individual elements (by

name), bromides; ... , chlorides; ... , fluorides; ... , iodides

Halo complexes formation of, 1498-1501 stability of, 1498-9, 1500 structural chemistry of, 1446-7 see also under individual elements (by name)

Handling techniques, 9-10, 1128, 1130-1, 1399

curium, 964 plutonium and compounds, 577, 659, 661,

740-1 Hanford (USA)

neptunium production process, 447-8, 448

Subject Index

plutonium separation plant, 513,526, 542, 543

Hartree-Fock( -Slater) calculations, 1202, 1220-3, 1221, 1640

Hazards, 10,661, 1128 Heat capacities

compounds (listed), 1315-46 ions in solution, 1290-1

Heavy elements, chemical properties predicted for, 1630-1, 1637

Heavy fermions, 1409-13 Heavy-ion bombardment methods, 1127,

1629, 1630 see also Lawrencium, ... ; Mendelevium,

... ; Nobelium, ... ; Element 104 ... 109, production methods

Helicon process, 182 Heptavalent ions

in aqueous solution, 1482-3 spectra of, 1273

Hermex process, 234 Hexavalent ions

in aqueous solution, 1482 hydrolytic behavior of, 1490-5 spectra of, 1272-3 see also Actinyl ions; Americyl ions; ...

Hexone process, 184,517,519, 521-5 see also Redox process

High-flux nuclear reactors,S, 8, 503, 990, 1028, 1125, 1652

Homoleptic compounds, 1589-92 Hund's rule, 1199, 1200 'Hutch' thermonuclear explosion, 1087 Hydration enthalpies (listed), 1293 Hydrides

structural chemistry of, 1426-7, 1432 see also under individual elements (by name)

Hydrolytic reactions, 1141, 1143, 1145-6, 1483-95

kinetics of, 1531-2 thermodynamics of, 1495-7 see also under individual elements (by name)

Hydrosphere actinide elements in, 1173-5 uranium content of, 195-6, 1170

Hydroxides activity products for, 1288-9, 1289 see also under individual elements (by name)

Hydroxo complexes, 1143, 1145, 1483-97 8-Hydroxyquinolinato complexes, 777, 778,

816,817, 1512, extraction data for, 1519 see also under individual elements (by name)

Hyperfine structure, 1230-1 widths listed for, 1224-9

Identification techniques, 10, 1630-1, 1633 Incandescent gas mantle production, 41 Indenyl compounds, 1167, 1459, 1459, 1563-5

Ingestion mechanisms, 1182-3 Interim 23 process, 184 Intermetallic compounds, 1398-9

band magnetism of, 1407-8,1407 close-packed layers in, 1398, /398 Laves phases 'in, 1399 magnetic susceptibility of, 1406, /406 specific heat electronic term coefficients for,

1407, 1407, 1409, 14JJ, 1413 thermodynamic properties of, 1282 see also under individual elements (by name)

Ion-exchange chromatography, 1131-2, JJ 32 Ion-exchange methods (for separation/

purification), 1131-2, 1526-31 anion exchange, 1530-1 cation exchange, 1526-9 criticality control for, 557, 559,561 distribution coefficients listed for, 558, 895 procedures listed for, 551 see also under individual elements (by

name), separation/purification Ion-exchange resins, radiation effects on,

1528, 1531 Ion types, 1140, JJ40 Ionic radii, 1164, 1447-8

(listed), JJ65, 1284, 1289, 1448 see also under individual elements (by name)

Ionization energies, 1231, 1292 calculation of, 1292 (listed), 1293

Ions in solution acid-base reactions, kinetics of, 1531-2 acidic properties of, 1483-95 aqueous solutions, 1480-3 color of, JJ40 complex formation by, 1146-7, 1497-1516 entropies for, 1280, 1282-3, 1284 formation enthalpies for, 1280, 1281, 1282 free energies of formation for, 1280, 1285-

90 in acid solution, 1285, 1286-7, 1288 in basic solution, 1287, 1288-90

high-temperature thermodynamic properties of,129O-1

oxidation states of, 1137, 1139-40, JJ39 oxidation-reduction reactions, kinetics of,

1532-9 reaction kinetics for, 474-6, 1531-9 reduction potentials for, 1142-3, 1286-7 stability of (listed), 1144, 1288 thermodynamic properties of, 1280, 1281,


Isotope shifts, 1199 -120 I (listed), 1200, 1201, 1224-9

Isotopes decay modes of, 1653-74 half-life values listed for, 1129, 1653-74 nuclear properties of, 1653-74

Subject Index

Isotopes (Contd.) radiation energies listed for, 1653--68 see also under individual elements (by name)

Isotopic exchange studies, 476, 477, 478-81

ludd-Ofelt theory, 1254

Kramers degeneracy, 1363 Kurchatovium: see Element 104

Lanthanide elements, actinides compared with, 9

condensed-phase versus free-ion spectra, 1251, 1252

crystal structures, 1389 divalency, 1086, 1305 divalent ions in solution, 1481 electronic configurations, 1135 f-electron shells, 1149 hydroxide activity constants, 1289 ion-exchange behavior, 1088, 1089, 1132,

1527, 1528, 1529, 1530 ionic radii, 1165, 1289 magnetic moments, 1049 metal sublimation enthalpies, 1281 pnictide lattice constants, 62, 64 reduction potentials, 1103 solid-state behavior, 62, 64 solvent extraction behavior, 1520, 1521 thenoyltrifluoroacetone extraction, 24 thermodynamic properties

of halides, 1305, 1306, 1307, 1307, 1309-11

of ions in solution, 1281 of oxides, 1295, 1296, 1300, 1301

transamericium elements, 966 Lanthanide shift rule, 912 Lanthanum, similarity of actinium to, 14 Laser effects, 977, 1050, 1253 Laser separation process, 173-4, 174, 175 Latimer diagrams, 1142-3, 1285, 1286-7 Laves-phase intermetallics, 490, 1399 Lawrencium

atomic properties of, llOI discovery of, 7, 10, 1099 electronic configurations of, llOI, 1103,

1135, 1631 hydration enthalpy for, 1293 ionic radii of, ll02, 1103, 1284 ionization energies for, 1293 ions in solution, llOI-2, 1103

stability of, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284,1346 isotopes, 1100

decay properties of, 1100, 1667, 1674 production methods for, 1099, 1100,

1100, 1125, ll27, 1667

metal, thermodynamic properties of, 1280, 1281, 1346

metallic radius of, 1102 oxidation states of, 1086, 1101, 1103, 1139 production methods for, 1099, 1100, 1100,

1125, 1127, 1667 reduction potentials of, 1102, 1103, 1143,

1287 separation/purification of, 1100-1 sesquioxide, thermodynamic properties of,

1296,1346 solution chemistry of, II 0 1-2, 1103 trichloride, thermodynamic properties of,

1309,1346 x-ray spectra of, 1101, 1101

Lea-Leask-Wolf method, 1364, 1368 Ligand field splittings, 1363-4, 1364, 1365 Liquid-liquid chromatography, Np-Pu separ-

ation,450-1 Liquid-liquid extraction techniques, 1132-3

see also Solvent extraction methods Liquid thermal diffusion process, 181 Liver, uptake of actinide elements in, 1179,

1180-1 Long-lived isotopes, ll28-30

(listed), 1129 Luminescence spectra, 585, 968, 995, 1253

see also under individual elements (by name) Lung tissues

clearance of actinide elements from, 1183 ingestation of plutonium into, ll82-3

Lymph fluid, actinide elements in, ll80

Magnetic properties, 1361-82 5fo ions, 1367 5[1 ions, 1367-72 5f2 ions, 1372-5 5£3 ions, 1375-7 5f4 ions, 1377 5fs ions, 1378 5f6 ions, 1378-9 5f7 ions, 1379 5f8 ions, 1380 5f9 ions, 1382 5f 11 ions, 1382 metals, 1405-13

Marine organisms, availability of trans-uranium elements to, 1174-5

Marvin radial integrals, 1245 Mass spectroscopy applications, ll90, 1191 Medical applications, 1190-2 Melting points: see individual compounds/

elements by name Mendelevium

atomic properties of, 1094 chlorides, thermodynamic properties of,

1305, 1309, 1345 discovery of, 7, 10, 1092

Subject Index

electron configurations of, 1094, 1103, 1135, 1204

free-ion energy level structure for, 1249 hydrated radius of, 1095 hydration enthalpy for, 1293 ion-exchange separation of, 1089, 1094,

1528 ionic radii of, 1095, 1103, 1284 ionization energy of, 1103, 1293 ions in solution, 1094-5

coordination number of, 1095 stability of, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284, 1345 isotopes, 1092, 1093

decay properties of, 1093, 1666, 1673 production methods for, 1092, 1093,

1125, 1127, 1666 metal, thermodynamic properties of, 1280,

1281,1345 metallic radius of, 1095 oxidation states of, 1103, 1139, 1139 oxidation -reduction reactions of, 1095 production methods for, 1092, 1093, 1125,

1127,1666 reduction potentials of, 1095, 1103, 1143,

1287 separation/purification methods, 1092--4

gas jet collection technique, 1093 ion-exchange processes, 1094 recoil separation technique, 1092-3

separation/purification of, 1092--4 sesquioxide, thermodynamic properties of,

1296,1345 solution chemistry of, 1094-5

Mesothorium II, 16, 19 Metal-metal bonding, 1623--4 Metallic radius, 1449

(listed), 1150, 1450 see also under individual elements (by name)

Metallic state, 1148-53, 1388-1413 Metals

alloying relationships for, 1397-9 atomic structure of, 1389-90 band magnetism of, 1407-8 crystal modifications, 1150, 1151, 1391,

1402-3 crystal structure of, 1149-51, 1150, 1389,

1391 elastic properties of, 1404 electrical properties of, 1394 electronic structures of, 1151-3, 1390,

1392 entropies of, 1280, 1281, 1397 Fermi level electron related properties for,

1392-3, 1394 local-moment magnetism of, 1406-7 magnetic properties of, 1394, 1405-13

f-electron effects on, 1394-5 mechanical properties of, 1403-5 melting points of, 1390

(listed), 1150, 1391 relationships with crystal structure,

1392 non-magnetic behavior of, 1409 plastic properties of, 1405 Poisson's ratio for, 229, 1405 polymorphic transformations of, 1151,

1402-3 preparation of, 1148, 1399-1401 pressure effects on, 1152-3, 1390 purification of, 1148, 1400-1 shear moduli of, 1405 single crystals, 140 I solid-solution alloys, 1397-8 specific heat electronic term coefficients for,

1394,1409 spin fluctuations in, 1408-9 Stoner criterion for band magnetism in,

1407,1409 sublimation enthalpies of, 1150, 1280, 1281,

1395 superconductivity of, 1153, 1409-13 tensile strengths of, 1404 thermodynamic properties of, 1150, 1279-

81,1280,1281, 1395, 1396, 1397 vaporization enthalpies of, 1150, 1280,

1281, 1395 yield strengths of, 1404 see also under individual elements (by

name); and also Intermetallic compounds

Metastable states, (defined), 1650 'Mike' thermonuclear explosion, 5, 1071,

1086, 1127 Molecular laser isotope separation (MLIS)

process, 173--4, 175 Monazite (mineral), 45

actinium in, 22 plutonium content of, 504 processing of, 46, 47, 48, 49 stability of, 46 typical analyses of, 45 uranium content of, 45, 504

Mossbauer spectroscopy americium, 899 neptunium, 488-91

electric field gradient (EFG) interactions, 488,489-90

hyperfine interactions detected by, 488 isomer shift hyperfine interactions, 488-9 magnetic hyperfine interactions, 488, 490 structural information from, 490-1

plutonium, 581-2 uranium, 216-17 see also under individual elements (by name)

Subject Index

Natural origins, actinide elements, 1170-1 Natural sources, 1122-3

see also under individual elements (by name) Neptunates, 458-9

magnetic properties of, 1370,1371, 1376 solution properties of, 465 thermodynamic properties of, 1302, 1304,

1336 Neptunium

absorption spectra of ions in solutions, 465, 467-9,46~ 468,485-7

acetate complexes, 464, 484 acetylacetonato complexes, 1455, 1511 aluminum compounds, 455 americium reduced by, 924, 925 analytical methods for, 485-91

colorimetry, 487 controlled potential coulometry, 487 Mossbauer spectroscopy, 488-91 radiometric methods, 485 spectrophotometric methods, 485-7 volumetric methods, 488

antimonides, 1437 arsenide, 1437 beryllide, 455, 1395, 1413 biological behavior of, 1178, 1184 bismuthide, 1437 borides, 455, 1433 borohydride, 463 bromides, 462,463, 489-90

crystal structure data for, 463, 1157, 1159, 1441

magnetic properties of, 1376 physical properties of, 1157, 1159 thermodynamic properties of, 1310, 1312,

1335 cadmium compounds, 455 carbides, 459


cation-cation complexes, 484 chalcogenides, 460

crystal structure data for, 1437, 1438 magnetic properties of, 1395

chlorides, 462, 463, 489-90 crystal structure data for, 463, 1157,

1159,1440 magnetic properties of, 1367, 1375-6,

1376 physical properties of, 1157, 1159 thermodynamic properties of, 1309, 1312,

1335 chloro complexes, 480, 481, 482, 483-4,

484,1499 complex halides

crystal structure data for, 464, 1444-5, 1445, 1448

electron energy level structures for, 1269, 1270, 1271

magnetic data for, 1365, 1376, 1377 thermodynamic properties of, 1336

complex ions in solution, 481-4 complex oxides, 457-9, 458, 490

magnetic properties of, 1370, 1371, 1376 thermodynamic properties of, 1302, 1304,

1336 compounds, 455-64

compared with uranium compounds, 444 see also Neptunyl ...

cyclo-octatetraene complexes, 1462, 1573, 1579

cyclopentadienyl compounds, 1167, 1552-3, 1554-5, 1559-60, 1563

decay series (4n+ 1),22 dioxide

crystal structure data for, 457, 1156 magnetic properties of, 1377 physical properties of, 1156 thermodynamic properties of, 1162, 1301,

1312, 1335 discovery of, 4, 6, 443-4 electron configurations for, 1135, 1203,

1204,1226 electron energy level scheme for divalent

ion, 1261 energy level parameters for, 1246, 1268-9 ethylenediaminetetraacetato complexes,

stability of, 1513 fluorides, 447, 451-2, 460-2, 736

crystal structure data for, 463, 1157, 1159, 1160, 1440


magnetic properties of, 1368-9 physical properties of, 461, 1157, 1159,

1160 preparation and properties of, 460-2 in separation processes, 447, 451-2 thermodynamic properties of, 1306, 1312,

1335 fluoro complexes, 484

stability of, 1498 free-ion energy level structure for, 1249 halides, 460-3

crystal structure data for, 463, 1157, 1158, 1159, 1160, 1440-1

magnetic properties of, 1376 physical properties of, 1157, 1158, 1159,


1309, 1312, 1335 Hartree-Fock calculations for, 1221, 1223 hydration enthalpy for, 1293 hydrides, 455-6

crystal structure data for, 455, 1155, 1432 magnetic properties of, 1377 physical properties of, 1155 thermodynamic properties of, 1335

Subject Index

hydrolytic behavior of, 1145 hydroxide

thermodynamic properties of, 1289, 1335 intermetallic compounds, 453, 455, 490

crystal structure data for, 455 magnetic properties (listed) for, 1394,

1395,1413 iodides, 462

crystal structure data for, 463, 1158, 1441 magnetic properties of, 1376 physical properties of, 1158 thermodynamic properties of, 1311, 1335

ionic radii of, 1165, 1284, 1289, 1448 ionization energies for, 1293 ions in solution, 465-84

absorption spectra, 465, 467-9, 467, 469, 485-6,486,1239,1263,1265

complex ions, 481-4 disproportionation reactions of, 471-2,

472, 476, 478-9 hydrolysis of, 1488, 1489 isotopic exchange studies, 476, 477, 478-

81 kinetic studies, 474-6 oxidation-reduction kinetics for, 1533,

1536 oxidation-reduction reactions, 471, 472-

81,473-4 oxidation states in, 465, 466, 1139 preparation of, 466 solvent extraction data for, 1519, 1522,

1524, 1525, 1526 stability of, 465, 471-2,1144,1288, 1482 thermodynamic properties of, 1280, 1281,

1284, 1312, 1334 isotopes, 444-5

decay properties of, 445, 1129, 1172, 1658, 1670-1

production methods for, 444-5, 445, 1124,1658

magnetic data for, 1365, 1367, 1368-9, 1370,1371,1376, 1377

marine organisms affected by, 1174 metal, 452-3

allotropic transformation enthalpies of, 453

allotropic transition temperatures for, 453 alloys, 453 crystal structure data for, 452-3, 454,

490,1150, 1391, 1396 mechanical properties of, 1404, 1405,

1405 Mossbauer spectroscopic results for, 490 physical properties of, 452-3, 454, 1150,

1391 preparation of, 452, 1401 thermodynamic properties of, 453, 1150,

1280, 1281, 1334, 1396 triple point for, 453

metallic radius of, 1150, 1450 Mossbauer spectroscopic methods for, 488-

91 electric field gradient data, 488, 489-90 isomer shift data, 488-9 magnetic hyperfine data, 488, 490 structural information from, 490-1

naturally occurring isotopes, 446, 1122, 1170

nitrato complexes, 482, 483 nitride, 459


nuclear spins and moments of, 1648 occurrence in nature of, 446, 1122, 1170 organometallic compounds, 464; see also

Neptunium, cyclo ... oxalato complexes, 483, 484, 1507 oxidation states, 444, 447, 465, 466, 1139

absorption spectra affected by, 465-9, 467,468

determination of, 487-8 oxides, 455, 456-7, 457

crystal structure data for, 457, 1155, 1156 non-stoichiometric, 456, 1163 physical properties of, 1156 thermodynamic properties of, 1156, 1162,

1296, 1301, 1312, 1335 see also Neptunium, complex oxides; ... ,

dioxide; ... , sesquioxide; ... , trioxide

oxyhalides, 461 crystal structure data for, 463, 1443 thermodynamic properties of, 1335

oxysulfides, 460, 1437 palladium compound, 455 peroxide, 457 phosphide, 460, 1437 pnictides, 460, 490

crystal structure data for, 1437 magnetic properties of, 1395

production methods for, 444-5, 445, 1124, 1658

redox kinetics of, 469-81 reduction potentials of, 470-1, 471,1142,

1286,1287 selenides, 460, 1437 separation/purification methods for, 446-52

ion-exchange procedures, 450-1, 551, 552, 553, 553

precipitation procedures, 447 solvent extraction processes, 447-50, 451 tributyl phosphate extraction processes,

447-9 trilaurylamine process, 450, 538 volatility methods, 451

sesquioxide thermodynamic properties of, 1296, 1335

silicides, 460, 1433

Subject Index

Neptunium (Contd.) solution chemistry of, 465-84 sulfates, 464 sulfato complexes, 481-2, 482,1503 sulfides, 460, 1437 tellurides, 460, 1437, 1438 thiocarbamato complexes, 1455 thiocyanato complexes, 1458, 1514 tin compound, 1395, 1407-8, 1407, 1413 trioxide hydrates

crystal structure data for, 457 thermodynamic properties of, 1335

Neptunium-237 decay product of, 112 natural occurrence of, 22, 111,446 nuclear properties of, 445 production of, 444-5, 446, 1124

Neptunium-239 decay products of, 4, 444 natural occurrence of, 446 nuclear properties of, 445

Neptunyl acetato complexes, 807, 1507 Neptunyl chloro complexes, 1.499 Neptunyl fluoro complexes, 1498 Neptunyl g1ycolato complexes, 1507 Neptunyl iminodiacetate complexes, 1516 Neptunyl ions

absorption spectra for, 467, 469, 1266 complexes, 483 disproportionation of, 471-2, 472, 476,

478-9, 1537, 1537 hydrolysis of, 1492-3, 1493 oxidation-reduction reactions, 479-81 reduction potentials of, 470-1, 471 solvent extraction of, 447, 448, 1520 stability in solution of, 1144, 1288 thermodynamic properties of, 1334

Neptunyl nitrate, 1336 Neptunyl oxalato complexes, 1507 Neptunyl oxydiacetate complexes, 1516 Neptunyl oxyfluoride, 461, 463 Neptunyl propionato complexes, 1507 Neptunyl sulfato complexes, 1503 Neutron activation analysis applications,

1190 Neutron irradiation reactions, 1123-7

limitations of, 1125--6 products from, 3-4, 443-4 see also under individual elements (by name)

Neutron sources, actinide elements as, 1189-90

Nilsson diagram, 1650 Nitrates

structural chemistry of, 1450, 1452 see also under individual elements (by name)

Nitrofluor process, 549-50 Nobelium

acetato complexes, 1507 atomic number determined for, 1096

atomic properties of, 1098 chlorides, 1098

thermodynamic properties of, 1305, 1309, 1346

complexes, 1099 discovery of, 7, 10, 1096 electronic configurations of, 1098, 1103,

Il35 free-ion energy level structure for, 1249 hydration enthalpy for, 1293 ionic radii of, 1099, Il03, 1284 ionization energies for, 1103, 1293 ions in solution, 1098-9, 1481, 1483

complexing tendency of, 1098, 1099 stability of, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284,1346 isotopes, 1096-7

decay properties of, 1097, 1667, 1673-4 production methods for, 1097, 1125,

1127,1667 metal, thermodynamic properties of, 1280,

1281,1346 metallic radius of, 1099 oxalato complexes, stability of, 1507 oxidation states of, 1l03, 1139, 1139 production methods for, 1097, 1125, 1127,

1667 reduction potentials of, 1098, 1099, Il03,

1143, 1287, 1481 separation/purification of, 1097-8 sesquioxide, thermodynamic properties of,

1296,1346 solution chemistry of, 1098-9 x-ray spectra of, 1098

Nozzle process (uranium isotope separation), 182

Nuclear fuel, long-lived actinide elements in, 1172-3, 1172

Nuclear fuel reprocessing, 112-18,447,452, 1176

Nuclear incineration, 1176-7 Nuclear power, 1188-9

political/social problems of, 1188-9 Nuclear properties, 1649-74

experimental techniques for, 1651-2 see also under individual elements (by

name), nuclear properties of isotopes Nuclear spins and moments, (listed), 1648 Nuclear systematics, 8 Nuclear waste disposal, 1176-8

geological repositories for, 1177-8

Oak Ridge National Laboratory (USA) electromagnetic separation plant, 180-1,

503 gas diffusion plant, 174, 176-7, 178, 180

Subject Index

High-Flux Isotope Reactor, 8, 990, 1028, 1125, 1652

liquid thermal diffusion plant, 181 plutonium ion-exchange process, 562, 562 Thorex process, 185 Transuranium Processing Plant, 992, 993,

1031, 1032, 1125 Oelsen-Wever index, 631, 631, 632 Oklo nuclear reactor, 194, 1I70-1 Optical spectra, 1235-73

divalent actinide-ion, 1260-2 model calculation of atomic parameters for,

1258-9 models for, 1240-3, 1258 quadrivalent actinide-ion, 1262-4, 1265 trivalent actinide-ion, 1240-57 see also under individual elements (by name)

Organometallic compounds, 1I64, 1166-9, 1547-1624

allyl complexes, 1460, 1548-50 amido-stabilized alkyls, 161I-13 arene complexes, 1463, 1572-3 bent sandwich structures, 1460, 1566, 1567 bond energies, 1600-4, 1601, 1604 carbonyls, 1169, 1589 with chelating cyclopentadienyl ligands,

1167, 1569-71, 1608-10 with chelating peralkylcyclopentadienyl

ligands, 1608-10 cyclo-octatetraene complexes, 1168, 1462-3,

1573-80 cyclopentadienyl complexes, 1166-7, 1167,

1458-9, 1550-60, 1592-8 dihapto-acyls, 1602, 1608, 1609 homoleptic compounds, 1589-92 modified cyclopentadienyl complexes, 1167,

1459, 1563-71, 1598-1610 pentadienyl compounds, 1571-2 peralkylcyclopentadienyl hydrides,

1614-18 phosphine-stabilized hydrocarbyls, 1606-8,

1611,1612 phosphohydrides, 1618-20, 1621 It-bonded, 1I64, 1I66-8, 1458-63, 1547-81 ring-bridged hydrides, 1620, 1622 a-bonded, 1168-9, 1588-1624 structural chemistry of, 1458-63

Oxidation -reduction reactions, 1141, 1144 kinetics of, 1532-9 see also under individual elements (by

name), ions in solution Oxides

structural chemistry of, 1418-24 thermodynamic properties of, 1292, 1294-

1300 see also under individual elements (by name)

Oxoplutonates: see Plutonates Oxyhalides

structural chemistry of, 1443-4, 1443

thermodynamic properties of, 1313 see also under individual elements (by name)

Paducah (USA), gas diffusion plant, 174, 177, 178,180

Parity-allowed/forbidden transitions, 1238 Paschen-Runge spectrograph, 213, 578, 1198 Pentadienyl complexes, 1571-2 Pentavalent ions

in aqueous solution, 1482 hydrolytic behavior of, 1489-90 spectra of, 1264-71 see also Actinyl ions; Americyl ions; ...

Peralkylcyclopentadienyl complexes, 1167, 1565-9, 1598-1608

Periodic table, 1137, Jl38, 1630-1, 1631, 1634 Perovskites, 1298 Peroxyuranates, 276, 279 Phosphates

structural chemistry of, 1450-2, 1453 see also under individual elements (by name)

Phosphato complexes, 1I47 formation and stability of, 1505-5 see also under individual elements (by name)

Phosphides, 62, 64 see also under individual elements (by name)

Phthalocyanine complexes, 1425, 1426, 1457 see also under individual elements (by name)

Pile equations, 506 Pitchblende (mineral), 188-9

chemical composition of, 189, 190 plutonium content of, 504 uranium content of, 504

Plasma desorption mass spectroscopy (PDMS), 1190, Jl91

Plutonates alkali-metal, 711, 713-14 alkaline-earth, 714-15 crystal structure data for, 7/6-17 magnetic properties of, 1370, 1371 thermodynamic properties of, 1302, 1304,

1340 Plutonium

absorption spectra of, 582, 583-4, 585-7, 784-6, 785, 787

acetates, 773 acetato complexes, 806-7

stability of, 808, 1507 see also Plutonyl acetato complexes

acetylacetonate, 777 complexes,816,817

acetylacetonato complexes, 816, 817, 1455, 1511

alloying behavior of, 624-5, 625, 626-7 alloying theories applied to, 625, 628-37

Darken-Gurry method, 632-3, 633, 634 Engel-Brewer theory, 633-5 melting-point depression method, 628,

630,630

Subject Index

Plutonium (Contd.) Miedema's method, 635-7, 638, 639 Oelsen-Wever index, 631, 631, 632 quasi-thermodynamic approach, 628, 629

alloys, 621-57 with aluminum, 623-4 with americium, 900 delta-phase retention in, 622, 638-40, 641 epsilon-phase retention in, 638 with neptunium, 453, 650 preparation of, 623-4 with uranium, 243, 654, 656, 660

alpha coefficients for, 824-5 aluminum compounds, 622

crystal structure data for, 642-3 thermodynamic properties of, 1339

aluminum oxycompounds, 718, 720, 722 aluminum phase diagram, 641, 656, 658 amidosulfonate complexes, 801 antimonides, 622, 680

crystal structure data for, 676, 1438 magnetic susceptibility of, 1406, 1406

applications for, 501-2, 1124, 1188, 1189, 1190-1

arsenates, 768-9 crystal structure data for, 763 physical properties of, 763 solubility of, 773 see also Plutonyl arsenates

arsenazo complex, 816 arsenide, 622, 679-80

crystal structure data for, 676, 1438 density of, 676 preparation methods for, 679

atomic properties of, 577 -87 autoradiolysis effects, 825-7 benzhydroxamate complex, 816 benzoate, 776 N-benzoylphenylhydroxylamine complex,

816 beryllide, 622, 643, 1340 biological behavior of, 1179, 1180, 1181-2 bismuthides, 622

crystal structure data for, 643-4, 1438 thermodynamic properties of, 1339

in blood, 1179 in bone tissues, 1181-2 borides,622,643,1433 borohydride, 755, 760 bromides, 622, 750-1

absorption spectra of, 748, 751 crystal structure data for, 732, 1338, 1441 magnetic properties of, 1376 physical properties of, 732, 734, 1158 preparation of, 750-1 thermodynamic properties of, 734, 1310,

1338 vapor-pressure data for, 734

bromo complexes, 755, 799,800, 802

cadmium compounds, 622, 644 crystal structure data for, 644 thermodynamic properties of, 1339-40

carbides, 622, 667 -73 chemical properties of, 673 crystal structure data for, 667, 670, 671,

1433 decomposition temperatures/pressures of,

672 lattice swelling due to self-irradiation,

667,671 magnetic structure of, 667 phase diagram for, 667, 668 preparation of, 669 thermodynamic properties of, 668, 671-2,

672,1339 carbon phase diagram, 668 carbonates, 764-6

crystal structure data for, 762 physical properties of, 762 see also Plutonyl carbonates

carbonato complexes, 762, 764-6 catechol complexes, 775, 779, 1187, ll87,

1513 cerium~balt phase diagram, 656-7,661 chalcogenides,622, 680-730 chelate compounds, 534-5, 774-5, 777-8,

779,780 chelating agents for, 534-5, 535, 774-5,

777-8, 779, 780, 1185-7 chlorides, 622, 745, 747-50

crystal structure data for, 732, 1157, 1440 physical properties of, 732, 734, ll57 separation/purification methods for, 575,


1309, 1312, 1338 see also Plutonium, tetrachloride; ... ,

trichloride chloro complexes, 754-5, 799, 800, 802,

803,803 crystal structure data for, 759 ion-exchange reactions of, 553, 554 phase diagrams for, 755, 758 physical prgperties of, 759 solubility of, 772 stability of, 1499

chromium oxycompounds, 718, 720, 722 citrato complexes, 810, 8ll cobalt compounds, 622, 644-5 complex carbides, 673, 674 complex halides, 754-5, 756-7, 759

crystal structure data for, 756-7, 759, 1444-5, 1446-7, 1446

electron energy level structures for, 1269, 1270, 1271-2

magnetic properties of, 1365, 1377 physical properties of, 756-7 thermodynamic properties of, 1340

Subject Index

complex ions in solution, 797 -817 complex oxalates, 764 complex oxides, 711, 712-29

with actinide oxides, 724-9 alkali-metal, 711, 713-14, 716-17 alkaline-earth, 714-15,716-17 with cerium dioxide, 724, 724 groups III to VII, 715, 718-19, 720-2,

723 lanthanides, 723-4 thermodynamic properties of, 1302, 1304,

1340 with thorium dioxide, 725 with uranium oxides, 725-9

complex selenides, 729-30 complexes, 797 -817

with monocarboxylic acid anions, 806-10 with monoprotonic acid anions, 798-803 with multiprotonic acid anions, 803-6 with N-polycarboxylic acid anions, 812-

13,814-15 with polycarboxylic acid anions, 810-12

compounds, 622, 657-780 characterization techniques used for, 659 see also Plutonates; Plutonyl, ...

compounds from aqueous solutions, 702-5, 760-71

crystal structure data for, 762-3 physical properties of, 762-3 solubility of, 771-3

conversion chemistry of, 564-77 generalized flow sheet for, 565

copper compounds, 622,645 core level spectra of, 580-1 critical mass of, 502 criticality control during recovery processes,

542, 548, 557, 559, 561 criticality factors for, 502, 502 cupferron complexes, 777 cyc10-0ctatetraene complexes, 780, 1462,

1573, 1579 magnetic properties of, 1377

cyc10pentadienyl complexes, 779-80, 1167, 1553

decontamination of, 506 by ion-exchange processes, 559, 560 by precipitation processes, 515, 516, 569,

571 desferrioxamino complexes, 1186-7 deuteride, 662, 663, 665

decomposition limits of, 665 thermodynamic properties of, 1337

diethylenetriaminepentaacetato complexes, 1186-7

1,3-diketone chelates, 534-5, 774, 777 dioxide, 685-90

actinide mixed oxides, 725, 726-9 cerium dioxide mixed oxides, 724, 724 chemical properties of, 700-2

compatibility of, 698, 700, 701 crystal structure data for, 682, 1156 Debye temperature for, 697 dissolution of, 700-1 fluorination of, 702, 732, 736 halides, 593 lanthanide mixed oxides, 723-4 magnetic properties of, 1377 microspherical form, 686, 688, 689, 701 mixed oxides, 723-9 physical properties of, 682, 690, 1156 preparation methods for, 687 qualitative characteristics of, 686 single crystals, 688, 690 sol-gel process for, 686,688,724, 725,

791 substoichiometric phase, 684, 684, 685,

690,692,696-7,697 thermodynamic properties of, 697, 699,

700, 1162, 1301, 1312, 1337 discovery of, 4, 6, 499-500 distribution coefficients listed for various

solvents, 520 electron configurations of, 577, 1135, 1200,


ion, 1261 electron radial distribution for, 1207 electronic structure of, 577 emission spectra of, 577 -80 energy level parameters for, 1246, 1268-9 equilibrium constant expressions for, 824-5 ethylenediaminetetraacetate complexes, 775,

812-13,814-15, 1186 stability of, 814-15, 1513 thermodynamics for formation of, 814,

1513 fluorides, 622, 733-45


intermediate fluoride, 736 physical properties of, 732, 734, 1157,

1159,1160 precipitation process, 572 preparation methods for, 574-5, 575,

733,734,741-3 thermodynamic properties of, 734, 1305,

1306, 1312, 1338 in volatility process, 548, 549 see also Plutonium, hexafluoride; ... ,

hydroxyfluorides; ... , oxyfluoride; ... , tetrafluoride; ... , trifluoride

fluoro complexes, 754-5, 799, 800, 802 crystal structure data for, 756-7 phase diagrams for, 754, 758 physical properties of, 756-7 precipitation process, 572-3, 574 preparation methods for, 754, 756-7 solubility of, 771-2

Subject Index

Plutonium (Contd.) stability of, 1498

Fourier-transform spectra of, 579, 579 free-ion energy level structure for, 1249 gallides, 622


gallium phase diagram, 641, 656, 659 germanides, 622, 647 germanium oxycompound, 719, 721 global inventory of, 1171, 1172, 1173 glycinato complexes, 807,809 glycolate complexes, 807,809, 810 gold compounds, 622, 643 hafnium compounds, 622, 647-8 halides, 622, 730-52

crystal structure data for, 732, 1157, 1158,1159,1160,1440-1

magnetic properties of, 1376 physical properties of, 732, 734, 1157,

1158, 1159, 1160 reduction to metal, 589-93 separation/purification methods for, 574-


1305,1309,1310,1311,1312,1338 vapor-pressure data for, 734 volatility of, 731, 734

halo complexes: see Plutonium, bromo ... ; ... , chloro ... ; ... , fluoro ... ; ... , iodo complexes

handling procedures for, 577, 659, 661 Hartree-Fock calculations for, 1221, 1223 hazards associated with, 1128 hexafluoride

absorption spectra of, 743, 744, 1272 chemical properties of, 745, 746 compared with neptunium hexafluoride,

736 crystal structure data for, 732, 1160, 1440 electron energy level structures for, 1271,

1272 fluorination equilibrium data for, 737-9,

740 handling techniques lor, 740-1 magnetic susceptibility of, 743 melting point of, 732, 742 physical properties of, 732, 741-3, 1160 preparation methods for, 737-41 radiation decomposition of, 743, 745 thermodynamic properties of, 742, 742,

1338 vapor-pressure data for, 742 vibrational frequencies for, 743, 743 volatility of, 731

hydration enthalpy for, 1293 hydrides, 622, 662-6

chemical properties of, 666 crystal structure data for, 664, 1155, 1432

decomposition temperatures/pressures for, 665, 665

handling techniques for, 666 magnetic properties of, 1378 phase diagram for, 663 physical properties of, 1155 preparation of, 662-3 thermodynamic properties of, 665, 666,

1337 hydrolytic behavior of, 1141 hydroxides, 702-3

solubility of, 772, 1289 hydroxyftuorides, 733 8-hydroxyquinolinate complexes, 777, 778,

816,817 indium compounds, 622, 648 intermetallic compounds, 621-57

crystal structure data for, 642-55 heats of formation for, 635-7, 637 see also Plutonium alloys

iodates, 770 solubility of, 771 see also Plutonyl iodate

iodides, 622, 751-2 crystal structure data for, 732, 1158, 1441 magnetic properties of, 1376 physical properties of, 732, 734, 1158 preparation of, 751-2 thermodynamic properties of, 734, 752,

1311, 1338 vapor-pressure data for, 734

iodo complexes, 802 ionic radii of, 1165, 1284, 1289, 1448 ionization energies for, 1293 ions in solution, 781-839, 782

absorption spectra of, 582, 583-4, 585-7, 784-7, 785, 787, 1239, 1263, 1265

autoreduction of, 826, 827 complexes, 797 -817 disproportionation reactions of, 820-5 electrochemical oxidation/reduction

processes, 839 hydrolytic behavior of, 787-97, 1488,

1489 oxidation states in equilibrium, 819-25 oxidation -reduction equilibria of, 817 -19 oxidation-reduction kinetics of, 828-34,

1533, 1536 oxidation-reduction reactions of, 834,

835-8, 839 preparation of, 782, 783 solvent extraction data for, 1519, 1522,

1523, 1526 stability of, 819-25, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284, 1312, 1337 iridium compounds, 622, 648-9 iron compounds, 622

crystal structure data for, 645-6

Subject Index

thermodynamic properties of, 1340 isotopes, 500-3

decay properties of, 501, 1172,1659,1671 production methods for, 500, 501,501,

502,503,1124,1/25,1659 lactato complexes, 807, 808, 809 lanthanum phase diagram, 641, 657 lead compounds, 622, 650-1 long-term toxicological effects of, 1184-5 luminescence spectra of, 585 magnesium compound, 622, 648 magnetic data for, 1365, 1376, 1377, 1378 manganese compound, 649, 662 manganese oxycompounds, 718, 720, 722 marine organisms affected by, 1174 medical applications of, 501, 1190-1 mercury compounds, 622, 648 metal, 587 -{;57

acid attack of, 620 allotropic transformation enthalpies of,

603,608 allotropic transformation entropies of,

608 allotropic transformation temperatures

for, 598-9, 600-1 alloys, 621-57; see also entry under

Plutonium, alloys atomic bond lengths in, 604, 605 boiling points of, 61 I chemical properties of, 617-21 compressibility of, 612 crucible materials attacked by, 618-21 crystal modifications, 598-9,600-1,602-

4,605,607, 1150, 1151, 1391, 1403 crystal structure data for, 600-1, 1150,

1391 Debye temperatures for, 609, 609 densities of, 600-1,1150,1391 elastic properties of, 612-13, 1405 electrical resistivity of, 613-14, 613 entropy of, 1280, 1337, 1396 first prepared, 589 fusion enthalpies of, 610, 611 Hall effect for, 614-15 heat capacities of, 608-10, 609, 610 liquid density of, 604, 606 liquid reagents, attack by, 618, 620 literature on, 588-9 low-temperature heat capacity of, 608-9,

609 magnetic susceptibilities of, 614, 615, 616,

6/7 mechanical properties of, 612-13, 1404-

5, 1404, 1405 melting point of, 610, 1150, 1391 melting-point depression of, 628, 630, 630 oxidation of, 617-18, 619 phase diagrams for, 641, 656-7, 656, 657,

658, 659, 660, 661

physical properties of, 597-{;17, 1150, 1391

plastic properties of, 612, 1404-5, 1404 preparation of, 589-95, 1401 pressure effects on, 599, 603 reactivity of, 617-21 refining of, 595-7 self-heating effect in, 577, 587-8, 599,

602,616 sublimation enthalpies of, 1105, 1280,

1281, 1337, 1396 surface tension of, 612 thermal conductivity of, 613 thermal expansion of, 602, 606-7, 607 thermodynamic properties of, 603, 607-

10,611, 1280, 1281, 1337, 1396 thermoelectric power of, 615-16, 618 vapor pressure relationships for, 610, 611,

612 viscosity of, 612 water reactivity of, 620

metallic radii for, 602, 605, 1150, 1450 molybdates, 719, 721, 723 molybdenum phase diagram, 641, 656 monoxide, 681

crystal structure data for, 682 density of, 682 thermodynamic properties of, 693-4,

1337 Mossbauer spectra of, 581-2 naturally occurring isotopes of, 503-5 nickel compounds, 622


nickel phase diagram, 656, 660 niobium oxycompounds, 718, 719, 720, 721 nitrates, 766-7

calcination of, 573-4 crystal structure data for, 763 physical properties of, 763 solubility of, 773 tributyl phosphate reactions, 527 see also Plutonyl nitrate

nitrato complexes, 531, 800-1, 802-3 ion-exchange reactions of, 550, 553-{;3

nitride, 622, 675, 677-8 chemical properties of, 677-8 compatibility of, 677 crystal structure data for, 676, 1438· Debye temperature for, 677 dinitride species, 678 magnetic susceptibility of, 677 preparation of, 675, 677 as reactor fuel, 678 thermodynamic properties of, 1339

nitro benzoate, 776 nuclear properties of isotopes, 501, 1659,

1671 nuclear spins and moments of, 1648

Subject Index

Plutonium (Contd.) occurrence in nature of, 503-5, 1122, 1170 optical emission spectra of, 212 -15 organic-acid compounds, 773-5, 776 organometallic compounds, 779-80; see

also Plutonium, cyclo ... osmium compounds, 622, 650 oxalate precipitation processes, 567-9,

773-4 oxalates, 761, 764

crystal structure data for, 762, 1454 physical properties of, 762 solubility plots for, 774, 775 see also Plutonyl oxalates

oxalato complexes, 764, 810 stability of, 811 thermodynamics for formation of, 811

oxidation states, 447, 450, 507, 509, 781, 782, 784, 1139

absorption spectra affected by, 583--4, 785,787

autoradiolysis effects on, 825-7 chemical properties of, 510 formula determination for, 784 precipitation reactions of, 511 preparation methods for, 782, 783 tributyl phosphate extractability affected

by, 528 oxides, 622, 680-705

chemical properties of, 698, 700-2 crystal structure data for, 682, 1155, 1156 densities of, 682 higher oxides, 690 hydrated species, 702-5 melting behavior of, 690 non-stoichiometric, 684, 684, 685, 690,

692-3, 695-7, 697, 1163 physical properties of, 682, 1155, 1156 ternary compounds, 711, 712-29 thermodynamic properties of, 693-7, 698,

1162,1296,1301, 1312, 1337 vaporization behavior of, 691-3, 693, 694 see also Plutonium, complex oxides; ... ,

dioxide; ... , monoxide; ... , ses-quioxide; ... , trioxide

oxyantimonide, 1438 oxygen difluoride reactions, 702, 737 oxygen phase diagram, 680, 681 oxyhalides, 730, 752-3

crystal structure data for, 732, 1443 physical properties of, 732 thermodynamic properties of, 1338 see also Plutonyl halides

oxyselenides, 710, 1438 oxysulfides

crystal structure data for, 706, 1438 densities of, 706 preparation of, 707, 708

oxytelluride

crystal structure data for, 712 density of, 712 preparation of, 711

palladium compounds, 622, 651 perchlorates

complex-forming ability of, 798 solubility of, 771

peroxide, 704-5, 770-1 precipitation process for, 570-2 solubility of, 770

perrhenates, 718-19, 721, 723 phosphates, 767-8

crystal structure data for, 763 physical properties of, 763 solubility of, 773 see also Plutonyl phosphates

phosphato complexes, 805, 806 phosphide, 622, 678-9

crystal structure data for, 676, 679, 1438 density of, 676 magnetic susceptibility of, 679 preparation of, 678-9 thermodynamic properties of, 1339

photoacoustic absorption spectra of, 587 picolinato complexes, 809, 810 platinum compounds, 622, 651 pnictides, 622, 675-80

crystal structure data for, 676 density of, 676

polymeric Pu(IV) species, 703, 781, 790-4, 1145

absorption spectra of, 582, 585, 703, 704, 785

colloidal characteristics of, 703, 793 depolymerization of, 793 formation of, 1489, 1531-2 hydrolytic formation of, 703, 790-3 pH effects on, 791, 792 precipitation behavior of, 793

production methods for, 500, 501, 501, 502, 503, 1124, 1125, 1659

protactinium oxycompound, 718, 721 redox reagents, action of, 834,835-8 reduction by Fe(II) of, 828-30, 831 reduction by U(IV) of, 830, 832-3

activation parameters for, 833 reduction potentials of, 818-19, 1142, 1286,

1287 removal from body fluids of, 1185-7 reviews on, 500 rhenium compounds, 622, 652,718-19, 721,

723 rhodium compounds, 622, 652 ruthenium compounds, 622, 652 salicylates, 776 scandium compounds, 622, 652-3 scandium oxycompounds, 718, 720, 722 scrap reclamation flow sheet, 566 selenides, 622, 708-9

Subject Index

crystal structure data for, 710, 1437, 1438 densities of, 710 magnetic susceptibility of (PuSe), 709 melting point of (PuSe), 709 ternary compounds, 729-30

separation/purification methods for, 505-77 Aquafiuor process, 549, 550 bismuth phosphate process, 362, 512-15 Butex process, 536 calcium hexafluoroplutonate precipitation

process, 572-3, 574 centrifugal-bomb technique, 590, 591 chelation process, 534-6, 537 chloride anion-exchange procedures, 553,

554 co-precipitation procedures, 509-16 conversion chemistry processes, 564-77 direct oxide reduction process, 593, 755 double-crucible techniques, 589-90, 590,

591 double-salt precipitation procedures,

515-16 electrochemical oxidation/reduction pro

cesses, 839 electrorefining processes, 595, 596, 597,

598,755 ether extraction processes, 540-1 fluoride precipitation process, 572, 573 fluoride volatility process, 547-8, 549 Halex process, 541 ion-exchange processes, 550-64, 1531 lanthanum fluoride cycle, 511-12 molten-metal extraction techniques, 544 molten-salt extraction techniques, 544,

546-7 nitrate calcination process, 573-4 nitrate ion-exchange procedures, 553-63 Nitrofluor process, 549-50 non-aqueous processes, 544, 546-50 oxalate precipitation processes, 567-9 peroxide precipitation process, 570-2 precipitation processes, 567-73,574 Pubex process, 542, 544, 545 Purex process, 525-34; see also main

entry: Purex ... pyrometallurgical slagging process, 547 Pyroredox process, 593-5,594, 755 Recuplex process, 542 Redox process, 521, 523, 524-5 Reflux process, 541 Rocky Flats processes, 546,546, 547,

548, 549, 550 solvent extraction procedures, 516-44 stationary-bomb technique, 590, 591,592,

593 thenoyltrifluoroacetone chelation, 535-6,

537,538 tributyl phosphate process, 525 -34 Trigly process, 540

trilaurylamine process, 538-40 zone-melting process, 595, 597

sequestrating agents for, 775, 779, 1186-7 sesquioxide

crystal structure data for, 682, 1155, 1422 densities of, 682 hyperstoichiometric phases, 684, 690, 693,

695 magnetic properties of, 1378 melting point of, 690 physical properties of, 682, 1155 preparation of, 683 thermodynamic properties of, 694-5,

1162, 1295, 1296, 1297, 1299, 1337 silicates, 719, 720, 721 silicides, 622, 674

crystal structure data for, 670, 674, 1433 density of, 670 reactivity of, 674

silicon phase diagram, 675 silver compounds, 622, 642 solid-state absorption spectra of, 585, 784 solution chemistry of, 781-839 spectral term analysis for, 578-80 sulfates, 769-70

crystal structure data for, 763 physical properties of, 763 solubility of, 772-3 thermodynamic properties of, 1339 see also Plutonyl sulfate

sulfato complexes, 804, 806, 1503 sulfides, 622, 705-8

crystal structure data for, 706, 1437, 1438 densities of, 706 magnetic susceptibilities of, 708, 709 preparation of, 707 -8, 707 thermodynamic properties of, 1338-9 see also Plutonium, monosulfide

tantalum compounds, 622, 653 tantalum oxycompounds, 718, 719, 721 tartrato complexes, 811, 812 tellurides, 622, 709, 711

crystal structure data for, 712, 1437, 1438 densities of, 712 magnetic susceptibilities of, 711 preparation of, 709, 711

tellurium oxycompound, 719, 721 tetrachloride, 749-50

absorption spectra of, 749-50, 750 physical properties of, 750 solubility of, 771 thermodynamic properties of, 750, 1312,

1338 tetrafluoride, 735-6

crystal structure data for, 732, 1159, 1440 physical properties of, 732, 734, 1159 preparation methods for, 575, 575, 733,

735-6 reactions of, 736

Subject Index

Plutonium (Contd.) thermodynamic properties of, 734, 1312,

1338 vapor-pressure data for, 734

thenoyltritluoroacetonato chelates, 535-6, 777,816

thiocarbamate compounds, 777, 778 thiocyanato complexes, 799

stability of, 1514 structure of, 1458

thoron complex, 816 tin compounds, 622, 653


toxicity of, 10, 661 toxicology of, 10,661, 1028, 1182, 1183--4 tracer studies, feasibility of, 500 transferrin complex, 1179 trichloride, 745, 747-9

absorption spectrum of, 585, 586, 587, 748,748

chemical properties of, 748-9 crystal structure data for, 732, 748, 1157,

1440 hydrolysis of, 749 magnetic properties of, 748, 1376, 1378 phase diagrams with other chlorides, 755,

758 physical properties of, 732, 734, 747, 1157 preparation methods for, 575, 576, 745,


1309,1338 vapor-pressure data for, 734

trifluoride, 735 absorption spectrum of, 585 crystal structure data for, 732, 1157,

1440 phase diagrams with other fluorides, 754,

758 physical properties of, 732, 734, 1157 preparation methods for, 574, 733, 735 reactions of, 736 solubility of, 771 thermodynamic properties of, 734, 1306,

1338 vapor-pressure data for, 731, 734

trioxide hydrate, 690, 703 tropolonato chelates, 777 uranium phase diagram, 243, 656, 660 uranium-oxygen phase diagram, 725, 725 vanadium oxycompounds, 718, 720, 721,

722,723 weighable amounts first isolated, 6, 500 x-ray spectra for, 580 zinc compounds, 622


zirconium compounds, 622, 655

Plutonium-238 applications for, 501-2, 1124 conversion chemistry of, 576-7 criticality factors for, 502 discovery of, 499 Mossbauer spectra of, 581 production of, 4, 446, 499, 500, 889

Plutonium-239 criticality factors for, 502, 502 discovery of, 6, 500 fissionability of,S, 500, 1188 half-life of, 501, 502 Mossbauer spectra of, 581 production of, 4, 171,444,500,1124

Plutonium-240 Mossbauer spectra of, 581-2

Plutonium-24I conversion chemistry of, 576-7 criticality factors for, 502 decay products of, 546

Plutonium-242, production of, 503, 890 Plutonium-244

occurrence in nature of, 505 production of, 503

Plutonyl acetate complexes, 773, 807,808 crystal structure data for, 762 magnetic susceptibility of, 773 physical properties of, 762

Plutonyl acetato complexes, stability of, 808, 1507

Plutonyl carbonates ammonium salts, 765-6, 765, 766 complexes, 765-6

Plutonyl per.:hlorates, solubility of, 771 Plutonyl chloride, 732, 753, 771

complex salts, 755, 759 Plutonyl chloro complexes, 803

absorption spectra of, 587, 588 stability of, 1499

Plutonyl chloroacetato complexes, 807,808, 1507

Plutonyl ethylenediaminetetraacetato complexes, 813

stability of, 815, 1513 Plutonyl fluoride, 732, 753, 771 Plutonyl fluoro complexes, 1498 Plutonyl furan compounds, 776

complexes in solution, 809 Plutonyl gIycolato complexes, 809, 1507 Plutonyl halides, 753

crystal structure data for, 732 physical properties of, 732 solubility of, 771

Plutonyl iminodiacetate complexes, 1516 Plutonyl ions

absorption spectra of, 584, 785, 1266 fine structure of, 786

disproportionation of, 1537, 1537 evidence for existence of, 784, 786

Subject Index

hydrolytic behavior of, 795-7, 1492-3, 1493

infrared spectrum of, 786 O-PU-O vibrational frequency for, 786 Raman spectral frequencies for, 786 stability of, 1144, 1288 thermodynamic properties of, 1337

Plutonyl nitrate, 766-7, 803 crystal structure data for, 763

Plutonyl oxalate, 761, 764, 812 crystal structure data for, 762 physical properties of, 762

Plutonyl oxalato complexes, 811,812 stability of, 811 thermodynamics for formation of, 811

Plutonyl oxydiacetate complexes, stability of, 1516

Plutonyl phosphates, 767-8 crystal structure data of, 763 physical properties of, 763

Plutonyl pyridino compounds, 776 complexes in solution, 809

Plutonyl sulfate, 770 complex salt, 770 crystal structure data for, 763 physical properties of, 763

Plutonyl thiopen compounds, 776 complexes in solution, 809

Pnictides structural chemistry of, 62, 64, 1435-6,


Polymeric ions, 1141, 1143, 1145, 1146 sorption of, 1175 see also Plutonium, ... ; Uranium, poly

meric ions Portable power sources, 501-2, 1189, 1190-1 Portsmouth (USA), gas diffusion plant, 174,

177,179,180 Precipitation methods

americium separation, 891 neptunium separation, 446, 447 plutonium separation, 509-16 protactinium separation, 119 uranium separation, 206-7

Production methods, 1123-7, 1653-68 heavy elements, 1127, 1629, 1630 see also entries under individual elements (by

name) Promotion energy function plots, 1297, 1298,

1299 Protactinium

absorption spectra of solutions, 143, 144, 147, 152

acetylacetonato complexes, 1455, 1511 alloys, 127, 128 americium complex oxides, 906 antimonides, 139 applications for, 102

arsenides, 139 atomic properties of, 125-6 beryllide, 128 borohydride, 141 bromides, 133


physical properties of, 1159, 1160 preparation of, 134 thermodynamic properties of, 1310, 1312,

1320 carbides, 129, 132

crystal structure data for, 129 magnetic susceptibility of, 129 thermodynamic properties of, 1320

carboxylate complexes in solution, 149, 150, 151

chalcogenides, 139 chlorides, 132-3

crystal structure data for, 135, 1159, 1440 magnetic properties of, 1367, 1367 physical properties of, 134, 1159 preparation of, 133 thermodynamic properties of, 1312. 1320

chloro complexes in solution, 144-5, 146 complex chalcogenides, 139 complex halides, 136

crystal structure data for, 137, 138 structure of, 1446, 1446, 1448 thermodynamic properties of, 1320

complex ions in solution, 143-51 complex oxides, 131,131,906 compounds, 128--41 cyclo-octatetraene complexes, 141, 1462,

1573, 1574 cyclopentadienyl complexes, 141, 1167, 1554

magnetic susceptibility of, 1368 discovery of, 15, 103-4 electrolytic reduction in solution of, 151 electron configurations of, 125, 1135, 1203,

1204, 1225, 1237, 1238 emission spectrum of, 125, 126 energy level parameters for, 1268 fluorides, 132, 132, 133, 135


physical properties of, 1158, 1159 preparation of, 133 thermodynamic properties of, 1312, 1320

fluoro complexes, 145-7, 148, 149 stability of, 1498

formate, 140, 141 magnetic susceptibility of, 1367-8

global inventory of, III halides, 131-6, 137-8

crystal structure data for, 135, 1159--60, 1440-1

physical properties of, 134, 1159--60 preparation of, 132, 133, 134

Subject Index

Protactinium (Con/d.) thermodynamic properties of, 1310, 1312,

1320 Hartree-Fock calculations for, 1221 hydration enthalpy for, 1293 hydride, 129

crystal structure data for, 129, 1155 physical properties of, 1155 structure of, 1427

hydrolysis of, 142-3, 152 hydroxide, activity products of, 1289 iodides, 133-4, 134, 135

crystal structure data for, 135, 1158, 1I59, 1I60, 1441

physical properties of, 136, 1I58, 1I59, 1I60

preparation of, 134 thermodynamic properties of, 1312, 1320

ionic radii of, 1I65, 1284, 1289, 1448 ionization energies for, 1293 ions in solution, 142-53

absorption spectra, 143, 144, 147,152 complexes in mineral acid solutions,

143-9 complexes with organic acids, 149, 150,

151 hydrolysis of, 142-3, 1141, 1145, 1486-7,

1488 oxidation of, 151-2 Pa(IV) complex formation, 152-3 polarography with, 151 redox behavior of, 151-2 stability of, 1I44, 1288 thermodynamic properties of, /280, 1281,

1284, 1312, 1320 iridium compound, 128 isolation of, 104 isotopes, 102, 104-11

decay properties of, 105, 1172, 1656, 1670 production methods listed fot, 105, 106,

107, 110, 1123, 1656 magnetic data for, 1367-8, 1367 metal, 126-7, 128

crystal structure data for, 128, 1I50, 1391 magnetic susceptibility of, 128 physical properties of, 128, 1I50, 1391 preparation methods for, 126-7, 1401 reactivity of, 127 single crystals, 127, 140 I superconductivity of, 127, 128, 1153, 1394 thermodynamic properties of, 128, 1150,

1280, 1281, 1320, 1396 vapor pressure of, 127, 128

metallic radius of, 128, 1I50, 1450 Mossbauer effects for, 125-{i, 127 naturally occurring isotope of, 102, III nitrato complexes, 139, 144, 145 nuclear properties of isotopes, 104-11, 105,

1655,1670

nuclear spins and moments of, 1648 occurrence in nature of, 111-12, 1170 origin of, 15, 104 oxalato complexes, 119, 139, 149, 150, 151 oxidation states of, \02, 142, 1139 oxides, 129-31

crystal structure data for, 130, 131, 1I56, 1421

physical properties of, 1156 ternary oxides with plutonium, 718, 721 thermodynamic properties of, 1301, 1312,

1320 oxyhalides

crystal structure data for, 135, 1443-4, 1443,1444

preparation of, 132, 133, 134 thermodynamic properties of, 1320

oxysulfide, 139, 140 phenylarsonato complexes, 141 phosphares, 140, 141 phosphides, 139, 140 phthalocyaninato complexes, 141 platinum compounds, 128 plutonium oxycompound, 718, 721 pnictides, 139 polymeric Pa(V) species, 1123-4 production methods for, 104-5, 106, 110,

ll23, 1656 quaternary ethylamino complexes, 140, 141 reduction potentials of, 151, 1I42, 1286 rhenium compound, 128 selenato complexes, 139, 140 separation/purification methods, 112-25

analyses of typical starting materials, 113 crystallization methods, 119 enrichment, 114-8 ion exchange, 120-1 macroscopic amounts of Pa-23I, 118-23 precipitation, 119 protactinium-233, 124-5 protactinium-234, 123-4 solvent extraction, 121-2

solution chemistry, 142-53 sulfato complexes, 139, 140, 145, 146,147 sulfide, 139 thiocyanato complexes, structure of, 1458 tropolonato complexes, 140, 141

Protactinium-231, 105, 106 alpha spectrum of, 108 gamma spectra of, 108, 109 large-scale purification of, 118-23 occurrence in nature of, III production of, 106

Protactinium-233, \09-10 occurrence in nature of, 111-12 purification of, 124-5

Protactinium-234, 106, 109 gamma spectra of, 110, 111 purification of, 123-4

Subject Index

Protactinium-234m, 106, 110 gamma spectrum of, 110 purification of, 123-4

Protactinyl acetylacetonato complexes, 1511 Protactinyl ion, 1145

hydrolysis of, 1489-90 solvent extraction data for, 1519

Pubex process, 542, 544,545, 1521 Pulse radiolysis technique, 1137, 1139 Purex process

advantages of, 534 decladding step in, 528-9,529 extractant used in, 517, 1518, 1521 fuel dissolution step, 530 modifications to, 533 neptunium separation by, 447, 528 plant-scale performance of, 534 plants listed, 526 plutonium separation by, 525-34 solvent extraction equilibria for, 1521-2,

1522 solvent used in, 517 two-cycle process, 529, 531,532, 533 uranium non-extractable by, 768

Pyroredox process, 593-5, 594, 755

Radioactinium, 15, 16 Radioactive series: see Decay series Radiochemical techniques, 9, 485

see also Tracer studies Rare-earth elements

actinide elements compared with 9, 444 recovery from monazite sands, 48, 49 see also Lanthanide ...

Recoil-atom catcher technique, 1093-4, 1097, 1101

Recuplex process, 542, 543 Redox behavior

actinium ions, 30, 32 americium ions, 915, 917-19, 917 berkelium ions, 1012-14, 1013 californium ions, 1052-4 neptunium ions, 469-71, 472-81 plutonium ions, 817-19 protactinium ions, 151-2 uranium ions, 396, 398-9

Redox process, 521, 524-5 advantages/disadvantages of, 524-5 extractant used in, 517, 1517 flow sheet for, 523 plant-scale performance of, 525

Reduction potentials, 1140-1, 1142-3, 1286-7

compared with f -d transition energies, 1206,1206

see also under individual elements (by name) Reflux (plutonium recovery) process, 541 Relativistic effects, superheavy elements, 1636,

1638-42

Relativistic Hartee-Fock calculations, 1200, 1220-3, 1221, 1223

Relativistic Hartree-Fock-Slater calculations, 1640

Reversed-phase chromatography, 25-6, 1133 Rocky Flats (USA)

americium separation plant, 546, 546, 547, 890, 891, 895

plutonium separation plant, 546,546, 547, 548,549,550

Ruckruckstiinde, 112 enrichment of, 114-15 typical analysis of, 113

Russell-Saunders coupling, 1363 metals, 1406

Rutherfordium: see Element 104

Salting-out effect, 1523, 1525-6 Sandwich complexes, 1168, 1573; see also

Cyclo-octatetraene ... Seawater, uranium content of, 195-6, 1505 Sequestering agents, 394, 775, 779 Silicides

structural chemistry of, 1433, 1434-5 see also individual elements

Solid solutions, metals, 1397-8 Solid-state behavior, actinides, 62 Solid-state compounds, 1154-69

binary compounds listed, 1154, 1155--{)0 non-stoichiometric systems, 1161-3

Solution chemistry, 1137, 1139-47, 1480-1538 see also under individual elements (by name)

Solution enthalpies halides, 1305, 1306, 1307, 1309-11 oxides, 1295, 1295, 1296, 1297, 1300, 1301

Solvent extraction chromatography (separation process), 1088, 1094, 1097-8, 1516-7

Solvent extraction equilibria, 1516-26 alkylammonium extractants, 1524-6 anionic extractants, 1518-21 neutral extractants, 1521-4

Solvent extraction processes, 519, 1132-3 extractants used in, 415, 517,1133,1517-

18, 1523 flow sheet for, 522 nomenclature for 520-1 organophosphorus extractants, 1519, 1520,

1521-2, 1522, 1523 oxidation state, effect on, 510 see also under individual elements (by

name), separation/purification methods for

Specific activities, 1669-74 definition of, 1674 (footnote) see also individual elements, isotopes ...

Specific heat electronic term in

intermetallics, 1407, 1407

Subject Index

Specific heat (Contd.) metals, 1394, 1409

temperature variation of intermetallics, 1408, 1408

Spectra: see Absorption ... ; Condensed-phase ... ; Emission ... ; Optical ... ; Solid-state ... ; Vapor-phase ... ; X-ray spectra

Spectral parameter fitting processes, 1216-20 and configuration interaction, 1218-19 truncation errors in, 1217 -18 and weak interactions, 1219-20

Spectral parameters, 1220-3 Spectrophotometric (analytical) methods,

485-6,486, 786-7 Spectroscopic studies, 1134-5

see also Absorption ... ; Emission spectra Spin-orbit interaction, 1214-16, 1241 Spontaneous fission, 1650 Stark effect, 1196 Stoner criterion, 1406 Structural chemistry, 1417-63

actinyl complexes, 1424-6 arsenates, 1453 borides, 1432-3, 1433, 1434 carbides, 1432-4, 1433 carbonates, 1449-50 carboxylates, 1454-5 chakogenides, 1435-6, 1437-8 chelate complexes, 1455-8 halides, 1436, 1439, 1440-1, 1442-3 halo complexes, 1446-7 hydrides, 1426-7, 1432 nitrates, 1450, 1452 organometallic compounds, 1458-63 oxides, 1418-24 oxyhalides, 1443-4, 1443 phosphates, 1450-2, 1453 pnictides, 1435-6, 1437-8 silicides, 1433, 1434-5 sulfates, 1452-4 thiocarbamates, 1455 see also under individual elements (by

name), crystal structure data ... Sublimation enthalpies

boiling points predicted by, 1636 (listed), 1150, 1280, 1281, 1315-46,

1395 as means of identifying elements, 1632

Sulfates structural chemistry of, 1452-4 see also under individual elements (by name)

Sulfato complexes formation of, 1502 formation and stability of, 1502, 1503 stability of, 1503 thermodynamics for formation of, 1503 see also under individual elements (by name)

Superactinide elements, 1633, 1642

Superconductivity, metals/intermetallics, 1153, 1409-13

experimental difficulties for, 1153 Superheavy elements, II

boiling point anomaly for, 1636 chemical properties predicted for, 1635-43 electronic structure of, 1633-5 island-of-stability concept for, II, 1629,

1643 nuclear properties predicted for, 1643 relativistic effects in, 1636, 1638-42 synthesis of, 1643-5

TBP process americium separation by, 892 extractant used in, 414, 517, 1518, 1521 neptunium separation by, 447-9 plants listed, 526 plutonium separation by, 525-34 uranium separation by, 208, 209 see also Purex process

Temperature-independent paramagnetism (TIP), 1362

Term analysis, emission spectra, 212-13, 578-90, \198-9

matrix method for, 12\1-14 Tetraammonium tricarbonatouranylate, 355,

356, 358 decomposition of, 355

Tetrad effect, 1447 Tetravalent ions

in aqueous solution, 1481-2 hydrolytic behavior of, 1484-9 spectra of, 1262-4, 1265

Thenoyltrifluoroacetonato complexes, 1147 extraction data for, 1519 see also under individual elements (by name)

Thenoyltrifluoroacetone, 517, 1147, 1512 in solvent extraction processes, 535-6, 537,

538, 1518, 1519 Thermochromatography, 1632 Thermodynamic properties, 1278-1347

gaseous atoms and ions, 1292 halides, 1300, 1303-14, 1347 hydrolytic reactions, 1495-7 ions in solution, 1282-91 (listed), 1315-46, 1347 literature covering, 1278-9 metals, 1279-81, 1395-7 organoactinides, 1600-4 oxidation -reduction reactions, 1532, 1532,

1536 of oxides, 1292, 1294-1300 see also under individual compounds (by

name) Thermonuclear explosive device testing, 5,

1071, 1086, 1087, 1127 Thiocarbamates, structural chemistry of, 1455

Subject Index

Thiocyanato complexes, 1514, 1514, 1515, 1530

l110racene, 83, 1462, 1573, 1574 l110racyclobutanes, 1602, 1606 l110rex process (U-233 separation), 184-6 l110rite (mineral), 43 l110rium

acetate thermodynamic properties of, 1318

acetato complexes stability of, 1507, 1508 structure of, 1454 thermodynamics for formation of, 1510

acetylacetonato complexes, 84 stability of, 1511 structure of, 1455

alkyls, 1590-1 allyl complexes, 1548 antimonides,63,66,1437 applications for, 41-2 arsenides, 63, 66, 1437 atomic spectroscopy of, 47-9 benzyls, 83, 1592 bismuthides, 63, 66, 1437 bis(pentamethylcyclopentadienyl) alkoxy-

hydrides, carbonylation of, 1616-18 bis(pentamethylcyclopentadienyl) alkyl

complexes, 1599, 1600-3 bond disruption enthalpies for, 1601,

1603 bis(pentamethylcyclopentadienyl) buta

dienido complex, 1599, 1599 bis(pentamethylcyclopentadienyl) com

plexes, 1599, 1600-2, 1601, 1603, 1604, 1605

structure of, 1605, 1607, 1608 bis(pentamethylcyclopentadienyl) hydride,

1614-15, 1615 borides, 54, 56, 1433 borohydro half-sandwich complexes, 1580 boron carbides, 58 bromides, 69, 73-4

crystal structure data for, 69, ll59, 1441 physical properties of, 74, ll59 preparation of, 73-4 thermodynamic properties of, 74, 1310,

1312, 1316-/7 butyrato complexes, stability of, 1508 carbides, 54, 56-8, 58

crystal modifications, 56 crystal structure data for, 54, 1433-4,

1433 phase diagram for, 58 physical properties of, 56-7 reactions of, 57-8 thermodynamic properties of, 13/7-18

carbonate, 79 complex salts, 79

carboxylates, 82

chalcogenides, 59, 65-6 chlorides, 69, 71-2, 73

crystal structure data for, 69, 1159, 1440 double salts, 72-3, 73 physical properties of, 72, 1159 preparation of, 71-2 solubility of, 73 thermodynamic properties of, 72, 1312,

1316 chloro complexes

stability of, 1499 chloroacetato complexes

stability of, 1507, 1508 chloropropionato complexes

stability of, 1508 cbromates, 81 cobalt compounds

thermodynamic properties of, 1319 complex halides, 69, 70-4

crystal structure data for, 68-9, 1445, 1446,1446

phase diagrams for, 70, 71 thermodynamic properties of, 1319

complex oxides, 60, 906 compounds, 53-84 concentration in lithosphere of, 1170 coordination number of, 85 cyclo-octatetraene half-sandwich complexes,

1580, 1581 cyclo-octatetraene sandwich complexes, 83,

1462, 1573, 1574, 1580, 1581 cyclopentadienyl complexes, 83, 84, 1167,

1552, 1553, 1559, 1592-5 bond energies for, 1594 magnetic properties of, 84, 1367

deuterides, thermodynamic properties of, 1316

dioxide, 59, 60, 61 crystal structure data for, 59, 1156 physical properties of, 1156 thermodynamic properties of, 1162, 1312,

1315 1 ,3-diphenylpropane-l ,3-dionato complex,

1456 discovery of, 41 electron configurations of, 47, 48, 49, 1135,

1203, 1204, 1224-5, 1229, 1237, 1238 emission spectra of, 47-9 ethylenediaminetetraacetato complexes,

stability of, 1513 fluorides, 67, 68

crystal structure data for, 68, ll58, 1440 double salts, 67, 71 hydrolytic reactions of, 67 phase diagrams with other fluorides, 70,

71 physical properties of, ll58 preparation of, 67 solubility of, 1500

Subject Index

Thorium (Con/d.) thermodynamic properties of, 1312, 1316

ftuoro complexes stability of, 1498 thermodynamics for formation of, 1501

formato complexes, stability of, 1508 germanides, thermodynamic properties of,

1318 glycolato complexes

stability of, 1507, 1508 thermodynamics for formation of, 1510

halides, 66-75 crystal structure data for, 68-9, 1158-9,

1440-1 physical properties of, 72, 74, 1158-9 preparation methods for, 67, 71---4 thermodynamic properties of, 72, 74,

1310, 1312, 1316-17 Hartree-Fock calculations for, 1221 hydration enthalpy for, 1293 hydrides, 53, 54, 55-6

crystal structure data for, 54, 1155, 1427 decomposition of, 55 physical properties of, 1155 reactions of, 55-6 ring-bridged, 1620-2, 1622 superconductivity of, 53 thermodynamic properties of, 1316

hydroxide, 75-6 absorption of carbon dioxide by, 76, 79 activity product of, 1289

hydroxybutyrato complexes, stability of, 1508

8-hydroxyquinolinato complexes, 84 iminodiacetate complexes, thermodynamics

for formation of, 1517 indium compound, thermodynamic proper

ties of, 1318 intermetallic compounds, thermodynamic

properties of, 1318-19 iodides, 69, 74-5

crystal structure data for, 69, 1157, 1159, 1441

physical properties of, 74, 75, 1157, 1159 preparation of, 74 thermodynamic properties of, 74, 1312,

1317 ionic radii of, 84, 1165, 1284, 1448 ionization energies for, 48, 1293 ions in solution, 84-6

cation exchange reactions, 85 complexes, 85-6 coordination number of, 85 hydrolysis of, 85, 1484-6, 1485, 1486,

1487,1488 solvent extraction data for, 1519 stability of, 1144, 1288, 1481, 1484 thermodynamic properties of, 1280, 1281,

1284, 1312, 1315

thermodynamics for hydrolysis of, 1495-7,1496

isobutyrato complexes, stability of, 1508 isotopes, 42-3, 44

decay properties of, 44, 1172, 1654-5, 1669-70

production methods listed for, 44, 1654-5

lactato complexes, stability of, 1508 lead compound, thermodynamic properties

of, 1318 liquid-liquid chromatography for Th(IV),

451 magnetic data for, 1367 maleato complexes, stability of, 1508 malonato complexes, stability of, 1508 metal,50-3

alloys, 51 boiling point of, 51 critical temperature for, 51 crystal structure data for, 50, 50, 1150,

1391 elastic constants for, 50 electrical properties of, 50 mechanical properties of, 1404, 1404,

1405 passivation of, 52 physical properties of, 50, 50, 1150, 1391 preparation of, 50-I, 1401 reactivity of, 51-2, 55 residue after hydrochloric acid reaction,

52 single crystals, 140 I superconductivity of, 51, 1394 thermal properties of, 50 thermodynamic properties of, 50, 1150,

1280, 1281, 1315, 1396 vapor pressure of, 50, 51

metallic radii of, 1150, 1450 metallocycle, 1612-13 minerals, 43, 45

plutonium in, 504 molybdates, 81-2 natural occurrence of, 43, 45 nickel compounds, thermodynamic proper

ties of, 1319 nitrates, 76-8

double salts, 78 solubility of, 77 thermodynamic properties of, 1317

nitrato complexes, 77, 78 nitrides, 61-2, 63


nuclear fuels based on, 42 nuclear spins and moments of, 1648 occurrence in nature, 43, 45 ore processing for, 46, 47, 48, 49 organometallic compounds, 83---4

Subject Index

magnetic properties of, 84, 1367 oxalate, 82, 1318 oxalato complexes, stability of, 1507, 1508 oxidation state of, 84, 1139 oxides, 58, 59, 60-1

crystal structure data for, 59, 1156, 1421 physical properties of, 1156 ternary oxides with plutonium, 725 thermodynamic properties of, 1162, 1312,

/3/5 see also Thorium, dioxide

oxine complexes, 84 oxyanion compounds, 75-82 oxydiacetate complexes, thermodynamics

for formation of, 1517 oxyhalides, 67, 72, 74, 75

crystal structure data for, 68, 69, 1443 preparation of, 67, 72, 74, 75 thermodynamic properties of, 72, 1316,

1317 . oxymetallates, 82 oxyperchlorate, 78 oxyselenides, crystal structure data for,

1437 oxysulfide, 65

crystal structure data for, 65, 1437 oxytellurides, crystal structure data for,

1437 pentamethylcyc10pentadienyl complexes,

1605-6, 16/0 perchlorate, 78 peroxide, 61 phosphates, 80-1 phosphides, 63, 66


phosphine complexes, 83 phthalato complexes, stability of, 1508 pnictides, 64, 66 propionato complexes, stability of, 1507,

1508 reduction potentials of, 1142, 1286, 1287 ring-bridged hydride, 1620-2, 1622 ruthenium organometallic compound,

1623-4, 1624 selenides, 59, 65

crystal structure data for, 59, 1437 separation/purification methods, 46, 52-3

ion-exchange procedures, 553, 554 silicides, 54, 56, 57

crystal structure data for, 54, 1433 phase diagram for, 57 thermodynamic properties of, 1318

silicocyc1opentadienyl complexes, 1609-10, 1614

silicon phase diagram, 56, 57 solution chemistry of, 84-6, 1141, 1145 succinato complexes, stability of, 1508 sulfate, 79-80

thermodynamic properties of, 1317 sulfate double salts, 80

structure of, 1452 -3 sulfato complexes


sulfides, 59, 64-5 crystal structure data for, 59, 1437 physical properties of, 64, 65 thermodynamic properties of, 1317

sulfites, 80 tellurides, 59, 65-6 tetrabenzyl complex, 83, 1592 tetramethylenediamino complexes, 1591,

1591 thallium compound, thermodynamic pro

perties of, 1318 thiocarbamato complexes, structure of, 1455 thiocyanato complexes

stability of, 1514 structure of, 1458

thiodiacetato complexes, thermodynamics for formation of, 1517

thioglycolato complexes stability of, 1507, 1508 thermodynamics for formation of, 15/0

tin compound, thermodynamic properties of, 1318

tris(cyc1opentadienyl) complexes, 1592, 1593-5

bond disruption enthalpies for, 1594 tritides, thermodynamic properties of, 1316 tropolonato complexes, 1456-7 zinc alloys, 53

thermodynamic properties of, 1319 Thucholite (mineral), 190, 191 Thujaplicin (IPT) chelates, 1147, 1512, 1518,

1519 Tobernite minerals, 190-1, 190, 1451, 1453

chemical composition of, 192, 192,372 Toxicity hazards, 10,661, 1128, 1182-7 Toxicology, 1182-7

ingestion mechanisms, 1182-3 long-term effects, 1184-5 of plutonium, 1183-4 removal methods, 1185-7 of uranium, 1184

Tracer studies, 9, 1130 neptunium, 445, 476, 477, 478-81 plutonium, 500 protactinium, 110 thermodynamic properties determined

using, 1281 Tramex process, 894, 965 Transeinsteinium elements, 1085-113, 1629-

45 see also Fermium; Lawrencium;

Mendelevium; Nobelium; Element 104 ... 121

Subject Index

Transition elements compared with actinides, 1149, 1389 electronic structure of, 1390, 1392

Transplutonium elements cyclopentadienyl complexes, 1553 ion-exchange behavior of, 553, 1089, 1527-

8, 1528, 1529 see Americium; Berkelium; Californium;

Curium; Einsteinium; Fermium; Lawrencium; Mendelevium; Nobelium

Transuranium elements, 6-7 actinyl ion absorption spectra, 928 early doubts about existence, 443 lanthanide elements compared with, 9,

444 weighable amounts first isolated, 6-7 see Neptunium; Plutonium; ...

Trigly process, 540 extractant used in, 415, 517

Trivalent ions in aqueous solution, 1481 hydrolytic behavior of, 1483--4 spectra of, 1239, 1240-57

effective operators for, 1244-5 free-ion models for, 1240-1 intensity calculations for, 1253-5,

1256 predictive model for, 1242-3

Tropolonato complexes, 777, 1147, 1512, 1518, 1519

extraction data for, 1519 see also under individual elements (by name)

Ultramicrochemical methods, 9, 1130-1 Uranates, 271-3, 276, 279

see also Uranium, complex oxides Uraninite (mineral), 189-90, 190 Uranium

absorption spectra for, 218, 219, 221, 222, 398, 1239, 1248, 1263, 1265

acetate, 339, 1329, 1454 see also Uranyl acetate ...

acetylacetonato complexes, 1455 stability of, 1511

alkoxides, 387 -90 chemical interrelationships among,

389 complexes, 390 physical properties of, 391-2 preparation of, 387, 389-90,389 reactions of, 387, 389, 390

alkylmercaptides, 336 alkyls, 1590 allenyl compounds, 368, 378 alloys, 233--4, 242, 243--4, 243, 247, 453 allyl complexes, 1460, 1549-50, 1549 aluminides, 234, 235, 236, 242

crystal structure data for, 236

magnetic properties of, 1408, 1408, 1413 phase diagram for, 242 thermodynamic properties of, 1330

aluminum isopropylate, 390 amides, 291, 313, 335--6 amido complexes

amide complexes, magnetic properties of, 1375

structure of, 1458 antimonides, 235, 292

crystal structure data for, 290, 1437 magnetic properties of, 293 physical properties of, 290 thermodynamic properties of, 1328

arene complexes, 1463, 1572-3, 1572 arsenates: see Uranyl arsenate ... arsenides, 235, 292

crystal structure data for, 290, 1437 magnetic properties of, 293, 294, 295 physical properties of, 290 preparation methods for, 292 thermodynamic properties of, 1327

atomic spectroscopy of, 212-15 benzylcyclopentadienyl chloro complex,

structure of, 1459, 1555, 1556 beryllide, 235, 236, 1331

magnetic properties of, 1409, 1412, 1413

bismuthides, 235, 292 crystal structure data for, 290, 1437 physical properties of, 290 thermodynamic properties of, 1328

bis(pentamethylcyclopentadienyl) complexes, 1566-70, 1566, 1568, 1600, 1602, 1603, 1604, 1619-21

bond disruption enthalpies for, 1602, 1603

bis( I, 3,5, 7 -tetramethylcyclo-octatetraene) complex, 1575, 1576

bis( 1,3,5, 7 -tetraphenylcyclo-octatetraene) complex, 1576, 1576

in blood, 1179 borides, 235, 280, 283--4

crystal structure data for, 281,1433 phase diagram for, 283 physical properties of, 281 thermodynamic properties of, 1330

borohydrides, 255--6 structure of, 255, 257, 258, 1432

borohydro derivatives, 1461, 1558, 1560-1 boron phase diagram, 283 bromides, 235, 327

crystal structure data for, 302, 329, 1157, 1159, 1160, 1441

magnetic properties of, 1376 mixed halides, 302-3, 327 physical properties of, 302, 328, 329,

1157, 1159, 1160 preparation of, 325, 327

Subject Index

thermodynamic properties of, 13/0, 1312, 1325

see also Uranyl bromide bromo complexes, 349, 350

stability of, 1499 see also Uranium, complex halides;

Uranyl bromo ... bromoalkoxides, 389 cadmium compounds, 235, 236

magnetic properties of, 1413 thermodynamic properties of, 1330

carbides, 235, 284-7 applications for, 287 crystal structure data for, 281, 1433 hydrolysis of, 284, 287 phase diagram for, 284, 285 physical properties of, 281 preparation methods for, 284, 286 thermodynamic properties of, 1328-9

carbollide complex, 1460-1, 1461 carbon phase diagram, 285 carbonate: see Uranyl carbonate ... carbonato complexes, 1504 chalcogenides, 235, 292-5, 298

crystal structure data for, 296-7 physical properties of, 296-7 thermodynamic properties of, 1326

chelate compounds, 392, 394, 395--6, 395 chelating agents listed for, 395 chlorides, 235


mixed halides, 302-3, 327 physical properties of, 301, 328,329,

1157, 1159, 1160 preparation of 325-7 thermodynamic properties of, 1309, 1312,

1324 see also Uranium, hexachloride; ... ,

pentachloride; ... , tetrachloride; ... , trichloride; Uranyl chloride

chloro complexes, 349, 349, 350 stability of, 1499 see also Uranium, complex halides;

Uranyl chloro ... chloroalkoxides, 389, 389 chlorophenoxides, 393 cobalt compounds, 234, 235, 236, 237, 242 cobalt phase diagram, 242 complex halides, 316-25, 328-32, 340

crystal structure data for, 318-24, 330-1, 1330-/, 1444-7, 1446


magnetic data for, 1365 phase diagrams for, 316, 317 physical properties of, 318-24, 330-1 thermodynamic properties of, 1332, 1333,

1334

complex oxides, 266, 270-3, 276, 279 magnetic properties of, 1368, 1370, 1371 phase diagram for CaO-U02 , 271, 272 physical properties of, 274-5 preparation methods for, 270, 270, 271 thermodynamic properties of, 1299, 1302,

1303, 1304, 1331, 1332, 1333 complex oxyhalides, 335 complexes

hexapositive, 351--68 historical background for U(IV), 347-8 ofU(V), 319, 330-1, 351 ofU(IV), 347-50,351 of U(III), 337, 347

compounds, 235, 248-336 compared with neptunium compounds,

444 see also Uranyl ...

compounds from aqueous solutions, 336--68 of UO~+, 340-7 of UO;, 339--40 of U(IV), 337-9 of U(III), 336-7, 337

concentration in lithosphere of, 1170 concentration in oceans of, 195--6, 1170 copper compounds, 235, 237 core level binding energies, 216 crown ether complexes, 385-7, 1457-8 cycIo-octatetraenyl complexes, 382-3,383,

1168, 1462, 1573-9 cycIopentadienyl complexes, 378-81, 1166,

1167, 1550-2, 1551, 1553--4, 1554, 1555-9,1557, 1560-3, 1566-9

crystal structures of, 379, 380 halo compounds, 380-1, 1553--4, 1555-9,

1556, 1561, 1562 magnetic properties of, 1374-5 reactions of, 379

cycIopentadienyl hydrocarbyl complexes, 1592, 1593, 1593, 1594, 1596-8

decay series (4n + 3), 14, 18, /07 deuteride

crystal structure data for, 251, 1155 Curie temperature for, 253 physical properties of, 1155 rate of formation of, 249 thermodynamic properties of, 1323

diethylamide, 335--6, 387 1,3-diketone chelates, 392, 394, 395 dioxide, 456

crystal structure data for, 267, 1156, 1419 crystal structure of, 260-1, 261 fluorination of, 305--6 hydrofluorination of, 304, 305 magnetic properties of, 1372-3 phase diagram with calcium oxide, 272 phase diagram with phosphorus

pentoxide/water, 377 phase relationships for, 259--60, 260, 266

Subject Index

Uranium (Contd.) physical properties of, 267, 1156 plutonium dioxide mixed oxides, 726-9 thermodynamic properties of, 1162, 1301,

1312, 1321 . dioxide monohalides, 333, 334, 340 I ,3-diphenylpropane-1 ,3-dionato complex,

1456 discovery of, 169 distribution coefficients listed for various

solvents, 520 economics of recovery of, 192, 194-5 electron configurations of, 211, 214, 214,

215,1135, 1203, 1204, 1225-6, 1237, 1238

electron energy level scheme for divalent ion, 1261

electron energy levels for tetravalent ion, 220 for pentavalent ion, 221

electron radial distribution for, 1243 emission spectra of, 212-15 energy level parameters for, 1246, 1247,

1268 ethoxides, 387, 389, 390, 391 ethylenediaminetetraacetato complexes, st,

1513 fluorides, 235, 299-300, 304-16


intermediate fluorides, 301, 306, 307, 308, 309

mixed halides, 302 physical properties of, 301, 1157, 1159,


1323 see also Uranium, hexafluoride; ... ,

pentafluoride; ... , tetrafluoride; ... , trifluoride; Uranyl fluoride

fluoro complexes, 349, 349, 350, 350 stability of, 350, 1498 thermodynamics for formation of, 1501 see also Uranium, complex halides;

Uranyl fluoro ... fluoro 1,3-dicarbonyl chelates, 394,395 fluoroethoxides

amine complexes, 389 physical properties of, 391

formate, 339 free-ion energy level structure for, 1249 gallides, 235


germanides, 1329 crystal structure data for, 281-2 physical properties of, 281-2

germanium compounds, 235, 281-2, 289 global inventory of, 196, 1170

glycollate, structure of, 1454 gold compounds, 235, 236 as gold recovery by-product, 193,207-8 halides, 235, 298-332

applications for, 298 crystal structure data for, 301-2, 312,

329, 1157, 1159, 1160 magnetic properties of, 1367, 1376 mixed halides, 302-3,327-8,1325 physical properties of, 301-2, 312-13,

329, 1157, 1159, 1160 thermodynamic properties of, 1306, 1309,

1310, 1312, 1323-5 vapor pressure relationships for, 312, 329 see also Uranyl halides

halo complexes, 349-50 see also Uranium, complex halides

Hartree-Fock calculations for, 1221, 1223 hexachloride, 301, 327, 328,329

crystal structure data for, 301, 1160, 1440 physical properties of, 301, 1160 thermodynamic properties of, 1324

hexafluoride, 308-16 carbon monoxide reaction with, 314 chemical properties of, 313-15,314 complexes, 318 critical constants for, 312 crystal structure data for, 301, 312, 313,

1160,1440 dielectric constants for, 313 fluorination ability of 313-14 hydrolysis of, 315 infrared/Raman frequencies for, 313 in isotope separation, 173-4, 175-6, 298 magnetic properties of, 313, 1367 in neptunium separation process, 451,

452 optical properties of, 313 in ore concentrate refining, 209, 210, 211 oxidation strength of, 315 phase diagrams for, 315-16, 316 physical properties of, 301, 308, 312-13,

1160· preparation methods for, 309, 310, 311 purification of, 311-12 spectral characteristics of, 1272, 1273 surface tension of, 313 thermal properties of, 312 thermodynamic properties of, 1323 transport regulations (USA) for, 311 triple point of, 308, 312 vapor pressure relationships for, 312 viscosity of, 312

hydration enthalpy for, 1293 hydrides, 235, 248-53, 254

chemical reactions of, 253, 254 crystal modifications, 251-3, 252 crystal structure data for, 251, 1155,

1426-7

Subject Index

electrical properties of, 253, 254 kinetics of formation of, 249 magnetic properties of, 253, 1375 physical properties of, 1155 preparation of, 248-9 pressure--composition isotherm for,

250-1,250 thermodynamic properties of, 251, 1323

hydrolytic behavior of', 337-8, 338, 339, 1141, 1145, 1146

hydroxide activity products of, 1289

2-iminoisoindolinato complexes, 384,385, 386

indenyl complexes, 381-2, 1459,1459, 1563-5, 1564, 1565

indium compound, 235, 238,1330 intermetallic compounds, 233--44 iodides, 235


magnetic properties of, 1376 mixed halides, 302-3, 327 physical properties of, 302, 328,329,

1158,1159 preparation of, 325 thermodynamic properties of, 1311, 1312,

1325 see also Uranyl iodide

iodo complexes, 329,331,332,350 ion-exchange separation of, 203-5, 1089,

1529 ionic radii of, 1165, 1284, 1289, 1448 ionic spectroscopy, 213-15 ionization energies for, 1293 ions in solution, 396-415

absorption spectra for, 218, 219, 221, 222,398,1239,1248,1263,1265

aqueous solvents, 396-9 complexes, 347--68 disproportionation reactions of, 339, 399 hydrolysis of, 1485, 1487-9, 1488 non-aqueous solvents, 399,407-15 oxidation-reduction behavior of, 400--6 oxidation-reduction kinetics for, 1533,

1536 oxidation states listed for, 397 solvent extraction data for, 1519, 1522,

1526 stability of, 1144, 1288 thermodynamic properties of, 1280, 1281,

1284, 1312, 1321 thermodynamics of hydrolysis of, 1496,

1496 iridium compounds, 235, 238

non-magnetic behavior of, 1409 iron compounds, 234, 235, 237,1331

magnetic properties of, 1413 isotope separation methods, 173 -86

chemical separation attempts, 182-3 electromagnetic separation, 177, 180-1 gas centrifuge separation, 181-2 gaseous diffusion process, 174-7,178-9,

180 laser separation, 173-4, 174, 175 liquid thermal diffusion, 181 nozzle process, 182 radioactive decay products, 183--6

isotopes, 171-2,172 decay properties of, 172, 1172, 1657, 1670 production methods listed for, 171-2,

172, 1657 lead compounds, 234, 235, 239, 282, 289

crystal structure data for, 282 physical properties of, 282 thermodynamic properties of, 1330

macrocyclic complexes, 383-5 magnetic data for, 253, 1365, 1367, 1367,

1368, 1372-5, 1376 manganese compounds, 234, 235, 238 mercaptides, 336 mercury compounds, 234, 235, 237, 238,

1331 metal, 222-47

allotropic transformation enthalpies of, 228

allotropic transition temperatures for, 228 alloys, 233-4, 242, 243-4, 243, 247, 453 chemical reactions of, 244-7 corrosion of, 245, 246, 247 crystal modifications, 229-30, 230, 231,

1150, 1391, 1402-3 crystal structure data for, 230, 231, 1150,

1391 Debye temperature for, 228 direct ingot process for, 226 elastic properties of, 229, 1405 electrical properties of, 228, 232-3, 233 hardness of, 228, 1404 irradiation effects in, 247 magnetic susceptibilities of, 232 mechanical properties of, 228, 1404, 1404,

1405 molten-salt electrolysis purification of,

227 oxidation of, 245 phase diagrams for, 242, 243 physical properties of, 226, 227 -8, 228,

1150, 1280, 1281, 1321, 1391, 1396 preparation methods for 223-7, 1401 purification of, 227 reactivity of, 222, 244-7 single crystals, 140 I superconductivity of, 232, 1153, 1394 tensile strength of, 228, 1404 thermal properties of, 228 thermodynamic properties of, 228, 231-2,

1150,1280,1281,1321,1396

Subject Index

Uranium (Contd.) valence-band spectroscopy, 216 vapor pressure relationships for, 228

metallic radii for, 1150, 1450 meta11acycle, 1612-13 methoxides, 387, 391 minerals

acid extraction procedures for, 198-200 arsenate-based, 367, 373--6, 1451, 1453 Belgian Congo ores, 193, 446, 504 Canadian ores, 192-3,504 carbonate-based, 190, 342, 356-7 Chattanooga Shale (USA) deposits, 195 Colorado (USA) ores, 191, 193,504 economic deposits of, 192-4 Elliott Lake (Canada) deposits, 192-3 Erzgebirge (Czechoslovakia) pitchblende,

193-4 geological origins of, 187-8, 189 lignite deposits, 195 low-grade deposits of, 194-6 marine shale deposits, 195 natural chain reactions in, 1170-1 neptunium in, 446 Oklo (Gabon) deposits, 194, 1170-1 phosphate-based, 190, 190,366,369-72,

1451,1453 plutonium in, 446, 504 Rand (South Africa) deposits, 193 Shinkolobwe (Zaire) deposits, 193 silicate-based, 190, 191, 339 uranium content of, 187, 187,504 vanadate-based, 190, 191 Wyoming Basin (USA) deposits, 193, 195 Zaire ores, 193,446,504

molybdenum compounds, 238, 243, 243, 343

molybdenum phase diagram, 243 Mossbauer spectroscopy for, 216-17 naming of, 169 naphthoxides, 390, 392, 393 naturally occurring isotopes, 171, 171 neutron irradiation products, 443, 446 nickel compounds, 234, 235, 239 nitrato complexes, see also Uranyl

nitrato ... nitride halides, 333, 335 nitrides, 235, 289, 291

chemical reactivity of, 291 crystal structure data for, 290, 1437 physical properties of, 290 preparation methods for, 289 thermodynamic properties of, 1327

nitrogen phase diagram, 291 nitrophenoxides, 393 nuclear properties of isotopes, 171-2, 172,

1657, 1670 nuclear spins and moments of, 1648 occurrence in nature of, 187 -96

optical emission spectra of, 212-15 ores

world production statistics for, 1123 see Uranium, minerals

organometallic compounds, 368, 378-87 see also Uranium, arene; ... , cyclo ... ;

Uranocene osmium compounds, 235, 239 oxalates, 337, 337, 339, 1329 oxalato complexes, 350, 351

stability of, 351 see also Uranyl oxalato ...

oxidation -reduction reactions, 4()()--6 oxidation states of, 397, 1139

absorption spectra affected by, 218-21 listed for ions in solution, 397

oxide halides, 333, 334-5 oxides, 235, 256-73, 276, 279-80

chemical reactions of, 279-80, 280 crystal structure data for, 267-9, 1156,

1419-21 crystal structures of, 261, 262 nitrogen oxide reactions of, 280 non-stoichiometric, 259-64, 1162, 1163 phase diagrams with phosphorus oxy-

compounds, 377 phase relationships for, 259-64, 266 physical properties of 266,267-9, 1156 preparation of, 265, 279 ternary oxides with plutonium, 725-9 thermodynamic properties of, 265-6,

1162,1296,1301,1312,1321-3 see also Uranium, complex oxides; ... ,

dioxide; ... , pentoxide; ... , ses-quioxide; ... , trioxide

oxygen phase diagrams, 260, 263, 266 oxyhalides, 332, 333, 334-5

crystal structure data for, 333, 1443 physical properties of, 332, 333 preparation of, 332, 334-5 thermodynamic properties of, 1313, 1323,

1324,1325 oxyhalo complexes, 335 oxyselenide, 296 oxysulfides, 296

crystal structure data for, 296, 1437 oxytelluride, 297, 1326 palladium compounds, 234, 235, 239 pentachlorides, 301,326-7,329

absorption spectra for, 1269, 1270, 1271 crystal structure data for, 301, 1159-60,

1439, 1440 physical properties of, 301, 1159-60 thermodynamic properties of, 1324 thionyl chloride complex, 326-7, 390

pentadienyl complex, 1571-2 pentaftuorides

complexes, 318-9 crystal structure data for, 301, 1159, 1440

Subject Index

disproportionation reactions of, 307, 308, 309

magnetic properties of, 1371-2 physical properties of, 301,1159 preparation of, 306 thermodynamic properties of, 1323 vapour pressure relationships, 308

perchlorate complexes, 350 peroxides, 269


peroxyuranates, 276, 279 phenoxides, 390, 392, 393 phosphates, 339

see also Uranyl phosphates phosphato complexes, 350

stability of, 350, 1505 see also Uranyl phosphato ...

phosphides, 235, 292 crystal structure data for, 290, 1437 magnetic properties of, 293, 294, 295 physical properties of, 290 preparation methods for, 292 thermodynamic properties of, 1327

phthaloeyaninato complexes, 383-4 crystal structure data for, 383 crystal structure of, 384

1to(;omplexes, 368, 378-83; see also Uranium, cyclo ...

platinum compounds, 235, 240 magnetic properties of, 1409, 1410, 1413

plutonium phase diagram, 243, 656, 660 plutonium-oxygen phase diagram, 725, 725 pnictides, 235, 289-92

crystal structure data for, 290 magnetic properties of, 293, 294, 295 physical properties of, 290 preparation methods for, 289, 292 singieo(;rystal production, 292 thermodynamic properties of, 1327-8

polymeric U(IV) species, 1145 polyuranates, 276, 277-8 preparation methods for, 283 pyridine compound, 327, 390 pyrophosphate, 1451 radioactivity of, discovery, 169-70 reduction potentials of, 396, 398, 399, 1142,

1286, 1287 reviews and bibliographies on, 170 rhenium compounds, 235, 240, 343 rhodium compounds, 234, 235, 240 ruthenium compounds, 234, 235, 240 in seawater, 195-6, 1504-5 selenides, 235, 295, 296, 298

crystal structure data for, 296, 1437 physical properties of, 296 thermodynamic properties of, 1326

selenium phase diagram, 299

separation/purification methods, 196-211 acid leaching procedures, 198-200, 1531 acid precipitation processes, 206-7 alkaline precipitation processes, 207 bacterial leaching, 200 calcination operations, 197-8 carbonate leaching, 200-2, 202 clarification of leach solutions, 202-3 flotation methods, 197 gravity separation methods, 197 heap leaching, 199 in situ leaching, 199 ion-exchange procedures, 203-5, 551,

552,553 leaching techniques, 198-203 literature on, 197 monazite sands recovery, 48, 49 neutralization precipitation processes,

206-7 percolation leaching, 199 peroxide precipitation process, 207 precipitation processes, 206-7 preconcentration methods, 197 pressure leaching, 199-200 recovery from leach solutions, 203-11 refining by fluoride volatility processes,

209, 210, 211 refining by solvent extraction, 208, 209 roasting operations, 197-8 solvent extraction processes, 205-6, 208,

393, 399, 413-14, 415, 517, 519 tributyl phosphate process, 208, 209

sequestering agent chelates, 394 sesquicarbide, 284 sesquioxide, thermodynamic properties of,

1296,1322 silicates, 339 silicides, 235, 287-9

crystal structure data for, 281, 1433, 1435 phase diagram for, 288, 288 physical properties of, 281 thermodynamic properties of, 1329

silico-organic compounds, 388, 391-2 silicon phase diagram, 288 silver compounds, 1331 solution chemistry of, 336-68 solvent extraction processes for, 205-6, 208,

399, 413-14, 415, 519 extractants listed for, 415, 517

spectral term analysis for, 213-15 spectroscopic measurements for, 211-21 sulfates, 336-7, 337, 339

magnetic properties of, 1373-4 thermodynamic properties of, 1326 see a/so Uranyl sulfate

sulfato complexes, 349, 350 stability of, 1503 see also Uranyl sulfato ...

sulfides, 235, 292-5

Subject Index

Uranium (Con/d.) crystal structure data for, 296, 1437 phase diagram for, 298 physical properties of, 296 preparation of, 295 thermodynamic properties of, 1326

sulfite, 339 sulfur phase diagram, 298 technetium compounds, 235, 241 tellurides, 235, 295, 297, 298

crystal structure data for, 297, 1437 physical properties of, 297 thermodynamic properties of, 1326

tellurium phase diagram, 300 tetrachloride, 301, 325, 328,329

crystal structure data for, 301, 1159, 1440 magnetic properties of, 1367, 1373 physical properties of, 30 I, 1159 structures of adduct compounds, 1442-3 thermodynamic properties of, 1312, 1324 in isotope separation, 298

tetrafluoride, 304--6 chemical reactions of, 306 complexes, 317,320-3 crystal structure data for, 301, 1159, 1440 in metal purification process, 224, 225 phase diagram with sodium fluoride, 317 physical properties of, 30 I, 306 preparation methods for, 304--6 solubility of, 1500 thermodynamic properties of, 1312, 1323

tetrakis( cyclopentadienyl) physical properties of, 1167 structure of, 1554, 1554

tetramethylenediamino complexes, 1591 thalli de, 235, 24 I, 1330 thenoyltrifluoroacetonato chelates, 394,

413-14 thenoyltrifluoroacetone chelation process

for, 413-14 thiocarbamato complexes, 1455 thiocyanato complexes, 349, 349

magnetic properties of, 1373 stability of, 1514 structure of, 1458 see also Uranyl thiocyanato ...

thiocyanato cyclopentadienyl complex, 1556, 1557

tin compounds, 235, 282, 289 crystal structure data for, 282 physical properties of, 282 thermodynamic properties of, 1329-30

titanium compound, 235, 241 toxicity of, 1184 trialkylsilyloxides, 388, 391-2 trichloride, 300, 301, 325,329


magnetic properties of, 1376

physical properties of, 301, 1157 thermodynamic properties of, 1309, 1324

trifluoride, 299 -300 chemical reactions of, 300 complexes, 324 crystal structure data for, 301, 1157, 1440 magnetic properties of, 1375, 1376 physical properties of, 301, 1157 preparation methods for, 299-300 thermodynamic properties of, 1306, 1323

trioxide crystal modifications, 264, 265 crystal structure data for, 268, 1156, 1421 phase diagram with phosphoric acid/

water, 377 phase relationships for, 266 physical properties of, 268, 1156 thermodynamic properties of, 1321-2

trioxide hydrates crystal structure data for, 269, 1421, 1422 physical properties of, 269 thermodynamic properties of, 1322-3

tris(cyclopentadienyl) alkylideno complexes, 1596-7, 1597

tris(cyclopentadienyl) chloro complex physical properties of, 1167 preparation of, 1555 structure of, 1458, 1555

tris( cyclopentadienyl) derivatives, 1555-9 tris(cyclopentadienyl) fluoro complex, 1459,

1556 tris(cyclopentadienyl) hydrocarbyl com-

plexes, 1592, 1593 tritide, thermodynamic properties of, 1323 valence-band spectroscopy for, 216 vapor-phase spectra of, 220 x-ray emission spectra of, 215 x-ray photoelectron spectroscopic studies

for, 216, 1395, 1396 zinc compounds, 235, 241, 1330

magnetic properties of, 1413 Uranium X, 103

genetic relationships, 106, 110 Uranium Xl' 110

separation of, 124 Uranium X2 , 106, 110

purification of, 123-4 see also Protactinium-234m

Uranium Z, 106, 110 purification of, 123-4 see also Protactinium-234

Uranium-232 isolation process, 183 production methods, 172, 183

Uranium-233, 171-2, 172 fissionability of, 1188 isolation processes, 184--6

hexone process, 184 Interim process, 184

Subject Index

Thorex process, 184-6 production methods, 172, 183

Uranium-234 isolation process, 186 natural abundance of, 171

Uranium-235 discovery of, 417 fissionability of, 171 natural abundance of, 171, 171

Uranium-238, natural abundance of, 171 Uranocene, 382-3, 1168, 1573

bonding in, 1577-9, 1578 crystal structure of, 383 magnetic properties of, 1374 physical properties of, 382 preparation of, 1573 structure of, 382, 383, 1462, 1573, 1574 substituted compounds, 1574-7

Uranyl acetate, 342-3, 345 crystal structure data for, 343 physical properties of, 342-3 thermodynainic properties of, 1329

Uranyl acetato complexes, 353-4, 353, 807 crystal structure of, 354, 354 stability of, 353, 1507, 1508 structure of, 1506 thermodynamics for formation of, 1510

Uranyl acetylacetonato complexes stability of, 1511 structure of, 1455-6

Uranyl amide, 291, 313 Uranyl arsenate, thermodynamic properties

of, 1328 Uranyl arsenato complexes, 362, 368

crystal structure data for, 373--6 hydrogen uranyl arsenate, 365 mineral equivalents of, 367, 373--6 physical properties of, 342, 373--6

Uranyl bromate, 341 Uranyl bromide, 333, 334 Uranyl bromo complexes, 353

stability of, 353, 1499 Uranyl butyrato complexes, stability of, 1508 Uranyl carbonate, 342, 343, 1329

phase diagram with sodium carbonate/water, 359

Uranyl carbonates, ammonium salts, 355, 356, 358

Uranyl carbonato complexes, 354-5, 355-7, 358-9

crystal structure data for, 356-7, 359 crystal structure of, 358, 1450 phase diagram for, 359 physical properties of, 356-7

Uranyl chlorate, 341 Uranyl chloride, 332,333, 340,345 Uranyl chloro complexes, 351, 352, 353

stability of, 351, 353, 1499 thermodynamics for formation of, 352

Uranyl chloroacetato complexes, 353 stability of, 353, 1507, 1508

Uranyl chloropropionato complexes, stability of, 1508

Uranyl chromate, 343 Uranyl citrato complexes, stability of, 1508,

1509 Uranyl complexes, 351-68 Uranyl compounds, 340-7

absorption spectra of, 219, 221, 222 bond lengths (U-O) in, 344,345, 1425 physical properties of, 341-3

Uranyl orown ether complexes, 386, 1458 Uranyl dihydroxide, 345, 1421

see also Uranium, trioxide hydrates Uranyll,3-diphenylpropane-I,3-dionato com

plex, 1456 Uranyl fluoride, 332, 333, 345, 347 Uranyl fluoro complexes, 351, 352, 353

stability of, 351, 353,1498 structure of, 1427 thermodynamic properties of, 352, 1333,

1334 thermodynamics for formation of, 352,

1501 Uranyl formate, 342 Uranyl formato complexes, stability of,

1508 Uranyl glycolato complexes


Uranyl halides, 332, 333, 334 thermodynamic properties of, 1324, 1325

Uranyl hexafluoropentane-2,4-dionato complex,1456

Uranyl hydroxide, 345 see also Uranium trioxide hydrates

Uranyl hydroxyacetato complexes, 353 Uranyl iminodiacetato complexes, stability of,

1516 Uranyl iodate, 341 Uranyl iodide, 333, 334 Uranyl ions

absorption spectrum of, 398 bonding in, 340, 344, 1367, 1425 disproportionation of, 1537, 1537 evidence for existence of, 340, 342, 344 hydrolysis of, 344, 346, 347, 1490-2, 1491,

1492, 1493-5, 1494 magnetic measurements for, 1367 molecular-orbital model for, 928 O-U -0 angle for, 344 oxygen exchange with, 344 Raman spectral frequencies for, 340, 344 solvent extraction data for, 1519, 1520 spectral characteristics of, 1273, 1273 stability of, 1144, 1288 structure of, 344,345, 1424, 1490 thermodynamic properties of, 1321

Subject Index

Uranyl ions (Contd.) thermodynamics of hydrolysis of, 1495,

1496 U-O bond distances in, 344, 345, 1425

Uranyl isobutyrato complexes, stability of, 1508

Uranyllactato complexes, stability of, 1508 Uranyl malato complexes, stability of, 1508 Uranyl maleato complexes, stability of, 1508 Uranyl malonato complexes, stability of, 1508 Uranyl molybdate, 343 Uranyl nitrate, 340, 342, 359, 361-2, 1143

bis(triethyl)phosphato complex, 413, 414 bond length relationships for, 345 crystal structure data for, 342 infrared spectral data for, 364 organic addition compounds, 409, 409 phase diagrams (nitric acid/water), 362, 363 physical properties of, 342 preparation of, 361 solubility in organic solvents, 399,407-12

distribution coefficients quoted, 408 organic amine nitrate effect, 4\0-11 salting-out effect, 409, 410, 411 values quoted, 407

solubility in water of, 364 thermodynamic properties of, 1327

Uranyl nitrato complexes, 351, 353, 362,364, 411-12

Uranyl oxalate, 343 crystal structure data for, 343 physical properties of, 343 thermodynamic properties of, 1329

Uranyl oxalato complexes, 358-9, 360-1 stability of, 1507, 1508

Uranyl oxydiacetato complexes, stability of, 1516

Uranyl phosphates, 365, 368, 369-72 Uranyl phosphato complexes, 353, 362, 368

crystal structure data for, 369-71 hydrogen uranyl phosphate, 365 mineral equivalents of, 366, 369-72 phase diagrams for, 377 physical properties of, 342, 369-71 stability of, 353, 1505

Uranyl phthalato complexes, stability of, 1508 Uranyl polynuclear complexes, 347 Uranyl propionato complexes, stability of,

1507,1508 Uranyl rhenate, 343 Uranyl salicylato complexes, stability of, 1508 Uranyl selenates, 341


Uranyl succinato complexes, stability of, 1508 Uranyl sulfates, 341

crystal structure data for, 341 phase diagram with water, 368, 378


Uranyl sulfato complexes, 351, 352, 352, 353, 368

stability of, 351, 353, 1503 thermodynamics for formation of, 352,

1503 Uranyl superphthalocyanine, 1425, 1426, 1457 Uranyl tartrato complexes, stability of, 1508 Uranyl te\1urate, 342 Uranyl thiocarbamato complexes, structure

of,1455 Uranyl thiocyanato complexes, 353

stability of, 353, 1514 thermodynamics for formation of, 1514,

1515 Uranyl thiodiacetate complexes, stability of,

1516 Uranyl thioglycolato complexes


Uranyl tricarbonato complexes physical properties of, 356-7 structure of, 1504 tetraammonium salt, 355, 356, 358

Uranyl tungstates, 343

Valence-band spectroscopy, 216 Van Arkel(-deBoer) process, 51, 53, 223,

1148,1401 Van Vleck equation, 1361 Vapor-phase spectra, 1196 Volatility properties, as means of chemical

identification, 1630-1

Weak interactions, 1219-20

X-ray photoemission spectroscopy (XPS), 216, 580-1, 1004, 1035

X-ray spectra americium, 899 fermium, 1089, 1090 lawrencium, 1101, 1101 nobelium, \098 plutonium, 580 uranium, 215

Ye\1ow cake (uranium ore concentrate) composition of, 276 production of, 207 refining of, 208

Zachariasen bond length -bond strength relationship, 897, 898, 1425

Zaire, uranium ore, 193 neptunium/plutonium content of, 446

Zeeman interactions, 1214, 1361 Zirconium phosphate ion exchangers, 896-7,

1528, 1529

Fundamental constants

Quantity Symbol Value SI unit Auxiliary value

Speed of light in vacuum c 2.997925 x 108 ms- I Elementary charge e 1.602189 x 10- 19 C Planck constant h 6.626 18 x 10 - 34 Js = 4.13570 x 10- 15 eV s; 1\ = h/21l Avogadro constant NA 6.02204 x 1023 mol- I Atomic mass unit lu 1.660 566 x 10- 27 kg = 931.5016 MeV: mass of l2C = 12 u Electron rest mass me 0.910953 x 10- 30 kg M. = NA·m. = 0.000 548 580u

= 0.5110034 MeV Proton rest mass mp 1.672649 x 10- 27 kg Mp = NA'mp = 1.0072765u

= 938.2796 MeV Neutron rest mass mn 1.674954 x 10- 27 kg Mn = NA'mn = 1.0086650u

= 939.573 1 MeV Faraday constant F 9.64846 x 104 Cmol- I =NA'e Rydberg constant R", 1.097373 x 107 m- I Rooh'c = 13.6058eV

Bohr radius ao 0.529177 x 10- 10 m = oc/41lR"" Electron magnetic moment /le 9.28483 x 10 - 24 Jr l

Proton magnetic moment /lp 1.410617 x 10- 26 JT- I Bohr magneton /lB 9.27408 x 10- 24 JT- I = e'/2' m. (l J T- I = 103 erg gauss-I) Nuclear magneton /IN 5.05082 x 10- 27 JT- I = e'/2'mp Molar gas constant R 8.31441 Jmol- I K- I = 0.082057Iitatmmol- 1 K- I

= 1.987 2 cal mol- I K - I Molar volume of Vrn 0.0224138 m3 mol- 1 = R· To/Po. To = 273.15 K. Po = 1 atm

ideal gas (s.t.p.) Boltzmann constant k 1.380 662 x 10 - 2J JK- I = R/NA; = 8.61735 x 1O- 5 eV K -I;

11k = 11604.5 KeV- 1

Pressure Pa bar kp/m2

1 Pa (Pascal) = 1 N/m2 1 10- 5 1.019716 X 10- 1

1 bar = 106 dyn/cm2 105 1 10.19716 x W 1 kp/m2 = 1 mm H2O 9.80665 0.980665 x 10-4 1 1 at = 1 kp/cm2 0.980665 x 105 0.980665 104

1 atm = 760 Torr 1.01325 x 105 1.01325 1.033227 x 104

1 Torr = 1 mm Hg 133.3224 1.333224 x 10 - 3 13.59510 Ilb/in2 = 1 psi 6.89476 x 103 68.9476 X 10- 3 703.069

Useful conversion factors

Work, energy, beat J kWh kcal Btu MeV

1 J (Joule) = 1 Ws = 2.778 x 10- 7 2.39006 X 10- 4 9.4781 X 10- 4 6.242 X 1012

1 Nm = 107 erg 1 kWh 3.6 x 106 1 860.4 3412.14 2.247 x 1019

1 kcal 4184.0 1.1622 x 10- 3 1 3.96566 2.6117 x 1016

1 Btu 1055.06 2.93071 x 10- 4 0.25164 1 6.5858 x 1Q15 (British thermal unit)

1 MeV 1.602 x 10- 13 4.450 X 10- 20 3.8289 X 10- 17 1.51840 X 10- 16

Molecular energy J/mol em - l/molecule K*/molecule eV/molecule

1 J/mol 1 0.0835935 0.12027 0.0103643 1 em -l/molecule 11.96266 1 1.43879 1.2398 x 10- 4

1 K/molecule 8.31444 0.69503 1 8.6173 x 10- 5

I eV /molecule 96484.6 8065.5 11604.5 1

* Kelvin (temperature unit)

Power kW PS kpm/s kcaljs

IkW = 1Q1 oerg/s 1 1.35962 101.972 0.239006 IPS 0.73550 1 75 0.17579 I kpm/s 9.80665 x 10- 3 0.01333 1 2.34384 x 10 - 3

I kcaljs 4.1840 5.6886 426.650 1

at atm Torr Ib/in2

1.019716 x 10- 5 0.986923 x 10 - 5 0.750062 X 10- 2 145.0378 X 10- 6

1.019716 0.986923 750.062 14.50378 10- 4 0.967841 x 10-4 0.735559 X 10- 1 1.422335 x 10- 3

1 0.967841 735.559 14.22335 1.033227 1 760 14.69595 1.359510 x 10- 3 1.315789 X 10- 3 1 19.33678 X 10- 3

70.3069 x 10 - 3 68.0460 x 10 - 3 51.7149 1

NUCLEAR SPINS AND MOMENTS OF THE ACTINIDES

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